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1.
Measurements of size-resolved particle number concentrations during the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia) field campaign were made at the Gosan super-site, South Korea. In East Asia, dust and precipitation phenomena play a crucial role in atmospheric environment and climate studies because they are major sources and sinks of atmospheric aerosols, especially in the springtime. Total Ozone Mapping Spectrometer (TOMS) Aerosol Index and backward trajectories are analyzed to investigate the spatial and temporal evolution of dust storms. The size distributions between dust and non-dust periods and times with and without precipitation are compared. In order to understand the temporal evolution of the aerosol size distribution during dust and precipitation events, a simple aerosol dynamics model is employed. The model predicted and observed size distributions are compared with the measured data. The results show that the coarse mode particle number concentrations increase by a factor of 10–16 during dust events. During precipitation, however, particles in the coarse mode are scavenged by impaction mechanism. It is found that the larger particles are more efficiently scavenged. The degree of scavenged particle varies depending on the rainfall rate, raindrop size distribution and aerosol size distribution.  相似文献   

2.
The link between the African Monsoon systems and aerosol loading in Africa is studied using multi-year satellite observations of UV-absorbing aerosols and rain gauge measurements.The main aerosol types occurring over Africa are desert dust and biomass burning aerosols, which are UV-absorbing. The abundance of these aerosols over Africa is characterised in this paper using residues and Absorbing Aerosol Index (AAI) data from Global Ozone Monitoring Experiment (GOME) on board ERS-2 and SCanning Imaging Absorption SpectroMeter for Atmospheric ChartograpHY (SCIAMACHY) on board Envisat.Time series of regionally averaged residues from 1995 to 2008 show the seasonal variations of aerosols in Africa. Zonally averaged daily residues over Africa are related to monthly mean precipitation data and show monsoon-controlled atmospheric aerosol loadings. A distinction is made between the West African Monsoon (WAM) and the East African Monsoon (EAM), which have different dynamics, mainly due to the asymmetric distribution of land masses around the equator in the west. The seasonal variation of the aerosol distribution is clearly linked to the seasonal cycle of the monsoonal wet and dry periods in both studied areas.The residue distribution over Africa shows two distinct modes, one associated with dry periods and one with wet periods. During dry periods the residue varies freely, due to aerosol emissions from deserts and biomass burning events. During wet periods the residue depends linearly on the amount of precipitation, due to scavenging of aerosols and the prevention of aerosol emissions from the wet surface. This is most clear over east Africa, where the sources and sinks of atmospheric aerosols are controlled directly by the local climate, i.e. monsoonal precipitation. Here, the wet mode has a mean residue of ?1.4 and the dry mode has a mean residue of ?0.3. During the wet modes a reduction of one residue unit for every 160 mm monthly averaged precipitation was found. Shielding effects due to cloud cover may also play a role in the reduction of the residue during wet periods.A possible influence of aerosols on the monsoon, via aerosol direct and indirect effects, is plausible, but cannot directly be deduced from these data.  相似文献   

3.
Dust storm events and their relation to climate changes in Northern China during the past 1000 years were analyzed by using different paleoclimate archives such as ice cores, tree rings, and historical documents. The results show that in the semiarid region, the temperature and precipitation series were significantly negatively correlated to the dust storm frequency on a decadal timescale. Compared with temperature changes, however, there was a closer correlation between precipitation changes and dust storm events on a centennial timescale. At this timescale, precipitation accounts for 40% of the variance of dust fall variations during the last 1700 years, inferring precipitation control on the formation of dust storms. In the western arid region, both temperature and precipitation changes are important forcing factors for the occurrence of dust storms in the region on a centennial timescale. In the eastern arid region, the relationship between dust storm events and climate changes are similar like in the semiarid region. As a result, the effects of climate change on dust storm events were manifested on decadal and centennial timescales during the last millennium. However, there is a phase shift in the relation between climate change and the dust storm frequency. A 1400 years reconstruction of the strength of the Siberian High reveals that long-term variations of spring Siberian High intensity might provide a background for the dynamic conditions for the frequency of historical dust storm events in Northern China.  相似文献   

