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龙岩大气颗粒物中多环芳烃源识别及污染评价
引用本文:何立芳,章汝平.龙岩大气颗粒物中多环芳烃源识别及污染评价[J].环境科学研究,2008,21(3):7-12.
作者姓名:何立芳  章汝平
作者单位:龙岩学院 化学与材料工程系,福建 龙岩 364000
基金项目:福建省自然科学基金 , 福建省教育厅科研项目
摘    要:采用恒能量同步荧光法,研究了龙岩市区不同功能区冬、春季大气颗粒物中多环芳烃(PAHs)的污染状况和污染来源,并对不同功能区的PAHs含量进行了评价. 结果表明:龙岩市区各功能区大气颗粒物中ρ(PAHs)为278.95~ 718.25 ng/m3,且冬季高于春季. 根据PAHs中一些特征标志物的比值,可判断冬、春季市区内PAHs主要来源于汽车尾气和燃煤污染. 采用苯并[a]芘(BaP)及苯并[a]芘等效致癌浓度(BaPE)来评价3个功能区大气颗粒物中PAHs的污染状况显示,冬季3个功能区苯并[a]芘含量(ρ(BaP))均超过国家标准(10 ng/m3),且ρ(PAHs)均严重超标. 

关 键 词:多环芳烃    恒能量同步荧光    大气颗粒物    污染来源    污染评价
文章编号:1001-6929(2008)03-0007-06
收稿时间:2007/9/12 0:00:00
修稿时间:2007年9月12日

Source Identification and Pollution Evaluation of Polycyclic Aromatic Hydrocarbons in Airborne Particulate
HE Li-fang and ZHANG Ru-ping.Source Identification and Pollution Evaluation of Polycyclic Aromatic Hydrocarbons in Airborne Particulate[J].Research of Environmental Sciences,2008,21(3):7-12.
Authors:HE Li-fang and ZHANG Ru-ping
Institution:Department of Chemistry and Materials Engineering, Longyan College, Longyan 364000, China
Abstract:The pollution state and source of polycyclic aromatic hydrocarbons (PAHs) in airborne particulate were studied using constant-energy synchronous fluorescence spectrometry technique in different function regions in Longyan City in winter and spring, and the pollution evaluation of PAHs in different function regions was made. The total ρ(PAHs) in the airborne particulate ranged from 278.95 to 718.25 ng/m3 in different function regions of Longyan City, andwas higher in winter than in spring. Based on some diagnostic index ratios of PAHs, the PAHs pollution of each function region mainly comes from automobile emission and coal burning pollution in winter and spring. The benzo[a]pyrene (BaP) and benzo[a]pyrene-equivalent carcinogenic concentration (BaPE) was adopted to evaluatethe PAHs pollution state in the airborne particulate of 3 function regions. It was shown that the mass concentration of BaP of 3 function regions in winter washigher than the national air quality standard (10 ng/m3), while the PAHs of each function region in winter were basically in serious excess of standard. 
Keywords:polycyclic aromatic hydrocarbons  constant-energy synchronous fluorescence spectrometry  airborne particulates  pollution source  pollution evaluation
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