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1.
In the 1960s at Porri?o, Spain, soil from a pesticide factory dump was placed in an uncontrolled land infill during demolition. Since then, organochlorine pesticides have degraded and migrated from their original location. Concentrations of lindane, DDT, dicofol, and related side products or degradation products were determined at depths of 0 to 20, 20 to 60 and 60 to 100 cm along a 300-m transect running between the land infill and a nearby river. Depthwise nonmonotonicities (lowest concentrations of DDT and dicofol were found in the 20- to 60-cm layer) were attributed to the occurrence of several successive spill episodes; in general, concentrations were highest or near-highest in the 0- to 20-cm layer. At the dump site, the analyte contents of the 0- to 20-cm layer were as follows: alpha-hexachlorocyclohexane (alpha-HCH), 25 mg kg-1; beta-HCH, 15 mg kg-1; gamma-HCH (lindane), 1.3 mg kg-1; delta-HCH, 0.5 mg kg-1; DDT, 2.5 mg kg-1; dicofol, 0.05 mg kg-1; DDD+DDE, 2.2 mg kg-1. The alpha-HCH/gamma-HCH ratio was higher than in commercial products, and the DDT/(DDD + DDE) ratio lower, suggesting the degradation of lindane and DDT with time. In general, the concentrations of HCH isomers, DDT, and dicofol fell with increasing distance from the dump site; in particular, the rapid fall in HCH concentrations illustrates the marked immobility of these species in the soil. By contrast, the combined concentration of the DDT degradation products DDD and DDE rose with distance from the dump site, which is attributed to their higher mobility.  相似文献   

2.
The most consumed food samples of cereals (rice, maize and wheat), vegetables (lentil, brinjal, carrot, bean, potato, tomato, onion and chili), fruits (banana, mango and jackfruit), fish (taki, rui, pangas and tilapia), egg (chicken and duck), milk (cow) and meat (chicken, duck, beef and mutton) were collected from some markets of Bogra district northern part of Bangladesh to evaluate the levels of arsenic (As) and associated health risk to the adult’s and child inhabitants. Arsenic is a highly toxic element, and its presence in food composites is a matter of concern to the world scientists. Target hazard quotients (THQs) and target carcinogenic risk were calculated to evaluate the non-carcinogenic and carcinogenic health risk from ingested arsenic. The highest and the lowest mean concentrations of arsenic were noted in the Tilapia fish [(0.94 mg/kg, wet weight (ww)] and beef (0.012 mg/kg, ww). The daily intakes of arsenic via foodstuffs were 1.92 and 3.30 µg/kg-bw/day for rural adults and children and 1.69 and 3.04 µg/kg-bw/day for urban adults and children, respectively. The result shows the highest THQs of arsenic in cereals and vegetables for both the rural and urban inhabitants which exceed the safe limit (>1) indicating that cereals and vegetables are the main food items contributing to the potential health risk. The estimated target cancer risks from ingesting dietary arsenic all exceeded 10?6, indicating increased risk of cancer for adults and children in the study area.  相似文献   

