Positive remediation on sedimentary P by combination of capping with calcium hydroxide and oxidation with perhydrol |
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Authors: | Chutian Xu Wei Yue Peirong Sun Shutong Chen Zhengying Wu Nan Xu Li Tang Guangzhou Sheng Dapeng Li |
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Institution: | 1. School of Environmental Science and Engineering, Suzhou University of Science and Technology, Suzhou 215009, China;2. Shanghai Engineering Research Center of Landscape Water Environment, Shanghai 200031, China |
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Abstract: | The capping is called passive remediation because the sedimentary P was released and then immobilized by the capping materials.However,the release depends on the environmental conditions.Therefore,a hypothesis was proposed that the oxidant was used to accelerate sedimentary P release and the capping material was used to capture those released P.It is positive remediation to reduce sedimentary P amount.The results show that soluble reac-tive phosphorus (SRP) concentration in the overlying water and pore water increased and then decreased gradually under the combination of sodium percarbonate (SPC) and Ca(OH)2,similar as that under the capping with single Ca(OH)2.The sedimentary P amount was re-duced considerably and P concentration in the capping layer increased obviously after 60 days,compared with the capping with single Ca(OH)2.All these indicated that oxidation improved the sedimentary P release and the released P was captured and immobilized by the capping material of Ca(OH)2.However,the acceleration of sedimentary P release due to the oxidation is obviously different from the traditional mechanism that the oxic condition in the sediment is favor of the immobilization on sedimentary P.It is attributed to the ox-idizability of ·OH from SPC.The reduction of mobile-P and the increase of Ca-P under the combined use are observed.This is similar as traditional mechanism of oxic condition.It is sure that positive remediation reduced sedimentary P amount,resulting in the decrease of P release risk in a long time. |
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Keywords: | Remediation Eutrophication Internal P control Sediment |
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