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1.
Ozone (O3), as a harmful air pollutant, has been of wide concern. Safe, efficient, and economical O3 removal methods urgently need to be developed. Catalytic decomposition is the most promising method for O3 removal, especially at room temperature or even subzero temperatures. Great efforts have been made to develop high-efficiency catalysts for O3 decomposition that can operate at low temperatures, high space velocity and high humidity. First, this review describes the general reaction mechanism of O3 decomposition on noble metal and transition metal oxide catalysts. Then, progress on the O3 decomposition performance of various catalysts in the past 30 years is summarized in detail. The main focus is the O3 decomposition performance of manganese oxides, which are divided into supported manganese oxides and non-supported manganese oxides. Methods to improve the activity, stability, and humidity resistance of manganese oxide catalysts for O3 decomposition are also summarized. The deactivation mechanisms of manganese oxides under dry and humid conditions are discussed. The O3 decomposition performance of monolithic catalysts is also summarized from the perspective of industrial applications. Finally, the future development directions and prospects of O3 catalytic decomposition technology are put forward. 相似文献
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3.
分析了反舰导弹射击精度评估领域命中概率与圆概率偏差、命中区域圆概率偏差的分歧,提出了制导概率椭圆偏差和制导概率圆偏差的新概念。将反舰导弹飞行末段雷达导引头波束覆盖区域与打击目标水面舰艇轮廓大小进行了比对,根据比对结果划分为雷达导引头波束完全覆盖、部分覆盖和内嵌于目标三个等级,对应提出了命中概率评估方法、制导概率椭圆偏差评估方法和制导概率圆偏差评估方法。通过反舰导弹对快艇、驱护舰和航母三类目标射击精度评估算例验证了反舰导弹射击精度评估总体方案的全面性和三类方法的适用性。 相似文献
4.
During the summers of 1991–1994, the Environmental Monitoringand Assessment Program (EMAP) sampled 344 lakes throughout thenortheastern United States using a proportional stratified sampling design based on lake size. Approximately one-quarter ofthe 344 lakes were sampled each year (4 years) for totalphosphorus to determine the proportion (and associated95% confidence intervals) of the northeast lake population 1ha (11,076 ± 1,699 lakes) that was in oligotrophic,mesotrophic, eutrophic, or heupereutropic (4 classes) conditionaccording to the total phosphorus criteria of the North AmericaLake Manegement Society. Estimates for the second, third, andfourth yr were developed as cumulative of the previous yrsamples and the current yr samples for the northeast as a wholeand for each of its three ecoregions (4 regions). New confidence intervals were computed for each cumulative yrcondition estimate. This produced a total (4 years × 4classes × 4 regions) of 64 cumulative yr tropic conditionestimates. Confidence intervals for 21% of these estimates didnot shorten with increased sample size. This phenomena raisedquestions about the accuracy of estimates based on cumulativesampling procedures. We explain why and how the phenomenon comesabout with both straight random and proportional randomsampling. Further, we present an example of the effects thisphenomenon has on lake tropic state condition estimates in thenortheastern United States. 相似文献
5.
A baseline for a project consists of estimates of annual emissions of greenhouse gases (GHG) for a given time period without implementing the project. A general three-step process for determining the baseline is suggested. The emission reduction of the project is given by the difference between the baseline and the monitored annual emissions. A preferred method, direct measurement of the emission reduction, is possible for some types of projects. Methods for estimating the annual baseline emissions are not necessary for the latter category, and a definition of this project category is suggested. IPCC Guidelines for National GHG Inventories categorise the emission sources so that only direct emissions from consumption of fuel and feedstock are calculated. There are thus no emission factors for indirect emissions (e.g. electricity consumption or km transported) or emission factors that depend on technology only, independent of consumption of fuel and feedstock. Technology-dependent emission factors may thus need to be developed for estimating indirect emissions and multi-project baselines. Consistency should be sought with the IPCC Guidelines when estimating annual baseline emissions and in monitoring project emissions to ensure comparability with the National Inventories. 相似文献
6.