3.
Nile tilapia and Nile perch samples from Lake Victoria were analyzed for lindane (gamma-1,2,3,4,5,6-hexachlorocyclohexane), aldrin (1,2,3,4,10,10-hexachloro-1,4,4a,5,8,8a-hexahydro-1,4:5,8-dimethanonaphthalene), alpha-endosulfan (6,7,8,9,10,10-hexachloro-1,5,5a,6,9,9a-hexahydro-6,9-methano-2,4,3- benzo(e) dioxathiepin-3-oxide), dieldrin (1,2,3,4,10,10-hexachloro-6,7-epoxy-1,4,4a,5,6,7,8,8a-octahydro-1,4,5,8-dimethanonaphthalene), DDE (p,p'-1,1-dichloro-2,2-bis-(4-chlorophenyl)ethylene), and DDT (p,p'-1,1,1-trichloro-2,2-bis-(4-chlorophenyl)ethane). No significant difference (alpha = 0.05) in the residue levels between fish types for lindane, alpha-endosulfan, p,p'-DDE, p,p'-DDT, and dieldrin was observed. The aldrin levels in Nile perch (Lates niloticus) were significantly higher than the levels in Nile tilapia (Oreochromis niloticus). No difference was observed in the distribution of residues in the different parts of Nile tilapia, although a difference for p,p'-DDE was observed in the Nile perch. No significant difference was observed in the average fat content of the tissue of Nile perch and Nile tilapia; however, the distribution of fat was significantly different in the different parts of the fish, with the abdominal portion having the highest amount of fat. There was no correlation observed in this study between fat content and organochlorine concentration. Lower p,p'-DDT residues levels compared with the p,p'-DDE levels observed in this study indicate that DDT is no longer in use. The levels of organochlorine pesticide residues found in fish samples in this study were below the FAO, U.S. FDA, Australian, and German extraneous residue limits and maximum residue limits. The concentration of organochlorine residues in surface water within the Napoleon Gulf of Lake Victoria was below detection limit (0.1 microg L(-1)).  相似文献   

4.
An inventory survey conducted to determine pesticide usage in a sub-catchment of the Nzoia sugarcane belt found a variety of pesticides used in the sub-catchment, which are reported in this paper. Analysis of soil samples from seven fallow experimental field plots left uncultivated for various periods from 3 to 96?months after cultivation with pesticide application indicated persistence of high concentrations of pesticide residues in the soil, with estimated soil half-lives (in years) ranging from 0.72 to 57.75 for organochlorines and from 1.13 to 8.25 for herbicides. The mean water concentrations (in ??g/L) of the pesticide residues in River Kuywa, which flows through the Nzoia Nucleus Estate sugarcane farms, ranged from 0.12 (lindane) to 1.36 (p,p??-DDT) for organochlorines and from 0.14 (atrazine) to 1.75 (diuron) for herbicides during the heavy rains period in August 2008 while the mean sediment concentrations (in ??g/g) ranged from 0.28 (lindane) to 1.87 (endrin) for organochlorines and 0.39 (hexazinone) to 4.61 (alachlor) for herbicides. The mean concentrations of residues in water during the light rain period in December 2008 ranged from 0.17 (p,p??-DDT) to 0.71 (aldrin) for organochlorines and 0.01 (atrazine) to 1.74 (alachlor) for herbicides while the sediment concentrations ranged from 0.38 (p,p??-DDT) to 1.145 (aldrin) for organochlorines and 0.74 (atrazine) to 1.98 (alachlor) for herbicides. Although DDT, aldrin, dieldrin, and endrin were not reported in the survey, their presence in the fallow experimental field plot soils and in River Kuywa water and sediment could indicate previous application, lack of recorded data or illegal usage since 1997 when they were banned. Notably, the concentrations of alachlor, diuron, cypermethrin, and hexazinone in the water column were substantial indicating their extensive usage and residual persistence in the sub-catchment, with subsequent wash-off and leaching into River Kuywa. The concentration levels of some of the individual pesticides exceeded the EU limit requirements for drinking water and indicated potential risk to humans and cattle if the water is used without treatment.  相似文献   

5.
2 were sampled in order to verify the impact of these problems on groundwater. All samples were analyzed for major ions, and about 30 of them for fecal coliforms and heavy metals. Nineteen samples were selected for pesticide analyses. The average nitrate content was 80 mg/liter, eight times the regional background value. Fecal coliforms were detected in 60% of the analyzed samples. Zinc content and a high Cl/HCO3 ratio were observed in the surroundings of the solid waste disposal area. Moreover, lindane and heptachlor pesticides were detected in ten samples.  相似文献   

