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闽西南土壤-水稻系统重金属生物可给性及健康风险
引用本文:林承奇,蔡宇豪,胡恭任,于瑞莲,郝春莉,黄华斌. 闽西南土壤-水稻系统重金属生物可给性及健康风险[J]. 环境科学, 2021, 42(1): 359-367
作者姓名:林承奇  蔡宇豪  胡恭任  于瑞莲  郝春莉  黄华斌
作者单位:厦门华厦学院环境与公共健康学院,厦门 361024;环境监测福建省高校重点实验室,厦门 361024;厦门华厦学院环境与公共健康学院,厦门 361024;华侨大学化工学院,厦门 361021;厦门华厦学院环境与公共健康学院,厦门 361024;华侨大学化工学院,厦门 361021
基金项目:国家自然科学基金项目(21777049);福建省中青年教师教育科研项目(JT180785);福建省高校杰出青年科研人才培育计划项目(MJK2018-31-158)
摘    要:结合简单的生物可给性提取法(SBET)与健康风险评价模型,研究了闽西南农田土壤-水稻系统中重金属的生物可给性及健康风险.结果表明,闽西南农田土壤和稻米中部分重金属已存在富集.土壤中Cd、Zn、Pb和Cu含量分别在32.4%、15.5%、14.1%和12.7%的区域超过农用地土壤污染风险筛选值(GB 15618-2018...

关 键 词:重金属  生物可给性  健康风险  土壤-水稻系统  闽西南
收稿时间:2020-05-23
修稿时间:2020-07-01

Bioaccessibility and Health Risks of the Heavy Metals in Soil-Rice System of Southwest Fujian Province
LIN Cheng-qi,CAI Yu-hao,HU Gong-ren,YU Rui-lian,HAO Chun-li,HUANG Hua-bin. Bioaccessibility and Health Risks of the Heavy Metals in Soil-Rice System of Southwest Fujian Province[J]. Chinese Journal of Environmental Science, 2021, 42(1): 359-367
Authors:LIN Cheng-qi  CAI Yu-hao  HU Gong-ren  YU Rui-lian  HAO Chun-li  HUANG Hua-bin
Affiliation:College of Environment and Public Health, Xiamen Huaxia University, Xiamen 361024, China;Key Laboratory of Fujian Universities for Environmental Monitoring, Xiamen 361024, China;College of Chemical Engineering, Huaqiao University, Xiamen 361021, China; College of Environment and Public Health, Xiamen Huaxia University, Xiamen 361024, China;College of Chemical Engineering, Huaqiao University, Xiamen 361021, China
Abstract:The bioaccessibility and health risks of heavy metals in soil-rice system of southwestern Fujian province were studied by combining a simple bioavailability extraction method (SBET) with a health risk assessment model. The results showed that some heavy metals in the agricultural soils and rice of southwestern Fujian province were enriched. The contents of Cd, Zn, Pb, and Cu were greater than the screening value of soil pollution risk for agricultural land (GB 15618-2018) by 32.4%, 15.5%, 14.1%, and 12.7% in the study areas, respectively. The accumulation ability of heavy metals was different and followed the approximately decreasing order of Cd > Zn > Cu > Ni > Hg > As > Cr > Pb. The bioaccessibility of heavy metals in soils and rice were quite different. The bioaccessibility of each heavy metal in rice was greater than the bioaccessibility of the heavy metals in soil, which indicated that the heavy metals in rice were more easily absorbed by the human body. The comprehensive non-carcinogenic risk index (HI) of heavy metals to adults and children was 2.71 and 4.06, respectively, indicating that there were non-carcinogenic risks. The comprehensive carcinogenic risk index (TCR) of heavy metals to adults and children was 1.42×10-3 and 5.28×10-4, respectively, indicating that there was a carcinogenic risk present. The non-carcinogenic risks were mainly due to As, while the carcinogenic risks were mainly contributed by Cd. The non-carcinogenic risk of children was higher than that of adults, while the carcinogenic risk of children was lower than that of adults. This result may be related to physiological characteristics, exposure period, and dietary intake. The dietary intake route may be the main pathway for heavy metals in the soil-rice system of southwest Fujian province to cause health risks. Therefore, more attention should be paid to the risks of dietary exposure in the risk management of heavy metals.
Keywords:heavy metal  bioaccessibility  health risk  soil-rice system  southwest Fujian Province
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