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三峡水库水环境中内分泌干扰物TBT的多介质迁移和归趋模拟
引用本文:高俊敏,张科,周彬,金芬,郭劲松,欧阳文娟,赵纯. 三峡水库水环境中内分泌干扰物TBT的多介质迁移和归趋模拟[J]. 环境科学学报, 2015, 35(5): 1350-1357
作者姓名:高俊敏  张科  周彬  金芬  郭劲松  欧阳文娟  赵纯
作者单位:重庆大学 三峡库区生态环境教育部重点实验室, 重庆 400045;重庆大学 三峡库区生态环境教育部重点实验室, 重庆 400045;重庆大学 三峡库区生态环境教育部重点实验室, 重庆 400045;中国农业科学院 农业质量标准与检测技术研究所农产品质量与食物安全重点实验室, 北京 100081;重庆大学 三峡库区生态环境教育部重点实验室, 重庆 400045;中国科学院重庆绿色智能技术研究院水库水环境重点实验室, 重庆 400714;中国科学院重庆绿色智能技术研究院水库水环境重点实验室, 重庆 400714;重庆大学 三峡库区生态环境教育部重点实验室, 重庆 400045
基金项目:国家自然科学基金青年基金(No.21107147);中央高校基本科研业务项目(No.106112012CDJZR210007); 中国科学院水库水环境重点实验室开放研究基金 (No. RAE2014AA04B)
摘    要:运用环境多介质QWASI等量浓度模型模拟了三峡水库水环境中内分泌干扰物TBT在各环境介质中的浓度分布及迁移归趋,同时讨论了三峡水库运行方式对库区水环境中TBT环境行为的影响.结果表明,QWASI模型能够较为合理地给出各个物理化学过程的速率参数,可对TBT在三峡水库这种超大型河道型水库中跨介质间的迁移传输、各环境相分布等作出定性和定量的模拟估计,模型输出结果与实测结果较为吻合.研究表明,三峡水库的运行方式对TBT在库区水环境中沉积物和水相间的迁移转化有重要影响.

关 键 词:三峡水库  TBT  多介质QWASI等量浓度模型  迁移及归趋
收稿时间:2014-06-17
修稿时间:2014-07-14

Simulation of multi-media transfer and fate of TBT in the aquatic environment of the Three Gorges Reservoir
GAO Junmin,ZHANG Ke,ZHOU Bin,JIN Fen,GUO Jingsong,OUYANG Wenjuan and ZHAO Chun. Simulation of multi-media transfer and fate of TBT in the aquatic environment of the Three Gorges Reservoir[J]. Acta Scientiae Circumstantiae, 2015, 35(5): 1350-1357
Authors:GAO Junmin  ZHANG Ke  ZHOU Bin  JIN Fen  GUO Jingsong  OUYANG Wenjuan  ZHAO Chun
Affiliation:Key Laboratory of the Three Gorges Reservoir Region's Eco-Environment, Ministry of Education, Chongqing University, Chongqing 400045;Key Laboratory of the Three Gorges Reservoir Region's Eco-Environment, Ministry of Education, Chongqing University, Chongqing 400045;Key Laboratory of the Three Gorges Reservoir Region's Eco-Environment, Ministry of Education, Chongqing University, Chongqing 400045;Key Lab of Agro-product Quality and safety, Institute of Quality Standards & Testing Technology for Agro-products, Chinese Academy of Agricultural Sciences, Beijing 100081;Key Laboratory of the Three Gorges Reservoir Region's Eco-Environment, Ministry of Education, Chongqing University, Chongqing 400045;Key Laboratory of Reservoir Aquatic Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714;Key Laboratory of Reservoir Aquatic Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714;Key Laboratory of the Three Gorges Reservoir Region's Eco-Environment, Ministry of Education, Chongqing University, Chongqing 400045
Abstract:In the study, the distribution, transfer and fate of the endocrine disruptors TBT in various environmental media of the Three Gorges Reservoir (TGR) water environment were simulated by a multimedia environmental QWASI equivalent model. The impacts of operation mode of TGR on TBT environment behavior were also discussed. The results showed that QWASI model not only gave reasonable rate parameters of various physical and chemical processes, but also made qualitative and quantitative simulation estimates of transfer and distribution for TBT among multimedia in the TGR, a large river-type reservoir. The output of model was basically consistent with the monitoring results. Moreover, the operation mode of the TGR showed an important influence on the environmental behavior of TBT in sediment and water of TGR.
Keywords:Three Gorges Reservoir(TGR)  TBT  multimedia QWASI equivalent model  transfer and fate
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