6.
Sediments may act as both a carrier for and a potential source of contaminants such as toxic organics in aquatic environments. This study investigated the spatial distribution of the pesticide DDT [1,1, 1-trichloro-2,2-bis(p-chlorophenyl)ethane] in sediments from the Cedar and Ortega Rivers located in the lower St. Johns River basin, Florida, USA, using field measurements and three-dimensional kriging analysis. High DDT concentrations were found near the junction of the Cedar and Ortega Rivers and at the north end of the Ortega River in the upper 0.5 m of the sediments, indicating that the sediment was enriched with DDT in the top layer although use of this chlorinated compound was banned in 1972. Further study revealed that the influence of sediment grain size or texture on DDT contamination was negligible in this river system and no linear correlations existed among DDT and its metabolites such as DDD [1,1-dichloro-2,2-bis(p-chlorophenyl)ethane] and DDE [1,1-dichloro-2,2-bis(p-chlorophenyl)ethylene]. Comparison of three-dimensional distribution of DDT content to the Florida sediment quality assessment guideline or probable effect level (PEL) showed several "hot spots" in the Ortega River sediments, where DDT contents exceeded the PEL value of 4.78 microg kg(-1). Such contamination may pose a significant hazard to aquatic life.  相似文献   

7.
We analyzed the changes in pesticide use and risk in the Province of Ontario, Canada, from 1973 to 1998 to monitor the success of Food Systems 2002, a program to reduce pesticide use by 50%. Pesticide risk was calculated by multiplying the amount of pesticide used (kilograms of active ingredient) by the Environmental Impact Quotient (EIQ), a score for the potential risk of pesticides to farmworkers, consumers, and the environment. Pesticide use increased by 46% from 1973 to 1983. From 1983, the baseline year for Food Systems 2002, to 1998, pesticide use decreased by 38.5% and risk declined 39.5%. The reductions in pesticide use and risk were primarily on corn (Zea mays L.) and tobacco (Nicotiana tabacum L.), the crops with the highest pesticide use in 1983. Total pesticide use on soybean [Glycine max (L.) Merr.] did not change, but the mean application rate (kg ha(-1)) decreased by 57%. Corn and soybean account for 65% of pesticide use, but have a relatively low pesticide use and risk per hectare and per tonne of production. Total pesticide use on tobacco, fruits, and vegetables was lower than on corn or soybean, but the pesticide use and risk per hectare were much higher. Small reductions in pesticide use on corn and soybean may allow a 50% reduction in pesticide use, but greater reductions in risk can be achieved by reducing the use of "high risk" pesticides on fruit and vegetables.  相似文献   

8.
ABSTRACT: A hydroelectric lake on the Oconee River in central Georgia was sampled on a quarterly basis for four years to determine the impact of three insecticides on the pesticide loading of fish. The insecticides carbofuran (2,3,-dihydro-2,2-dimethyl-7-benzofuranyl methyl-carbamate), fenvalerate [cyano(3-phenoxyphenyl)methyl 4-chloro alpha (1-methylethyl)benzeneacetate], and azinphosmethyl [0,0-Dimethyl S-(4-oxo-1,2,3-benzotriazin-3-(4H)-ylmethyl phosphorodithioate] were used to control cone and seed insects on a pine seed orchard that is adjacent to Lake Oconee. Fish populations in areas of the lake that receive runoff from treated and untreated portions of the seed orchard were sampled using gill nets. Water and fish samples were collected monthly in 1981–1983 and quarterly in 1984. Species collected included carp (Cyprinus carpio), sucker (Catostomus spp., Erimyzon spp., Moxostoma spp., Minytrema spp.), bass (Micropterus spp.), channel catfish (Ictalurus punctatus), spotted gar (Lepisosteus spp.), and bluegill sunfish (Lepomis macrochirus). Few carbofuran residues (< 7 percent of fish samples contained detectable residues) and no azinphosmethyl or fenvalerate residues were detected despite measured inputs into the lake after insecticide application. Persistent agricultural insecticides including dieldrin, lindane, DDT, and toxaphene were detected in 32, 36, 58, and 83 percent of sampled fish, respectively. Screening for 20 other insecticides resulted in no detection of residues at a detection limit of 30–100 μg kg-1.  相似文献   

