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Source identifications of PM10 aerosols depending on hourly measurements of soluble components characterization among different events in Taipei Basin during spring season of 2004
Authors:Chang Shih-Yu  Fang Guor-Cheng  Chou Charles C-K  Chen Wei-Nai
Affiliation:Research Center for Environmental Changes, Academia Sinica, Nankang, Taipei, Taiwan.
Abstract:Continuous measurements of hourly PM10 soluble ions were performed by the in situ IC technology in order to assess the impact of Asian outflows on local air quality. The intensive aerosol observation was carried in Taipei from 11 February 22:00 to 7 April 19:00, 2004. Concentrations of the water-soluble ions (Cl(-), NO(-)(2), NO(-)(3), SO(2-)(4), Na(+), NH(+)(4), K(+), and Ca(2+)) were measured in a total of 3,300 samples. The characteristics of air pollutant events in Taipei Basin were classified as frontal dust, dust, northeast monsoon, south wind and sea/land breeze according to the hourly meteorology and air pollutant concentrations. Factor analysis was conducted based on hourly data for 13 variables to find the group of variables with similar behavior. According to the source characteristics of high loading species, the possible sources of PM10 aerosols in each group were identified. Three to four factors were identified for each event. The total variances of frontal dust, dust, northeast trade, south wind, and sea/land breeze events were explained about 85%, 86%, 76%, 77%, and 80%, respectively, indicating that the identified factors were satisfactory.
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