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红壤丘陵区冬季大气湿沉降化学特征及森林冠层对其截留作用机制
引用本文:郝卓,高扬,张进忠,于贵瑞.红壤丘陵区冬季大气湿沉降化学特征及森林冠层对其截留作用机制[J].环境科学,2015,36(12):4403-4413.
作者姓名:郝卓  高扬  张进忠  于贵瑞
作者单位:西南大学资源环境学院, 重庆 400716;中国科学院地理科学与资源研究所, 生态网络观测与模拟重点实验室, 北京 100101;中国科学院地理科学与资源研究所, 生态网络观测与模拟重点实验室, 北京 100101;西南大学资源环境学院, 重庆 400716;中国科学院地理科学与资源研究所, 生态网络观测与模拟重点实验室, 北京 100101
基金项目:国家自然科学基金项目(31570465);中国科学院秉维优秀青年人才项目(2012RC202)
摘    要:通过对亚热带千烟洲流域的冬季湿沉降化学特征及森林穿透雨进行研究,揭示亚热带流域森林冠层对大气湿沉降中的营养元素(C、N、P、S)及金属元素(K、Ca、Na、Mg、Al、Fe、Mn、Zn)的截留与作用机制.结果表明:1亚热带丘陵区冬季大气湿沉降以酸沉降为主,p H变化范围在3.49~7.0之间,冬季酸沉降离子中以SO_4~(2-)和NO_3~-为主,其月平均沉降通量分别为4.68 kg·hm~(-2)和0.36 kg·hm~(-2),痕量金属元素中以Zn、K、Ca沉降为主,其沉降通量分别为1.72、0.56、0.36 kg·hm~(-2);2森林林冠对溶解性有机碳(DOC)、溶解性总氮(DTN)、总磷(TP)以及痕量元素Ca、Mg、Mn有明显的截留与离释作用,离释百分比达到64.69%、206.75%、301.38%、137.94%、405.25%、1 226.60%;而对Zn、SO2-4具有很好的吸收作用,吸收百分比为73.50%和12.51%,显著降低了亚热带流域冬季酸沉降对土壤生态系统的危害.

关 键 词:红壤  湿沉降  林冠截留  穿透雨  痕量金属
收稿时间:2015/6/29 0:00:00
修稿时间:2015/7/31 0:00:00

Chemical Characteristics of Atmospheric Wet Deposition in Winter and Its Forestry Canopy Interception Mechanism in Red Soil Hilly Area
HAO Zhuo,GAO Yang,ZHANG Jin-zhong and YU Gui-rui.Chemical Characteristics of Atmospheric Wet Deposition in Winter and Its Forestry Canopy Interception Mechanism in Red Soil Hilly Area[J].Chinese Journal of Environmental Science,2015,36(12):4403-4413.
Authors:HAO Zhuo  GAO Yang  ZHANG Jin-zhong and YU Gui-rui
Institution:College of Resources and Environment, Southwest University, Chongqing 400716, China;Key Laboratory of Ecosystem Network Observation and Modeling, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China;Key Laboratory of Ecosystem Network Observation and Modeling, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China;College of Resources and Environment, Southwest University, Chongqing 400716, China;Key Laboratory of Ecosystem Network Observation and Modeling, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China
Abstract:In order to disclose the interception mechanism of forestry canopy to atmospheric wet deposition, the concentrations of nutrients (C, N, P, S) and trace elements (K, Ca, Na, Mg, Al, Fe, Mn, Zn) in wet deposition and through fall in winter were monitored in Subtropical Qianyanzhou basin. The results showed that the wet deposition in this area was mainly acid deposition, the pH of which ranged from 3.49 to 7.0. The major components of wet deposition were nitrate (NO3-) and sulfate ions (SO42-), the monthly average deposition fluxes of which were 4.68 kg ·hm-2 and 0.36 kg ·hm-2, and trace elements (Zn, K, Ca) with monthly average deposition fluxes of 1.72, 0.56 and 0.36 kg ·hm-2, respectively. Non-metallic nutrients such as dissolved organic carbon (DOC), dissolved total nitrogen (DTN), total phosphorus (TP), Ca, Mg and Mn were easy to leach, the dilution rate could reach up to 64.69%, 206.75%, 301.38%, 137.94%, 405.25% and 1226.60%, respectively. Moreover, the Zn and sulfate ion (SO42-) could be well absorbed by forests canopy, the absorption proportions of which were 73.50% and 12.51%, respectively.
Keywords:red soil  wet deposition  canopy interception  through fall  trace metal
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