首页 | 本学科首页   官方微博 | 高级检索  
     

电晕-介质阻挡协同放电降解连续流丙酮
引用本文:王星敏, 吴潇潇, 何龙斌, 丁社光, 余纯丽. 电晕-介质阻挡协同放电降解连续流丙酮[J]. 环境工程学报, 2018, 12(3): 848-854. doi: 10.12030/j.cjee.201704059
作者姓名:王星敏  吴潇潇  何龙斌  丁社光  余纯丽
作者单位:1.重庆工商大学环境与资源学院, 重庆 400067; 2.催化与功能有机分子重庆市重点实验室, 重庆 400067
基金项目:重庆市社会事业与民生保障科技创新专项 (cstc2015shmszx20003) 重庆市科委应用开发项目 (cstc2014yykfA-5003) 重庆市教委应用基础项目( KJ1400607)
摘    要:利用自制等离子体反应器开展电晕-介质阻挡协同放电降解连续流丙酮研究,利用均匀设计法获得适宜的丙酮降解参数及其相互关联性,通过解析电晕-介质阻挡协同放电机理,结合丙酮降解热力学性能分析,获得影响丙酮降解的主要因素。结果表明:丙酮降解的适宜条件为反应器电压9.60 kV、空气流量1.4 L·min-1、在丙酮气体流量20 mL·min-1的连续流体系下,电晕-介质阻挡协同放电3 min、初始质量浓度为1.807 mg·L-1的丙酮单次循环降解率可达35.01%。解析等离子体放电过程和热力学性质发现,丙酮降解受协同放电活性粒子与反应温度的双重影响。

关 键 词:低温等离子体   协同放电   丙酮   臭氧消耗率

Corona dielectric barrier co-discharges for acetone degradation in a continuous flow
WANG Xingmin, WU Xiaoxiao, HE Longbin, DING Sheguang, YU Chunli. Corona dielectric barrier co-discharges for acetone degradation in a continuous flow[J]. Chinese Journal of Environmental Engineering, 2018, 12(3): 848-854. doi: 10.12030/j.cjee.201704059
Authors:WANG Xingmin  WU Xiaoxiao  HE Longbin  DING Sheguang  YU Chunli
Affiliation:1.College of Environment and Resources, Chongqing Technology and Business University, Chongqing 400067, China; 2.Chongqing Key Lab of Catalysis & Functional Organic Molecules, Chongqing 400067, China
Abstract:A homemade plasma reactor is designed for acetone degradation through corona dielectric barrier co-discharge in a continuous flow. The operation conditions for acetone degradation were carefully optimised using a uniform design method. The results show that the acetone degradation rates could reach 35.01% with the initial concentration of 1.807 mg·L-1, and under an acetone and air gas flow of 20 mL·min-1and 1.4 L·min-1 ,respectively. The corona media barrier co-discharge was carried out for 3 min under 9.60 kV. The factors that induce the acetone degradation are identified based upon the studies on the mechanism of corona dielectric barrier co-discharge and thermodynamic analysis. It concludes that both corona dielectric barrier co-discharges and reaction temperature could affect the degradation of acetone.
Keywords:low temperature plasma  looperative discharge  acetone  ozone consumption rate
本文献已被 CNKI 等数据库收录!
点击此处可从《环境工程学报》浏览原始摘要信息
点击此处可从《环境工程学报》下载全文
设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号