《环境科学学报(英文版)》2023,35(3):641-649
Exposure to endocrine disruptors (EDCs) could disrupt thyroid hormone homeostasis. However, human epidemiological studies reported inconsistent observations, and scarce information on the effect of a mixture of chemicals. The aim of the present study was to examine the associations of multiple chemicals with thyroid hormones among adults from China. We measured serum levels of thyroid hormones and urinary levels of 11 EDCs, including six phthalate metabolites, bisphenol A (BPA), bisphenol F (BPF), bisphenol S (BPS), perchlorate, and thiocyanate among 177 healthy adults without occupational exposure. Associations of multiple urinary analytes with serum thyroid hormones were examined by performing general linear regression analysis and bayesian kernal machine regression analysis. These EDCs were detected in almost all samples. After adjusting for various covariates, we observed only BPF significantly associated with total thyroxin (TT4) (β=-0.27, 95% confidence interval (CI) [-0.41, -0.14]), total triiodothyronine (TT3) (β=-0.02 95% CI [-0.03, -0.01]), free T4 (fT4) (β=-0.02, 95% CI [-0.03, -0.01]), and free T3 (fT3) (β=-0.04, 95% CI [-0.07, -0.01]), and mono-(2-ethyl-5-oxohexyl) phthalate (MEOHP) and monoethyl phthalate (MEP) positively associated with TT4 (β=0.24, 95% CI [0.01, 0.48]) and fT4 (β=0.02, 95% CI [0.01, 0.04]), respectively. Moreover, we observed significant dose-response relationships between TT4 and the mixture of 11 EDCs, and BPF was the main contributor to the mixture effect, suggesting the priority of potential effect of BPF on disrupting thyroid function under a real scenario of human exposure to multiple EDCs. Our findings supported the hypothesis that human exposure to low levels of EDCs could alter thyroid hormones homeostasis among non-occupational healthy adults. 相似文献
7.
随机模拟在常州运河水质规划中的应用 总被引:1,自引:0,他引:1
以常州运河的水质规划为实例,讨论了确定性水质模型的随机模拟。讨论中引进了主观概率和客观概率的概念,用泰勒级数确定客观概率分布,用可能最大机率法估计主观概率分布,并给出了在实施不同规划方案时的水质概率曲线和水质达标的保证率。计算结果表明,使水质恶化的各种随机因素的作用不容忽视,各种水污染治理措施只能降低水质超标的风险水平。 相似文献
8.
Flamos Alexandros Anagnostopoulos Konstantinos Askounis Dimitris Psarras John Butzengeiger Sonja van der Gaast Wytze 《Mitigation and Adaptation Strategies for Global Change》2004,9(2):103-120
This paper presentse-SEREM (Smart Emission ReductionEstimation Manual), a cost-free, easilyaccessed and updated, web-based manual forestimating emission reductions from Joint Implementation (JI) andClean Development Mechanism (CDM) projects. e-SEREM's main functions arethe selection of a benchmark for a specificproject type in the power or heat sectorand the calculation of the annual andcumulative emission reductions accrued bythis project for its crediting lifetime.e-SEREM was developed in order to test itsapplicability and practicality in assistingproject developers and evaluators toelaborate baselines easily and calculatethe emission credits earned by candidate JIor CDM projects hosted in several countries. 相似文献
9.
南水北调中线不同调水方案下的汉江水华发生概率分析 总被引:1,自引:0,他引:1
为评估南水北调中线工程对汉江中下游水华的影响,从汉江水华的成因机理分析入手,提出了汉江水华发生概率的计算模型.该模型由河流一维水动力学模型、水体富营养化模型以及随机数生成模型组成,它不仅可以模拟汉江水华的发生机理,而且可以对诱发水华的各种因子进行随机抽样组合,从而求出中线调水不同方案实施后汉江水华的发生概率.计算结果表明,在现状情况下汉江水华的发生概率为9.2%,南水北调中线各调水方案(无引江济汉工程)实施后,汉江水华发生的概率将有一定程度的增加,而如果调水方案与引江济汉工程同时兴建将大大减少汉江水华发生的概率.最后提出建议,汉江自身的水污染治理是减少水华发生概率的最根本措施,而丹江口水库和引江济汉工程的联合调度将会减小汉江水华发生的概率. 相似文献
10.
新疆强对流暴雨的气候特征和概率分布模式研究 总被引:9,自引:1,他引:9
应用1980—2001年的6h降水量资料和雨量时程方程,首次给出了新疆地区强对流暴雨的划分标准;分析了强对流暴雨的气候特征、大气环流背景、影响系统、变化趋势和概率分布模式;发现,20世纪90年代强对流暴雨次数有明显的增加,Poisson分布拟合强对流暴雨频率分布尚好,还计算了各地每年(雨季)强对流暴雨发生n次以上的概率。 相似文献