An overview on the processes and technologies for recycling cathodic active materials from spent lithium-ion batteries |
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| Authors: | Xihua Zhang Yongbing Xie Xiao Lin Haitao Li Hongbin Cao |
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| Institution: | 1. National Engineering Laboratory for Hydrometallurgical Cleaner Production Technology, Research Centre for Process Pollution Control and Key Laboratory of Green Process and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, No. 1 Zhongguancun North Second Street, Beijing, 100190, China
2. University of Chinese Academy of Sciences, Beijing, China
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| Abstract: | This paper aims to make an overview on the current status and new tendency for recycling cathodic active materials from spent lithium-ion batteries. Firstly, it introduces several kinds of pretreatment technologies, followed by the summary of all kinds of single recycling processes mainly focusing on organic acid leaching and synergistic extraction. Then, several examples of typical combined processes and industrial recycling processes are presented in detail. Meanwhile, the advantages, disadvantages and prospect of each single process, combined process, as well as industrial recycling processes, are discussed. Finally, based on a novel acidic organic solvent, the authors briefly introduce an environmental friendly process to directly recycle and resynthesize cathodic active material LiNi1/3Co1/3Mn1/3O2 from spent lithium-ion batteries. The preliminary experimental results demonstrated the advantages of low reaction temperature, high separation efficiency and organic solvent cycling and preventing secondary pollution to the environment. This process may be used for large-scale recycling of spent lithium-ion batteries after further study. |
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