Aqueous-phase formation of N-containing secondary organic compounds affected by the ionic strength |
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作者姓名: | Yuqi Gan Xiaohui Lu Shaodong Chen Xinghua Jiang Shanye Yang Xiewen Ma Mei Li Fan Yang Yewen Shi Xiaofei Wang |
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作者单位: | 1. Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention,Department of Environmental Science and Engineering,Fudan University;2. Shanghai Institute of Pollution Control and Ecological Security;3. Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Great Bay Area,Southern University of Science and Technology;4. Institute of Mass Spectrometry and Atmospheric Environment,Guangdong Provincial Engineering Research Center for On-line Source Apportionment System of Air Pollution,Jinan University;5. Environmental Monitoring Station of Pudong New District;6. Shanghai Municipal Center for Disease Control&Prevention |
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基金项目: | supported by the National Natural Science Foundation of China (Nos.21976034,42077193,92044301,and21906024); |
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摘 要: | The reaction of carbonyl-to-imine/hemiaminal conversion in the atmospheric aqueous phase is a critical pathway to produce the light-absorbing N-containing secondary organic compounds(SOC). The formation mechanism of these compounds has been wildly investigated in bulk solutions with a low ionic strength. However, the ionic strength in the aqueous phase of the polluted atmosphere may be higher. It is still unclear whether and to what extent the inorganic ions can affect the SOC formation. Here we...
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