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Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles
Authors:Weigang Wang  Chao Peng  Chenjuan Deng  Ting Lei  Jun Zheng  Jun Zhao  Dongbin Wang  Zhijun Wu  Lin Wang  Yan Chen  Mingyuan Liu  Jingkun Jiang  Anpei Ye  Maofa Ge
Institution:State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Beijing National Laboratory for Molecular Sciences (BNLMS), CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China;State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China;School of Environment Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China;School of Atmospheric Sciences, Sun Yat-sen University, Zhuhai, Guangdong 519082, China;State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China;7. Key Laboratory for the Physics and Chemistry of Nanodevices, Department of Electronics, School of Electronics Engineering and Computer Science, Peking University, Beijing 100871, China;8. University of Chinese Academy of Sciences, Beijing 100049, China
Abstract:Atmospheric nanoparticles are crucial components contributing to fine particulate matter (PM2.5), and therefore have significant effects on visibility, climate, and human health. Due to the unique role of atmospheric nanoparticles during the evolution process from gas-phase molecules to larger particles, a number of sophisticated experimental techniques have been developed and employed for online monitoring and characterization of the physical and chemical properties of atmospheric nanoparticles, helping us to better understand the formation and growth of new particles. In this paper, we firstly review these state-of-the-art techniques for investigating the formation and growth of atmospheric nanoparticles (e.g., the gas-phase precursor species, molecular clusters, physicochemical properties, and chemical composition). Secondly, we present findings from recent field studies on the formation and growth of atmospheric nanoparticles, utilizing several advanced techniques. Furthermore, perspectives are proposed for technique development and improvements in measuring atmospheric nanoparticles.
Keywords:Corresponding author    Nanoparticle  Measurement techniques  Size distributions  Physical properties  Chemical composition
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