Effects of different sediment fractions on sorption of galaxolide |
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Authors: | Lixia Jin Mengchang He Jinghuan Zhang |
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Institution: | State Key Laboratory of Water Environment Simulation, School of Environment, Beijing Normal University, Beijing 100875, China |
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Abstract: | Sorption isotherms of galaxolide (HHCB) of different fractions from two sediments with different mineral and organic carbon contents were determined to compare HHCB sorption behavior and contribution to the total sorption. The HHCB sorption isotherms that used the batch equilibration method were studied on different sediments of different fractions. The sorption isotherms of 600°C heating fractions were detailed using the linear model, while the other fractions were nonlinear and fitted well with the Freundlich model. The dissolved organic carbon (DOC) removed, NaOH extracted, and 375°C heating fractions showed more nonlinear sorption than the original sediments, which suggested more heterogeneous sorption sites in these fractions. Compared to the original sediments, the 375°C heating fractions had higher carbonnormalized distribution coefficient (K oc) values, indicating a higher sorption affinity for HHCB. Among the different sediment fractions, the contribution of the 600°C heating fractions to the overall sorption were the lowest (< 20%), while the 375°C heating fractions were the highest (up to 85%). |
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Keywords: | galaxolide (HHCB) sorption organic carbon sediment carbon-normalized distribution coefficient (Koc) |
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