9.
A human health assessment of hazardous air pollutants in Portland, OR   总被引:1,自引:0,他引:1  
Ambient air samples collected from five monitoring sites in Portland, OR during July 1999 to August 2000 were analyzed for 43 hazardous air pollutants (HAP). HAP concentrations were compared to carcinogenic and non-carcinogenic benchmark levels. Carcinogenic benchmark concentrations were set at a risk level of one-in-one-million (1x10(-6)). Hazard ratios of 1.0 were used when comparing HAP concentrations to non-carcinogenic benchmarks. Emission sources (point, area, and mobile) were identified and a cumulative cancer risk and total hazard index were calculated for HAPs exceeding these health benchmark levels. Seventeen HAPs exceeded a cancer risk level of 1x10(-6) at all five monitoring sites. Nineteen HAPs exceeded this level at one or more site. Carbon tetrachloride, 1,3-butadiene, formaldehyde, and 1,1,2,2-tetrachloroethane contributed more than 50% to the upper-bound lifetime cumulative cancer risk of 2.47x10(-4). Acrolein was the only non-carcinogenic HAP with hazard ratios that exceeded 1.0 at all five sites. Mobile sources contributed the greatest percentage (68%) of HAP emissions. Additional monitoring and health assessments for HAPs in Portland, OR are warranted, including addressing issues that may have overestimated or underestimated risks in this study. Abatement strategies for HAPs that exceeded health benchmarks should be implemented to reduce potential adverse health risks.  相似文献   

10.
Occupational exposure limits (OELs) developed by authorities play a key role in the implementation of programs to protect workers against hazardous chemicals. Unfortunately, many hazardous substances do not have OELs or the OEL could be outdated. To assure the health of the workers, it is therefore useful for companies to develop corporate OELs. An inhouse strategy will be presented hereafter. Expertise in toxicology, industrial hygiene, and occupational health should be available within the company and clear selection criteria for substances are needed. A corporate OEL is only developed for hazardous substances (e.g., carcinogenic or reprotoxic) with a high potential for worker exposure when an appropriate national OEL or threshold limit value is not available. The methodology to calculate corporate OELs is based on the existing methods for national or community OELs and also on the guidance from the European Union's (EU) regulation on the Registration, Evaluation, Authorisation and Restriction of Chemicals (REACH). For carcinogenic substances with a nonthreshold mode of action, there is always a residual chance that a cancer develops even when the exposure of workers is low. To establish an OEL for these substances, the “German traffic light model” is recommended. It is pragmatic, defines an unacceptable, tolerable, and acceptable risk level when workers are exposed to these substances, and determines risk management for exposure reduction. Overall, the professional practice to develop OELs is a good example of corporate leadership to proactively protect the health of workers.  相似文献   

11.
ABSTRACT: Bed sediments of the San Joaquin River and its tributaries were sampled during October 7–11, 1985, and analyzed for organochiorine pesticide residues in order to determine their areal distribution and to evaluate and prioritize needs for further study. Residues of DDD, DDE, DDT, and dieldrin are widespread in the fine-grained bed sediments of the San Joaquin River and its tributaries despite little or no use of these pesticides for more than 15 years. The San Joaquin River has among the highest bed-sediment concentrations of DDD, DDE, DDT, and dieldrin residues of major rivers in the United States. Concentrations of all four pesticides were correlated with each other and with the amount of organic carbon and fine-grained particles in the bed sediments. The highest concentrations occurred in bed sediments of westside tributary streams. Potential tributary loads of DDD, DDE, DDT, and dieldrin to the San Joaquin River were computed from bed-sediment concentrations and data on streamfiow and suspended-sediment concentration in order to identify the general magnitude of differences between streams and to determine study priorities. The estimated loads indicate that the most important sources of residues during the study period were Salt Slough because of a high load of fine sediment, and Newman Wasteway, Orestimba Creek, and Hospital Creek because of high bed-sediment concentrations. Generally, the highest estimated loads of DDD, DDE, DDT, and dieldrin were in Orestimba and Hospital Creeks.  相似文献   

