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放电等离子体降解三氯乙烯
引用本文:晏乃强,杨虹,吴祖成,谭天恩,李道棠. 放电等离子体降解三氯乙烯[J]. 环境科学, 2001, 22(3): 11-14
作者姓名:晏乃强  杨虹  吴祖成  谭天恩  李道棠
作者单位:上海交通大学生态与环境工程系,上海, 200240
基金项目:国家自然科学基金资助项目(29576261)
摘    要:采用2种放电方式和2种反应器对三氯乙烯进行降解,脉冲放电和交流放电均对三氯乙烯有较好的降解效果,且电压越高降解率越大.对脉冲放电,当气体停留时间为15s、三氯乙烯初始浓度1350mg/m3、电压42kV时空腔式反应器对三氯乙烯的降解率接近100%;对交流放电,使用32kV的电压可使降解率达98%,且频率越高降解效果越好.与脉冲放电相比,交流放电的功率消耗量大、能量利用率低,且填充式反应器的能量利用率也低于空腔式反应器.对于空腔式反应器,三氯乙烯降解率达80%时所需的脉冲和交流放电能量消耗分别为4.9W·h/m3和116W·h/m3.

关 键 词:放电等离子体  三氯乙烯降解  放电反应器  能量消耗
文章编号:0250-3301(2001)03-04-0001
收稿时间:2000-08-29
修稿时间:2000-08-29

Degradation of Trichloroethylene by Discharge Plasma Process
Yan Naiqiang,Yang Hong,Wu Zucheng,Tan Tianen and Li Daotang. Degradation of Trichloroethylene by Discharge Plasma Process[J]. Chinese Journal of Environmental Science, 2001, 22(3): 11-14
Authors:Yan Naiqiang  Yang Hong  Wu Zucheng  Tan Tianen  Li Daotang
Affiliation:Department of Ecology and Environmental Engineering, Shanghai Jiao Tong University, Shanghai 200240, China.
Abstract:Two types of discharge and two kinds of discharge reactors was employed to decompose trichloroethylene (TCE) in air. The results showed that both pulsed discharge and AC discharge were efficient to the degradation of TCE. Under the pulsed discharge with peak voltage of 42kV, gas resident time of 15s and TCE initial concentration of 1350mg/m3, the degradation efficiency of TCE was close to 100% in the hallow reactor and the higher voltage results in a higher degradation efficiency. For the AC discharge, the degradation efficiency of TCE reached 90% with applied voltage of 30kV. Meanwhile, increasing the applied frequency of AC voltage can enhance the degradation of TCE. The energy consumption for TCE degradation by AC discharge was higher than that by pulsed discharge. The energy consumption for TCE degradation efficiency of 80% by pulsed and AC discharge were 4.9W·h/m3 and 116W·h/m3, respectively. In addition, the energy consumption in the packed reactor was higher comparing with that in the hallow one.
Keywords:discharge plasma  degradation of TCE  discharge reactor  energy consumption
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