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1.
In Finland the deposition of strontium-89 (90Sr) and strontium-90 (90Sr) has been monitored since the early 1960s. The measured cumulative 90Sr deposition in 1963-2005 is on average 1200 Bq m−2, of which 150 Bq m−2 originates from the Chernobyl accident. Adding to this the deposition in 1945-1962 produces a value of 2040 Bq m−2 for the cumulative deposition in Finland. The nuclear explosion-derived deposition up to 1985 obtained in this study, 1850 Bq m−2, is in good agreement with the zonal 90Sr deposition of 1740 Bq m−2 in the 60°N-70°N latitude band estimated by UNSCEAR. The regional deposition patterns of 89Sr and 90Sr following the Chernobyl accident resemble those of the refractory nuclides such as 239,240Pu and 95Zr. The total deposition of Chernobyl-derived 90Sr in Finland was about 5.3 × 1013 Bq. This activity corresponds to 0.027% of the reactor core inventory and 0.66% of the atmospheric emissions from the accident. The corresponding figures for 89Sr are 4.5 × 1014 Bq, 0.023% and 0.56%, respectively. 相似文献
2.
F. Monna F. van Oort P. Hubert J. Dominik J. Bolte J.-L. Loizeau J. Labanowski J. Lamri C. Petit G. Le Roux C. Chateau 《Journal of environmental radioactivity》2009
An 80-year soil archive, the 42-plot experimental design at the INRA in Versailles (France), is used here to study long-term contamination by 137Cs atmospheric deposition and the fate of this radioisotope when associated with various agricultural practices: fallow land, KCl, NH4(NO3), superphosphate fertilizers, horse manure and lime amendments. The pertinence of a simple box model, where radiocaesium is supposed to move downward by convectional mechanisms, is checked using samples from control plots which had been neither amended, nor cultivated since 1928. This simple model presents the advantage of depending on only two parameters: α, a proportional factor allowing the historical atmospheric 137Cs fluxes to be reconstructed locally, and k, an annual loss coefficient from the plow horizon. Another pseudo-unknown is however necessary to run the model: the shape of historical 137Cs deposition, but this function can be easily computed by merging several curves previously established by other surveys. A loss of ∼1.5% per year from the plow horizon, combined with appropriate fluxes, provides good concordance between simulated and measured values. In the 0–25 cm horizon, the residence half time is found to be ∼18 yr (including both migration and radioactive decay). Migration rate constants are also calculated for some plots receiving continuous long-term agricultural treatments. Comparison with the control plots reveals significant influence of amendments on 137Cs mobility in these soils developed from a unique genoform. 相似文献
3.
A. Tieber H. Lettner P. Bossew A. Hubmer B. Sattler W. Hofmann 《Journal of environmental radioactivity》2009
Cryoconites are airborne sediments which accumulate on the surface of glaciers. In samples of cryoconites a temperate Austrian glacier high activity concentrations of anthropogenic radionuclides were found, which stem from global and Chernobyl fallouts. Radionuclides identified were 137Cs, 134Cs, 238Pu, 239+240Pu, 90Sr, 241Am, 60Co, 154Eu, 207Bi, and 125Sb. 相似文献
4.
R. Khanbilvardi V Shestopalov I. Onishchenko V Bublyas V Gudzenko 《Journal of the American Water Resources Association》1999,35(4):887-898
ABSTRACT: An experimental one-year fieldwork has been conducted in the vicinity of the Chernobyl NPP, within an agricultural watershed, to study the transfer of radionuclides brought into the environment by the disaster of 1986. Presented are results of observation of the washout of 137Cs from the runoff plot both in natural conditions and under artificial rainfalls. Beside traditional hydro-logical methods, new techniques were used allowing to consider microtopographical peculiarities of the runoff plot and their role in the redistribution of radionuclides. The estimate of the annual mass balance for the soil and the radionuclides within the runoff plot has shown that, regardless of significant areal variation of their concentration, the 137Cs washout with the solid runoff resulted from artificial rainfalls amounts to some 1 percent of its reserves in the uppermost 5 cm of the topsoil. The same parameter for the natural runoff is lower by an order of magnitude. Both these factors of self-purification are about two times less than natural radioactive decay of 137Cs. 相似文献
5.