12.
Relative cancer risks of chemical contaminants in the great lakes   总被引:1,自引:0,他引:1  
Anyone who drinks water or eats fish from the Great Lakes consumes potentially carcinogenic chemicals. In choosing how to respond to such pollution, it is important to put the risks these contaminants pose in perspective. Based on recent measurements of carcinogens in Great Lakes fish and water, calculations of lifetime risks of cancer indicate that consumers of sport fish face cancer risks from Great Lakes contaminants that are several orders of magnitude higher than the risks posed by drinking Great Lakes water. But drinking urban groundwater and breathing urban air may be as hazardous as frequent consumption of sport fish from the Great Lakes. Making such comparisons is difficult because of variation in types and quality of information available and in the methods for estimating risk. Much uncertainty pervades the risk assessment process in such areas as estimating carcinogenic potency and human exposure to contaminants. If risk assessment is to be made more useful, it is important to quantify this uncertainty.  相似文献   

13.
Heavy metals in suburban soils pose both indirect and direct health risks. This study assessed the concentrations of Cr, Zn, Pb, and Cd in Jengka (Malaysia) suburban soil and estimated the human health risk. Health risk assessment (HRA) was utilized to assess non-cancer and cancer risks. The concentrations of heavy metals increased in the following order: Cd < Zn < Cr < Pb. The heavy metals were found to be divided into two components using principal component analysis (PCA), with PC1 comprising Pb and Cd and PC2 containing Zn and Cr. PC1 originates from anthropogenic sources, while PC2 is often from mixed anthropogenic and natural sources. Despite having the lowest mean concentration, Cd was enriched based on the geo-accumulation index (Igeo) and enrichment factor (EF). Average hazard index values were below the acceptable threshold (HI < 1) for dermal and inhalation pathways suggesting a low non-cancer risk. Jengka suburban soil had total lifetime cancer risk values slightly higher than the acceptable threshold (1 × 10−5). Skin contact was the most prominent contributing exposure pathway for both non-carcinogenic and carcinogenic risks. This study suggests that heavy metal bioactivity levels be used to make a plausible HRA of heavy metal pollution in suburban soils.  相似文献   

14.
Pesticide risk mitigation by vegetated treatment systems: a meta-analysis   总被引:2,自引:0,他引:2  
Pesticides entering agricultural surface waters threaten water quality and aquatic communities. Recently, vegetated treatment systems (VTSs) (e.g., constructed wetlands and vegetated ditches) have been proposed as pesticide risk mitigation measures. However, little is known about the effectiveness of VTSs in controlling nonpoint source pesticide pollution and factors relevant for pesticide retention within these systems. Here, we conducted a meta-analysis on pesticide mitigation by VTSs using data from the scientific literature and the European LIFE ArtWET project. Overall, VTSs effectively reduced pesticide exposure levels (i.e., the majority of pesticide retention performances was >70%). A multiple linear regression analysis of 188 retention performance cases identified the two pesticide properties, organic carbon sorption coefficient value and water-phase 50% dissipation time, as well as the VTS characteristics overall plant coverage and hydraulic retention time for targeting high efficacy of pesticide retention. The application of a Tier I risk assessment (EU Uniform Principle) revealed a higher toxicity reduction for hydrophobic and nonpersistent insecticides compared with less sorptive and not readily degradable herbicides and fungicides. Overall, nearly half (48.5%) of all pesticide field concentrations ( = 130) failed Tier I standard risk assessment at the inlet of VTSs, and 29.2% of all outlet concentrations exceeded conservative acute threshold levels. We conclude that VTSs are a suitable and effective risk mitigation strategy for agricultural nonpoint source pesticide pollution of surface waters. Further research is needed to improve their overall efficacy in retaining pesticides.  相似文献   

