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Source contribution of atmospheric aerosols in Japan by chemical mass balance method
Institution:1. Department of Analytical Chemistry, Faculty of Science and Technology, University of the Basque Country UPV/EHU, P.O. Box 644, 48080 Bilbao, Basque Country, Spain;2. Department of Analytical Chemistry, Faculty of Pharmacy, University of the Basque Country UPV/EHU, P.O. Box 450, 01080 Vitoria-Gasteiz, Basque Country, Spain;3. Department of Plant Biology & Ecology, Faculty of Science and Technology, University of the Basque Country UPV/EHU, P.O. Box 644, 48080 Bilbao, Basque Country, Spain;1. Ocean College of Minjiang University, Fuzhou, 350118, China;2. College of Environment and Resources, Institute of Remote Sensing Information Engineering, Fujian Provincial Key Laboratory of Remote Sensing of Soil Erosion, Fuzhou University, Fuzhou, 350116, China;3. Key Laboratory of Spatial Data Mining & Information Sharing of Ministry of Education, Fuzhou University, Fuzhou, 350116, China;4. Fuzhou Environmental Monitoring Center, Fuzhou, 350001, China;1. State Key Laboratory of Pollution Control and Resources Reuse, School of the Environment, Nanjing University, Nanjing 210023, China;2. Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology (CICAEET), Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control (AEMPC), School of Environmental Sciences and Engineering, Nanjing University of Information Science and Technology, Nanjing 210044, China;3. Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China;1. State Key Laboratory of Metastable Materials Science and Technology, College of Materials Science and Engineering, Yanshan University, Qinhuangdao 066004, PR China;2. School of Resources and Materials, Northeastern University at Qinhuangdao, Qinhuangdao 066004, PR China;3. MOE Engineering Research Center for Brittle Materials Machining, Huaqiao University, Xiamen, 361021, PR China
Abstract:The seasonal variation and regional features of source contributions to atmospheric particulates in Japan were investigated using a Chemical Mass Balance (CMB) method. The elemental concentrations of aerosol particles measured at the nine different National Air Surveillance Network from April 1977 to March 1985 were used in this study. Variations of estimated source contributions were also discussed for various analytical conditions regarding the types of release source and chemical species employed in the CMB analysis.When elements other than indicator elements of the assumed source types were added in the analysis by the CMB method, the contributions of some of source types were strongly affected. Soil source contribution was most significant among the five assumed sources at every site and was elevated in spring every year. On the other hand, the contributions of anthropogenic sources had peaks in early winter.
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