As part of a joint USA/USSR Environmental Agreement to determine the distribution and concentration of Chernobyl radioactivity in the northwest Black Sea area, the sediment from eight stations was collected and analyzed to assess the ability of this material to adsorb radiocaesium. Batch tests were conducted in which Cs-137 tracer was added to mixtures of sediment and bottom water, with contact solutions ranging from 85 Bq ml-1 to 1,760 Bq ml-1. This work was done in an argon atmosphere at 9.5°C, which is the average temperature of the sediment. Isotherms were linear for all cores and distribution ratios (RD) calculated from the slopes of the isotherms ranged from 660 to 1,660 ml g-1. These isotherms fit a simplified Freundlich isotherm. Correlations of RD to a number of sediment parameters describing texture and mineralogy were determined. A close relationship was observed between RD for caesium and the percentage of illite contained in the samples. 相似文献
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An uptake parameter u (L kg−1 d−1) and a loss rate parameter k (d−1) were estimated for the patterns of accumulation and loss of 133Cs by three fish species following an experimental 133Cs addition into a pond in South Carolina, USA. These u and k parameters were compared to similar estimates for fish from other experimental ponds and from lakes that received 137Cs deposition from Chernobyl. Estimates of u from ponds and lakes declined with increasing potassium concentrations in the water column. Although loss rates were greater in the experimental ponds, the times required to reach maximum Cs concentrations in fish were similar between ponds and lakes, because ponds and lakes had similar retentions of Cs in the water column. The maximum Cs concentrations in fish were largely determined by initial Cs concentrations in the water column. These maximum concentrations in fish and the times required to reach these maxima are potentially useful indicators for assessments of risks to humans from fish consumption. 相似文献
8.
Yu. A. Maklyuk A. M. Maksimenko S. P. Gashchak M. D. Bondarkov I. V. Chizhevskii 《Russian Journal of Ecology》2007,38(3):181-189
Between 1986 and 1994, a decrease in nonalimentary 90Sr and 137Cs intake and changes in the accessibility of radionuclides in the soil-plant link of their cycle resulted in a 10-to 100-fold decrease in their specific activity (SA) in the bodies of small mammals inhabiting the Chernobyl zone, and a similar decrease was observed in the radionuclide transition factor (TF) in the soil-animal chain. Between 1995 and 2005, no consistent increase or decrease in SA or TF could be revealed against the background of a combined effect of different physicochemical and ecological factors. It is suggested that subsequent changes in the level of radioactive contamination of small mammals will generally reflect only the dynamics of physical 90Sr and 137Cs decay, but, nevertheless, seasonal and local variations in this level will be significant. 相似文献
9.
Pokarzhevskii A. D. Uspenskaya E. Yu. Filimonova Zh. V. 《Russian Journal of Ecology》2003,34(2):73-79
The contents of 137Cs in the soil, plant, and animal samples collected in the ecosystems of protected areas from the White Sea to the Black Sea in 1999 slightly differ from those in the period between 1980 and 1984. As a result of global fallout after the Chernobyl accident, the content of radioactive cesium in the soil has increased only on the territory of the Biological Station of Moscow State University at the White Sea, whereas that in the litter and plants has increased in virtually all areas studied. The isotope content in animals is actually equal to that recorded between 1980 and 1984. The mobility of 137Cs in the soil–plant link has increased, which may be due to fallout after the accident. The duration of a complete radionuclide cycle in ecosystems decreases from 10 half-life periods in northern regions to 2.5 half-life periods in the southern regions. The Chernobyl disaster has caused no significant changes in the global radioactive background in the European part of the Russian Federation. 相似文献
10.
Mietelski JW Maksimova S Szwałko P Wnuk K Zagrodzki P Błazej S Gaca P Tomankiewicz E Orlov O 《Journal of environmental radioactivity》2010,101(6):488-493
Results are presented for 137Cs, 90Sr and plutonium activity concentrations in more than 20 samples of terrestrial invertebrates, including species of beetles, ants, spiders and millipedes, collected in the highly contaminated area of the Chernobyl exclusion zone. The majority of samples were collected in Belarus, with some also collected in the Ukraine. Three other samples were collected in an area of lower contamination. Results show that seven samples exceed an activity concentration of 100 kBq/kg (ash weight - a.w.) for 137Cs. The maximum activity concentration for this isotope was 1.52 ± 0.08 MBq/kg (a.w.) determined in ants (Formica cynerea). Seven results for 90Sr exceeded 100 kBq/kg (a.w.), mostly for millipedes. Relatively high plutonium activity concentrations were found in some ants and earth-boring dung beetles. Analyses of activity ratios showed differences in transfer of radionuclides between species. To reveal the correlation structure of the multivariate data set, the Partial Least-Squares method (PLS) was used. Results of the PLS model suggest that high radiocesium activity concentrations in animal bodies can be expected mainly for relatively small creatures living on the litter surface. In contrast, high strontium activity concentrations can be expected for creatures which conduct their lives within litter, having mixed trophic habits and a moderate lifespan. No clear conclusions could be made for plutonium. 相似文献