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北京冬季大气颗粒物数浓度的粒径分布特征及来源
引用本文:段菁春,李兴华,谭吉华,柴发合. 北京冬季大气颗粒物数浓度的粒径分布特征及来源[J]. 环境科学研究, 2009, 22(10): 1134-1140
作者姓名:段菁春  李兴华  谭吉华  柴发合
作者单位:中国环境科学研究院,北京,100012;清华大学环境科学与工程系,北京,100084
基金项目:国家重点基础研究发展计划(973)项目,中国博士后科学基金项目,中国环境科学研究院中央级公益性科研院所基本科研业务专项 
摘    要:监测北京市冬季远郊区(密云)、交通道路(北四环)和生活区(清华大学)采样点的CO,NO,NO2,SO2等浓度,同时监测大气细颗粒物(FPs,粒径为0.1~2.5 μm)和超细颗粒物(UFPs,粒径<0.1 μm)的数浓度, 利用正交矩阵因子(PMF)法对FPs和UFPs数浓度的粒径分布特征和来源进行了研究. 结果表明:在远郊区采样点共有4个影响因子, 其中主因子1,4可能与长距离运移有关, 主因子2可能来自1 km外的村庄生活排放, 主因子3为附近铁路机车排放;在交通道路采样点共有3个影响因子, 其中主因子1,3可能均来自机动车排放, 主因子2来自燃煤污染;在生活区采样点共有3个影响因子, 其中,主因子1可能与机动车排放有关, 主因子2,3可能均来自燃煤排放. 

关 键 词:正交矩阵因子分析  超细颗粒物  源解析
收稿时间:2009-01-21
修稿时间:2009-04-10

Size Distribution and Source Apportionment of Atmospheric Particle Number Concentration in Winter in Beijing
DUAN Jing-chun,LI Xing-hu,TAN Ji-hua and CHAI Fa-he. Size Distribution and Source Apportionment of Atmospheric Particle Number Concentration in Winter in Beijing[J]. Research of Environmental Sciences, 2009, 22(10): 1134-1140
Authors:DUAN Jing-chun  LI Xing-hu  TAN Ji-hua  CHAI Fa-he
Affiliation:1.Chinese Research Academy of Environmental Sciences, Beijing 100012, China2.Department of Environmental Science and Engineering, Tsinghua University, Beijing 100084, China
Abstract:Based on monitoring records of CO, NO, NO2, SO2 and particle number concentration collected at a remote site, a roadside site and an urban residential site in Beijing in winter, the size distribution pattern of number concentration of fine particles (FPs, 0.1-2.5 μm) and ultrafine particles (UFPs, <0.1 μm), and their possible sources were examined using the EPA PMF model. At the remote site, four factors were identified. Factors 1 and 4 may be related to long distance transport, factor 2 to village emissions one kilometer away, and factor 3 to nearby locomotive emissions. At the roadside site, three factors were identified, of which factors 1 and 3 may be related to vehicle emissions and factor 2 to emissions from coal combustion. At the urban residential site, three factors were identified, ofwhich factor 1 may be related to vehicle emissions and factors 2 and 3 to emissions from coal combustion. 
Keywords:PMF   ultrafine particle   source apportionment
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