4.
The Tibetan Plateau (TP) is an ideal place for monitoring the atmospheric environment of low to mid latitudes. In total 54 soil samples from the western TP were analyzed for major and trace elements. Results indicate that concentrations of some typical “pollution” elements (such as As) are naturally high here, which may cause incorrect evaluation for the source region of these elements, especially when upper continental crust values are used to calculate enrichment factors. Because only particles <20 μm are transportable as long distances, elemental concentrations of this fraction of the TP soils are more reliable for the future aerosol related studies over the TP. In addition, REE compositions of the TP soils are unusual, highly characteristic and can be used as an effective index for identifying dust aerosol from the TP.  相似文献   

5.
A Mt. Geladaindong (GL) ice core was recovered from the central Tibetan Plateau (TP) spanning the period 1940–2005 AD. High-resolution major ion (Na+, K+, Ca2+, Mg2+, Cl?, SO42?, NO3?) time-series are used to investigate variations in atmospheric dust loading through time. The crustal source ions vary seasonally with peaks in dust concentrations occurring during the winter and spring which are consistent with atmospheric dust observations at local meteorological stations. However, both similarities and dissimilarities are displayed between the decadal variation of atmospheric dust in the GL core and dust observation records from meteorological stations, which can be attributed to local environmental effects at the stations. This paper compares the 1980s and 1970s as case periods for low and high atmospheric dust loading, respectively, two periods reflecting shifts in spring atmospheric circulation (a weakening of zonal and meridional winds) from the 1970s (a period of enhanced dust aerosol transportation to central TP) to the 1980s (a period of diminished dust aerosol transportation to central TP), especially a significant decrease of meridional wind speeds in the 1980s. GL ice core dust proxies (Ca2+ and K+) are correlated with Total Ozone Mapping Spectrometer (TOMS) Aerosol Index (AI) data in spring over the TP and in the northwestern China (especially for K+). Thus variability of crustal ions in central TP ice core provides a proxy for reconstructing a history of atmospheric dust loading not only on the TP, but also in northwestern China.  相似文献   

6.
To study the mixing and transformation of Asian dust with pollution in the two dust storms over the northern China in 2006, both TSP and PM2.5 samples were collected at three sites of northern China in addition to the dry deposition samples collected in an episode in Beijing. 23 elements, 15 ions, and 16 PAHs in each sample were analyzed. The two dust storms in northern China were observed in April 8–10 (DS1) and April 16–18 (DS2). Compared to DS2, DS1 was weaker and more polluted with stronger mixing between crustal and pollutant aerosols during their long-range transport. The concentrations of pollution species, e.g. pollution elements, ions, and PAHs were higher in DS1 than that in DS2, while the crustal species showed adverse variation. The correlation between chemical species and Al and between PAH(4) and PAH(5,6) further confirmed the stronger chemical transformation and aerosol mixing in DS1 than that in DS2. Back trajectory and chemical analysis revealed that in DS1 the air masses at Beijing were mostly from southern or southwestern direction at lower altitude with much more pollution, while in DS2 the air masses were mostly from the northwestern and northern direction with dust mainly, which explained why there was a stronger mixing of dust with pollution aerosol in DS1 than that in DS2 over Beijing.  相似文献   

7.
This study applies observational data composed of hourly weather and aerosol to discuss the aerosol characteristics within different weather systems. Based on cluster analysis, spring weather in Taipei Basin 2004 was characterised as five weather systems: humid/low south wind speed, dry cold/high east wind speed, humid cold/east wind, dry cold/northeaster, and northwestern convection wind. Under the humid/low south wind speed and northwestern convection wind systems, there are predominant influences of local vehicle/motor pollutant emissions and secondary pollution on the air quality. Asian dust storms were usually occurred under the weather of dry cold/high east wind speed. The regional air quality is more acceptable during the period of prevalent humid cold/east wind and dry cold/northeaster.  相似文献   

