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Mapping of tritium emissions using absorption vapour samplers
Authors:Gergely Vodila,Mihá  ly Molná  r,Mihá  ly Veres,É  va Svingor,Istvá  n Futó  ,Istvá  n Barnabá  s,Sá  ndor Kapitá  ny
Affiliation:1. Laboratory of Environmental Studies, Institute of Nuclear Research (ATOMKI) of Hungarian Academy of Sciences, H-4001 Debrecen, Hungary;2. Isotoptech Co. Ltd., Debrecen, Hungary;3. Radioactive Waste Treatment and Disposal Facility, H-2166 Püspökszilágy, Hungary
Abstract:Püspökszilágy Radioactive Waste Treatment and Disposal Facility (RWTDF) is a typical near-surface engineered repository designated to store low- and intermediate-level wastes from various institutes, research facilities and hospitals in Hungary. Two automatic combined 14C–tritium sampling units installed at the facility sample the air 2 m above surface. The one installed near the vaults detects tritium (T) activities two orders of magnitude higher than the far reference sampling unit. To localize the T emissions, 19 small absorption vapour samplers filled with silica gel were settled onto the ground surface. After the saturation of the silica gel, the water was recovered and its T concentration was measured with a low-background liquid scintillation counter. The absorption vapour samplers are cheap, simple and easy-to-use. We present the samplers and the T distribution map constructed from the data, which helps to localize the T emission.
Keywords:Tritium   Absorption vapour sampler   Silica gel   Desorption   Liquid scintillation counting   Npp   Hungary
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