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Source apportionment of PM10 in six cities of northern China
Institution:1. Key Laboratory of Coastal Zone Environmental Processes and Ecological Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences, Yantai, China;2. Key Laboratory of Cities'' Mitigation and Adaptation to Climate Change in Shanghai (China Meteorological Administration), College of Environmental Science and Engineering, Tongji University, Shanghai, China;3. State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing, China;4. University of Chinese Academy of Sciences, Beijing, China;1. Environment Research Institute, Shandong University, Jinan 250100, China;2. Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hung Hom, Kowloon 999077, Hong Kong, China;3. Qingdao Environmental Monitoring Central Station, Qingdao 266003, China;4. Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Abstract:Ambient PM10 was sampled in six northern China cities (Urumqi, Yinchuan, Taiyuan, Anyang, Tianjin and Jinan) from December 1999 to July 2002, and analyzed for 16 chemical elements, two water-soluble ions, total carbon, and organic carbon. In addition, chemical source profiles consisting of the same particulate components were obtained from a number of naturally occurring geological sources (soil dust from exposed lands) and sources of atmospheric particulates resulting from human activities (resuspended dust, cement, coal combustion fly ash, vehicle exhaust, and secondary particles). Ambient and source data were used in a chemical mass balance (CMB) receptor model to determine the major source of PM10 in these six cities. Results of CMB modeling showed that the major source of ambient PM10 in all the cities was resuspended dust. Significant contributions from coal fly ash were also found in all six cities.
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