8.
Rainfall is a key link in the global water cycle and a proxy for changing climate; therefore, proper assessment of the urban environment’s impact on rainfall will be increasingly important in ongoing climate diagnostics and prediction. Aerosol optical depth (AOD) measurements on the monsoon seasons of the years 2008 to 2010 were made over four metro regional hotspots in India. The highest average of AOD was in the months of June and July for the four cities during 3 years and lowest was in September. Comparing the four regions, Kolkata was in the peak of aerosol contamination and Chennai was in least. Pearson correlation was made between AOD with climatic parameters. Some changes in the parameters were found during drought year. Temperature, cloud parameters, and humidity play an important role for the drought conditions. The role of aerosols, meteorological parameters, and their impacts towards the precipitation during the monsoon was studied.  相似文献   

9.
Abstract

This study is a part of an ongoing investigation of the types and locations of emission sources that contribute fine particulate air contaminants to Underhill, VT. The air quality monitoring data used for this study are from the Interagency Monitoring of Protected Visual Environments network for the period of 2001–2003 for the Underhill site. The main source-receptor modeling techniques used are the positive matrix factorization (PMF) and potential source contribution function (PSCF). This new study is intended as a comparison to a previous study of the 1988–1995 Underhill data that successfully revealed a total of 11 types of emission sources with significant contributions to this rural site. This new study has identified a total of nine sources: nitrate-rich secondary aerosol, wood smoke, East Coast oil combustion, automobile emission, metal working, soil/dust, sulfur-rich aerosol type I, sulfur-rich aerosol type II, and sea salt/road salt. Furthermore, the mass contributions from the PMF identified sources that correspond with sampling days with either good or poor visibility were analyzed to seek possible correlations. It has been shown that sulfur-rich aerosol type I, nitrate aerosol, and automobile emission are the most important contributors to visibility degradation. Soil/dust and sea salt/road salt also have an added effect.  相似文献   

10.
We used aerosol data from 4 sites along the west coast of the U.S. to evaluate the role of transport, seasonal pattern, chemical composition and possible trends in the marine background aerosol for the Pacific Northwest. For the Crater Lake samples, the data have been segregated using 10 day back isentropic trajectories to evaluate the role of transport. Our analysis of the segregated data indicates that the trajectories can successfully separate “locally influenced” from “marine background” aerosol, but are not able to identify a significant difference in the mean concentrations during marine vs Asian transport pathways.The background marine aerosol has an annual mean and median concentrations of 2.0 and 1.5 μg m−3, respectively, for particles less than 2.5 μm diameter. There is a seasonal pattern in all components of the aerosol mass, with a summer maximum and winter minimum. This pattern is most likely due to the strong seasonal pattern in precipitation, which peaks in winter, combined with enhanced sources in summer. The Crater Lake marine aerosol composition is dominated by organics (∼40% by mass), with smaller contributions from sulfates, mineral dust and elemental carbon. Analysis of the background marine aerosol found no apparent trend since 1988. This is in contrast to results reported by Prospero et al. (J. Geophys. Res. 108 (2003) 4019) for nss-SO42− samples from Midway Island in the North Pacific. Comparison of the mean concentrations for each site shows that the Midway samples are significantly more influenced by Asian industrial sources of sulfur, compared to Crater Lake, which implies a substantial loss of nss-SO42− from Asian sources that occurs during transit across the Pacific to Crater Lake due to precipitation scavenging.  相似文献   

11.
Data on mass-levels of PM10 measured at regional background sites across the Mediterranean Basin, available from Airbase (European Environmental Agency) and from a few aerosol research sites, are compiled. PM10 levels increase from north to south and west to east of the Basin. These variations are roughly coincident with the PM10 African mineral dust load. However, when subtracting the African dust from mean PM10 levels using a consistent methodology, the PM10 background levels are still 5–10 μg m?3 higher in the Eastern Basin (EMB) when compared with those in the Western (WMB), mainly due to the higher anthropogenic and sea spray loads.As regards for the seasonal trends, these are largely driven by the occurrence of African dust events, resulting in a spring-early summer maximum over the EMB, and a clear summer maximum in the WMB, although in this later region the recirculations of aged air masses play an important role. Furthermore, a marked seasonal trend is still evident when subtracting the African dust load. This is characterised by a high summer maximum (driven by low precipitation, high insolation) and a winter minimum (intense synoptic winds).Important inter-annual variations in the dust contribution are detected, more evident in the southern sites. These differences are generally associated with the occurrence of extreme dust events. Generally, the years with higher dust contributions over the EMB correspond with lower contributions over the WMB, and vice versa.The characterization of individual particles, collected in both basins during African dust events, by scanning electron microscopy reveals only slight differences between them. This fact probably reflects the high degree of mixture of mineral dust from different sources before the transport towards the receptor sites.  相似文献   

