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Contrasting cesium dynamics in neighboring deep and shallow warm-water reservoirs
Authors:John E Pinder III  TG Hinton  FW Whicker
Institution:a Department of Biology, Texas Christian University, Ft. Worth, TX 76129, USA
b Institute for Radiation Protection and Nuclear Safety, Cadarache, 13115 France
c Department of Environmental and Radiological Health Sciences, Colorado State University, Fort Collins, CO 80523-1618, USA
Abstract:To measure the long term retention and seasonal dynamics of an initial 4 kg addition of 133Cs into an 11.4-ha, 157,000 m3 reservoir (Pond 4, near Aiken, South Carolina, USA), the concentrations and inventories of 133Cs in the water column were measured at periodical intervals for 522 days following the 1 August, 1999 release. After rapid declines in concentrations and inventories during the first 90 days, the 133Cs concentrations in the water column declined at an average proportional rate of 0.004 d−1. However, there were periods of less rapid and more rapid rates of declines, and these were correlated with periods of increasing and decreasing K concentrations in the water column. The decline rates were less and the K concentrations greater in the winter than in the summer. In the deeper, neighboring monomictic reservoirs of Par Pond and Pond B, a yearly cycle of increasing and decreasing 137Cs concentrations in the water column is driven by anoxic remobilization of Cs from the sediments into a persistent summer hypolimnion. In Pond 4, whose mean depth of 1.6 m is too shallow to support a persistent anoxic hypolimnion, the pattern of yearly dynamics for K and Cs appear to be related to the accumulation and release of these elements from the extensive, seasonal macrophyte communities. The contrasting results between Pond 4 and Pond B suggest that a full appreciation of the relative importance of 1) anoxic remobilization and 2) accumulation and release by macrophytes in these systems remains to be established.
Keywords:137Cs  133Cs  Reservoir  Water column  Sediments  Macrophytes  Remobilization  Typha latifolia  Nymphaea odorata
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