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沉降除藻协同沉积物覆盖对藻华水体甲烷释放的影响
引用本文:朱琳,于江华,施文卿,易齐涛,曹华勇,蒲寅羽. 沉降除藻协同沉积物覆盖对藻华水体甲烷释放的影响[J]. 环境科学, 2019, 40(9): 4238-4243
作者姓名:朱琳  于江华  施文卿  易齐涛  曹华勇  蒲寅羽
作者单位:南京信息工程大学环境科学与工程学院, 江苏省大气环境监测与污染控制高技术研究重点实验室, 南京 210044,南京信息工程大学环境科学与工程学院, 江苏省大气环境监测与污染控制高技术研究重点实验室, 南京 210044,南京水利科学研究院生态环境研究中心, 南京 210029,安徽理工大学地球与环境学院, 淮南 232001,南京信息工程大学环境科学与工程学院, 江苏省大气环境监测与污染控制高技术研究重点实验室, 南京 210044,南京信息工程大学环境科学与工程学院, 江苏省大气环境监测与污染控制高技术研究重点实验室, 南京 210044
基金项目:国家自然科学基金项目(41701112);南京信息工程大学启动经费项目(20181015)
摘    要:本研究以藻华水体甲烷释放为对象,利用模拟柱培养实验,探究了沉降除藻和沉积物覆盖复合技术对富营养化甲烷释放的影响.结果表明,沉降除藻结合沉积物覆盖处理可有效改善水环境,实现对甲烷释放的控制,但不同覆盖材料的效果存在差异;活性炭效果要优于土壤和沸石.相比于对照体系水体溶解氧(DO)2. 5 mg·L-1和氧化还原电位(ORP)100 m V,沉积物界面ORP -125 m V,沉降除藻协同活性炭覆盖体系中水体DO和ORP分别升高至3. 1 mg·L-1和174 m V,沉积物界面ORP逆转为168 m V,实验期间甲烷释放量相对于对照组减少90. 2%.研究结果在富营养水体甲烷减排方面具有指导性意义.

关 键 词:甲烷  藻华  沉降除藻  沉积物覆盖  氧化还原电位
收稿时间:2018-10-20
修稿时间:2019-03-26

Synergy of Algal Sedimentation and Sediment Capping for Methane Emission Control in Bloom Waters
ZHU Lin,YU Jiang-hu,SHI Wen-qing,YI Qi-tao,CAO Hua-yong and PU Yin-yu. Synergy of Algal Sedimentation and Sediment Capping for Methane Emission Control in Bloom Waters[J]. Chinese Journal of Environmental Science, 2019, 40(9): 4238-4243
Authors:ZHU Lin  YU Jiang-hu  SHI Wen-qing  YI Qi-tao  CAO Hua-yong  PU Yin-yu
Affiliation:Jiangsu Key Laboratory of Atmospheric Environmental Monitoring & Pollution Control, School of Environmental Science & Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China,Jiangsu Key Laboratory of Atmospheric Environmental Monitoring & Pollution Control, School of Environmental Science & Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China,Center for Eco-environmental Research, Nanjing Hydraulic Research Institute, Nanjing 210029, China,School of Earth and Environment, Anhui University of Science and Technology, Huainan 232001, China,Jiangsu Key Laboratory of Atmospheric Environmental Monitoring & Pollution Control, School of Environmental Science & Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China and Jiangsu Key Laboratory of Atmospheric Environmental Monitoring & Pollution Control, School of Environmental Science & Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China
Abstract:This study tested a strategy in simulated column systems to control methane emissions from algal bloom waters using the combined technology of algae sedimentation and sediment capping. The results demonstrated that the synergy of algal sedimentation and sediment capping can effectively improve the water environment and reduce methane emissions; however, the improvement rate differed among capping materials. The use of activated carbon yielded better performance on the water environment improvement and methane emission control than soil and zeolite. Compared with the control system, the dissolved oxygen and redox potential in the water were increased from<2.5 mg·L-1 to 3.1 mg·L-1 and from<100 mV to 174 mV, respectively. In addition, the redox potential in the surface sediment was reversed from -125 mV to 168 mV after algal sedimentation with subsequent activated carbon capping. As a result, methane emissions in the algal sedimentation-activated carbon capping systems were decreased by 90.2% over the incubation period relative to the control system. This study provides useful insights into methane emission control in eutrophic waters.
Keywords:methane  algal bloom  algal sedimentation  sediment capping  redox potential
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