12.
Concentrations of ions in storm rainwater in Texas have been monitored for each 0.254 mm increment of precipitation. The changes in concentrations have been analyzed to investigate the role of differential rates of scavenging of particulate matter of differing particle size, and especially the major acid and base components. The empirical trend at the onset of rainfall is a chemical fractionation of acids and bases with correspondingly wide pH variations. These results are confirmed by model calculations, which show a significant preferential scavenging of calcium relative to sulfate in the first 10 mm of rainfall, resulting in fractionation of bases and acids from their atmospheric concentrations. Previous studies, using Target Transformation Factor Analysis of ion concentrations in storm precipitation and regional ambient aerosol data, statistically determined the average source for acidic secondary species and alkaline particulate matter. Two types of crustal sources were identified as western and eastern soil dust. In this study, an alternate physical explanation for these two soil dust factors is offered. As a storm progresses, the elements in the local soil dust are fractionated as a result of their differential rates of precipitation scavenging, enriching species predominantly in the fine particle size and depleting elements predominantly in the coarse particle size. This fractionation process results in a single source having different elemental ratios at the beginning and at the end of a rain event. For Austin, Dallas, and Tyler, Texas, the soil dust previously identified as being from eastern sources could, instead, be a fractionated form of the western soil source.  相似文献   

13.
This study is a part of an ongoing investigation of the types and locations of emission sources that contribute fine particulate air contaminants to Underhill, VT. The air quality monitoring data used for this study are from the Interagency Monitoring of Protected Visual Environments network for the period of 2001-2003 for the Underhill site. The main source-receptor modeling techniques used are the positive matrix factorization (PMF) and potential source contribution function (PSCF). This new study is intended as a comparison to a previous study of the 1988-1995 Underhill data that successfully revealed a total of 11 types of emission sources with significant contributions to this rural site. This new study has identified a total of nine sources: nitrate-rich secondary aerosol, wood smoke, East Coast oil combustion, automobile emission, metal working, soil/dust, sulfur-rich aerosol type I, sulfur-rich aerosol type II, and sea salt/road salt. Furthermore, the mass contributions from the PMF identified sources that correspond with sampling days with either good or poor visibility were analyzed to seek possible correlations. It has been shown that sulfur-rich aerosol type I, nitrate aerosol, and automobile emission are the most important contributors to visibility degradation. Soil/dust and sea salt/road salt also have an added effect.  相似文献   

14.
The Chihuahuan Desert region is an important contributor to atmospheric dust loading and transport in North America; however, specific dust sources in this region are poorly characterized. Major dust events frequently are characterized by multiple dust plumes developing nearly simultaneously over a large region. Remote sensing data were used to identify the source locations and associated land cover for the most extreme dust events in the Chihuahuan Desert since 2002. Analysis of infrared channels utilizing brightness temperature differences was used to analyze data from geostationary and polar-orbiting satellites, from which dust sources were determined and located. This methodology was applied to the five dust events in the region that resulted in “hazardous” PM10 levels in Texas per the USEPA’s Air Quality Index. Source locations determined from satellite images were used in conjunction with LANDSAT data and Google Earth? images to determine the corresponding land-surface features. Agricultural lands, playas, and their edges are pointed out as focus areas for dust emission, at least during the most intense events. The 130 dust plume initiation sites were relatively uniformly spaced over the landscape, not clumped into a few “hotspots,” suggesting the role of spatiotemporally random meteorological factors in determining major points of emission within and between dust storms. These findings provide an initial characterization of Chihuahuan Desert dust source locations and establish a baseline for continued research in determining potential locations for future dust outbreaks in the southwestern U.S. and northwestern Mexico.  相似文献   

