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氨水土壤混合物脱除CO2温室气体的实验研究
引用本文:曾清华,王亦飞,吴颖,于广锁,于遵宏. 氨水土壤混合物脱除CO2温室气体的实验研究[J]. 环境污染治理技术与设备, 2009, 0(9): 1630-1634
作者姓名:曾清华  王亦飞  吴颖  于广锁  于遵宏
作者单位:华东理工大学煤气化教育部重点实验室,上海200237
基金项目:长江学者和创新团队发展计划资助项目(IRT0620)
摘    要:为了脱除CO2温室气体,提出了利用氨水土壤混合物去除CO2的新方法。分别考察了土壤颗粒粒径、CO2初始流量、氨水浓度(质量比)和温度对CO2脱除量和脱除率的影响。实验结果表明,该方法去除CO2的量较土壤物理吸附量和氨水化学吸收量的总和提高了大约15%;随着氨水浓度的增大,CO2的脱除率和脱除量都增大;随着土壤颗粒粒径和CO2初始流量的增大,CO2的脱除率和脱除量都减小;当温度由22℃升高到31℃,CO2的脱除率随着温度的升高而增大,但是继续升高温度到40℃,CO2的脱除率反而下降。

关 键 词:CO2  土壤  氨水

Study on removal of CO2 greenhouse gas by mixture of ammonia and soil
Zeng Qinghua Wang Yifei Wu Ying Yu Guangsuo Yu Zunhong. Study on removal of CO2 greenhouse gas by mixture of ammonia and soil[J]. Techniques and Equipment for Environmental Pollution Control, 2009, 0(9): 1630-1634
Authors:Zeng Qinghua Wang Yifei Wu Ying Yu Guangsuo Yu Zunhong
Affiliation:Zeng Qinghua Wang Yifei Wu Ying Yu Guangsuo Yu Zunhong ( Key Laboratory of Coal Gasification of Ministry of Education, East China University of Science and Technology, Shanghai 200237, China)
Abstract:A new method was proposed for removing CO2 greenhouse gas by using the mixture of ammonia and soil.The effect of soil particle size,CO2 initial flux,ammonia concentration and temperature on CO2 removal capacity and CO2removal efficiencies were investigated respectively.The experimental results show that CO2removal capacity of this method is 15% larger than the sum of soil physical adsorption capacity and ammonia absorption capacity;CO2 removal efficiencies and removal capacity increase with increase of ammonia concentration and decrease with increase of CO2 initial flux and soil particle size ; when the temperatures increase from 22 ℃ to 31 ℃ , the CO2 removal efficiencies increase with the increasing temperatures, and then fall when the temperatures continue to rise to 40 ℃.
Keywords:CO2  soil  ammonia
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