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洱海入湖河流水体悬浮颗粒物有机碳氮来源特征
引用本文:倪兆奎,王圣瑞,赵海超,焦立新,金相灿.洱海入湖河流水体悬浮颗粒物有机碳氮来源特征[J].环境科学研究,2013,26(3):287-293.
作者姓名:倪兆奎  王圣瑞  赵海超  焦立新  金相灿
作者单位:1.中国环境科学研究院, 环境基准与风险评估国家重点实验室, 北京100012
基金项目:国家自然科学基金项目(U1202235,41103070);国家水体污染控制与治理科技重大专项(2012ZX07102-004)
摘    要:以洱海主要入湖河流水体悬浮颗粒物为研究对象,运用稳定同位素技术,研究了不同季节、不同河流水体悬浮颗粒物中有机碳、氮的来源,探讨了其与流域环境和人类活动之间的关系. 结果表明:①入湖河流水体悬浮颗粒物δ13C的离散程度为夏季<秋季<冬季<春季,变化范围分别为-25.1‰~-16.9‰、-30.0‰~-10.7‰、-20.9‰~-11.0‰和-28.6‰~-14.4‰;δ15N的离散程度为冬季>夏季>春季>秋季,变化范围分别为-0.5‰~8.8‰、5.4‰~10.6‰、3.4‰~7.9‰和6.2‰~8.7‰. ②入湖河流水体悬浮颗粒物有机质的来源,春季以陆源C3植物和自生有机质为主,并且C3植物来源的有机质贡献呈逐渐增大趋势;夏季主要来源于陆源C3植物;秋季仍以陆源C3植物和水生植物的混合来源为主,但水生植物来源有机质比例有所上升;冬季则以陆源C3、C4植物和水生植物来源有机质混合来源为主. ③入湖河流水体悬浮颗粒物中的氮,春季主要来源于土壤流失和水生植物残体,并且土壤流失氮比例逐渐升高;夏季主要来源于土壤流失;秋季来源于土壤流失、化学肥料和水生植物死亡的共同作用;冬季来源于化学肥料、土壤流失和水生植物,并且化学肥料带来的氮比例有所上升. 

关 键 词:悬浮颗粒物    稳定碳氮同位素    季节性变化    来源
收稿时间:2012/7/17 0:00:00
修稿时间:2012/12/8 0:00:00

The Sources of Organic Carbon and Nitrogen of Suspended Particulate Matter in Inflow River of Erhai Lake
NI Zhao-kui,WANG Sheng-rui,ZHAO Hai-chao,JIAO Li-xin and JIN Xiang-can.The Sources of Organic Carbon and Nitrogen of Suspended Particulate Matter in Inflow River of Erhai Lake[J].Research of Environmental Sciences,2013,26(3):287-293.
Authors:NI Zhao-kui  WANG Sheng-rui  ZHAO Hai-chao  JIAO Li-xin and JIN Xiang-can
Institution:1.State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences Beijing 100012, China2.Department of Agricultural Science, Hebei North University, Zhangjiakou 075131, China
Abstract:The sources of organic carbon and nitrogen and the seasonal changes of their suspended particulate matter from inflow river of Erhai Lake were studied by stable isotope techniques. The relationships of the two contents with natural and anthropogenic activities were also discussed. The results showed that ratios of the carbon and nitrogen isotopes of suspended particulate matters were -28.6‰ to -14.4‰ and 3.4‰ to 7.9‰ in spring,-25.1‰ to -16.9‰ and 5.4‰ to 10.6‰ in summer,-30.0‰ to -10.7‰ and 6.2‰ to 8.7‰ in fall, and -20.9‰ to -11.0‰ and -0.5‰ to 8.8‰ in winter, respectively. The seasonal changes of their isotopic compositions were observed in the study area. The C3plants and aquatic plants were mainly the mixed source of the organic matter in spring, and the contribution of C3plants source gradually increased; in summer it mainly came from land-based sources of C3plants; in fall it was still C3plants and aquatic plants mixed source, but the contribution of aquatic source increased; when winter, C4plants mixed into C3and aquatic plants source. The nitrogen source in the spring derived from soil erosion and aquatic plant residue, but the contribution of soil erosion was higher; it mainly came from soil erosion in summer; mixed soil erosion, fertilizer and the death of algae in fall; soil erosion, fertilizer and plant residues were the source and the contribution of nitrogen from fertilizer increased in winter. 
Keywords:suspended particulate matter  stable organic carbon and nitrogen isotope  seasonal changes  source
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