15.
At urban areas in south Europe atmospheric aerosol levels are frequently above legislation limits as a result of road traffic and favourable climatic conditions for photochemical formation and dust suspension. Strategies for urban particulate pollution control have to take into account specific regional characteristics and need correct information concerning the sources of the aerosol.With these objectives, the ionic and elemental composition of the fine (PM2.5) and coarse (PM2.5–10) aerosol was measured at two contrasting sites in the centre of the city of Oporto, roadside (R) and urban background (UB), during two campaigns, in winter and summer.Application of Spatial Variability Factors, in association with Principal Component/Multilinear Regression/Inter-site Mass Balance Analysis, to aerosol data permitted to identify and quantify 5 main groups of sources, namely direct car emissions, industry, photochemical production, dust suspension and sea salt transport. Traffic strongly influenced PM mass and composition. Direct car emissions and road dust resuspension contributed with 44–66% to the fine aerosol and with 12 to 55% to the coarse particles mass at both sites, showing typically highest loads at roadside. In fine particles secondary origin was also quite important in aerosol loading, principally during summer, with 28–48% mass contribution, at R and UB sites respectively. Sea spray has an important contribution of 18–28% to coarse aerosol mass in the studied area, with a highest relative contribution at UB site.Application of Spatial Variability/Mass Balance Analysis permitted the estimation of traffic contribution to soil dust in both size ranges, across sites and seasons, demonstrating that as much as 80% of present dust can result from road traffic resuspension.  相似文献   

16.
Quantitative information on the contribution of dust storms to atmospheric PM10 (particulate matter with an aerodynamic diameter ≤10 µm) levels is still lacking, especially in urban environments with close proximity to dust sources. The main objective of this study was to quantify the contribution of dust storms to PM10 concentrations in a desert urban center, the city of Beer-Sheva, Negev, Israel, during the period of 2001–2012. Toward this end, a background value based on the “dust-free” season was used as a threshold value to identify potentially “dust days.” Subsequently, the net contribution of dust storms to PM10 was assessed. During the study period, daily PM10 concentrations ranged from 6 to over 2000 µg/m3. In each year, over 10% of the daily concentrations exceeded the calculated threshold (BVt) of 71 µg/m3. An average daily net contribution of dust to PM10 of 122 µg/m3 was calculated for the entire study period based on this background value. Furthermore, a dust storm intensity parameter (Ai) was used to analyze several storms with very high PM10 contributions (hourly averages of 1000–5197 μg/m3). This analysis revealed that the strongest storms occurred mainly in the last 3 yr of the study. Finally, these findings indicate that this arid urban environment experiences high PM10 levels whose origin lies in both local and regional dust events.

Implications:The findings indicate that over time, the urban arid environment experiences high PM10 levels whose origin lies in local and regional dust events. It was noticed that the strongest storms have occurred mainly in the last 3 yr. It is believed that environmental changes such as global warming and desertification may lead to an increased air pollution and risk exposure to human health.  相似文献   


17.
ABSTRACT

Spaceborne sensors allow near-continuous aerosol monitoring throughout the world. This paper illustrates the fusion of Sea-Viewing Wide Field-of-View Sensor (SeaWiFS) and TOMS satellite data with surface observations and topographic data during four extreme aerosol events: (1) the April 1998 Asian dust storm that impacted the west coast of North America, (2) the May 1998 Central American forest fire smoke that impacted eastern North America, (3) the intense fall 1999 northern California fires, and (4) the massive February 2000 Sahara dust storm. During these dust and smoke events, the aerosol was visualized on true color SeaWiFS images as a distinct yellowish dye, the result of the aerosol increasing the reflectance of darker surfaces (ocean and land) and decreasing the reflectance of clouds. TOMS imagery also indicated increased aerosol absorption in the affected areas, while surface monitors measured major reductions in visual range. Fusing these data aids in the determination of the aerosol's spatial, temporal, and optical properties and provides supporting evidence for characterizing what is being visualized as dust or smoke. A 3-dimensional perspective of the events is obtained when incorporating topographic data and provides insight into the vertical properties of the aerosol plumes.  相似文献   

18.
To examine the diversity of chemical and physical properties of aerosol particles, in particular dust, over the North Pacific, aerosols were collected along ∼32°N latitude between 140°E and 170°W longitude aboard the NOAA R/V Ronald H. Brown during the Asian Pacific Regional Aerosol Characterization Experiment (ACE-Asia) in the spring 2001. A total of 11,482 aerosol particles were examined through individual-particle analysis. Results indicate that dust particles over this region were dominated primarily by Si-rich particles, including aluminosilicates that contain Fe. Fe is also present as separate Fe-rich particles. Additional common particle types include Ca- and S-rich particles; many of the later appear to represent soil-derived calcium carbonate and its reaction products whereas the former are predominantly reaction products of sea salt and sulfate. Particles are often aggregates of different types including pollution-derived substances and highly heterogeneous, both internally and externally. Dust particles are non-spherical, having circularities from 1.0 up to 4.5, suggesting the high degree of complexity of particle shape. The majority of dust particles were dominated by particles with median diameters from 0.67 to 1.26 μm. However, dust particles with diameters of 5 μm or even larger do exist associated with those events of dust originated from Asian desert areas. The existence of soot and Fe-rich particles over this region indicates the influence of fossil fuel sources in Asia. Aerosol Fe from both Asian desert and fossil fuel combustion may contribute to the nutrient Fe in the surface waters of the North Pacific basin. Therefore, the transport of Asian dust associated with species of fossil fuel burning in the spring may play an important role in altering the natural composition of aerosols over the North Pacific.  相似文献   

19.
Hourly data of PM10 concentration collected from an air quality-monitoring network has been analyzed over Taiwan from 1994 to 1999. Fourteen sites from 72 monitoring stations were selected to evaluate the spatial and seasonal variations in the regions of north, southwest, south, east and National Park. The selected monitoring sites are located in a suburban environment, except Nantz and Linyuan that are located in industrial areas. Moreover, Yangming and Hengchuen are located in National Park. Spatial and seasonal variations of PM10 concentrations are rather large over Taiwan. Annual average in south is approximately six times higher than in National parks. In northern sites, the highest concentration occurs in March–May, which is attributed to the occurrence of dust storms in arid regions of central Asia and the transport of dust by northeasterly monsoon. A marked seasonal variation of PM10 concentrations can be observed both in southwestern and southern regions. The pattern is characterized by high concentrations in winter and low in summer. Appearance of the highest monthly PM10 concentration in winter of south may be in part due to the lowest number of monthly precipitation days and low temperature, both of which occurred in winter. The frequency of PM10 daily mean concentration for exceeded 150 μg m−3 is 15% during winter in south, which reflects the serious pollution problem there. Monitoring sites in National Park are representatives of remote environments, but the PM10 concentrations are still affected by the dust storms and human activities.  相似文献   

20.
Spaceborne sensors allow near-continuous aerosol monitoring throughout the world. This paper illustrates the fusion of Sea-Viewing Wide Field-of-View Sensor (SeaWiFS) and TOMS satellite data with surface observations and topographic data during four extreme aerosol events: (1) the April 1998 Asian dust storm that impacted the west coast of North America, (2) the May 1998 Central American forest fire smoke that impacted eastern North America, (3) the intense fall 1999 northern California fires, and (4) the massive February 2000 Sahara dust storm. During these dust and smoke events, the aerosol was visualized on true color SeaWiFS images as a distinct yellowish dye, the result of the aerosol increasing the reflectance of darker surfaces (ocean and land) and decreasing the reflectance of clouds. TOMS imagery also indicated increased aerosol absorption in the affected areas, while surface monitors measured major reductions in visual range. Fusing these data aids in the determination of the aerosol's spatial, temporal, and optical properties and provides supporting evidence for characterizing what is being visualized as dust or smoke. A 3-dimensional perspective of the events is obtained when incorporating topographic data and provides insight into the vertical properties of the aerosol plumes.  相似文献   

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