15.
In the present study, a meta‐analysis was carried out to clarify the association between disinfection byproducts (DBPs) in drinking water and human cancer risk worldwide. Kidney, colorectal, esophagus, urinary bladder, brain, breast, leukemia, lung, and rectum cancers were selected to perform this analysis. According to preferred reporting items for systematic review and meta‐analysis protocol (PRISMA) guidelines, the relevant studies were identified and selection criteria (inclusion and exclusion criteria) were applied. Next, effective subgroups in these studies (gender, type of drinking water source, and type of DBPs) were analyzed. The quality of the studies was evaluated using the Newcastle‐Ottawa Scale. In addition, this overall study included analyses of 16 case–control and 3 cohort studies. The overall odds ratio (OR) with 95% confidence intervals (CI) between DBPs and cancer risk was 1.01 (95% CI, 0.94–1.09). The summary ORs of cancer risk were 1.04 (95% CI, 0.89–1.19) for kidney; 0.98 (95% CI, 0.87–1.09) for colorectal; 1.07 (95% CI, 0.84–1.29) for esophagus; 0.93 (95% CI, 0.80–1.06) for pancreatic; 1.00 (95% CI, 0.83–1.18) for brain; 1.13 (95% CI, 0.99–1.26) for breast; 0.93 (95% CI, 0.72–1.13) for leukemia; and 1.18 (95% CI, 1–1.36) for lung cancers. The results of this meta‐analysis suggested that there is not a significant association between DBPs in water and cancer risk. In addition, subgroup analysis shows a positive association with colorectal and kidney cancer risk in men, as well as colon and breast cancers in females. Studies of both genders have shown a significant association between lung and pancreatic cancers. Moreover, this study finds a significant relationship between cancer rate and consumers of city water and bottled water sources. In analyzing different types of DBPs in water, chlorine and trichloromethane show a significant association in increasing cancer risk.  相似文献   

16.
The status of combined heavy metal and organo-chlorine pesticide (OCPs; i.e. HCH and DDT) pollution was investigated and the soil environmental quality of the Taihu Lake watershed, one of the most developed regions in China, was evaluated using a fuzzy comprehensive assessment. Statistical analyses showed the presence of combined pollution in the soil. At many sampling sites, heavy metal concentrations were above corresponding background values, indicating the effects of extraneous pollutants. It has been over 20 years since China banned the use of OCPs, but they can still be found in soil samples of this region. HCH levels at all investigated sites were below the Chinese Environmental Quality Standard for Soils. Fuzzy comprehensive assessment showed that the overall soil quality in this region could be categorized as class I. Nevertheless, the high coefficients of variation for levels of DDT, Cd and Hg indicated the existence of some point-source pollution. Continuous monitoring and further studies of the region are recommended to prevent pollution of farmland from these sources.  相似文献   

17.
The policy instruments that provide information on a firm’s or facility’s environmental performance, such as the U.S. Toxic Release Inventory (TRI) and the Pollutant Release and Transfer Register system (PRTRs) used in some European countries and Japan, play an important role in encouraging firms or facilities to improve their environmental performance, if investors, consumers and residents recognize their environmental performance. This study uses a hedonic approach to explore how the Japanese rental housing market responds to carcinogenic risk arising from releases and transfers of chemical substances produced and used at close facilities. We found that residents do not perceive carcinogenic risk generated more than 1.0 km away from their residence and that they seem to recognize the increased carcinogenic risk at distances from 0.5 km to 1.0 km away; a 1% increase in carcinogenic risk reduces the average rent by 0.0007%. The distance at which residents perceive the risk arising from such facilities is less than in previous studies. This suggests that the risk perception recognized in previous studies may capture the other externalities in addition to the chemical risk because the risk is measured by the distance.  相似文献   

18.
This article highlights recent research on the beneficial use of selected low frequency electromagnetic fields (EMF) as a safe alternative therapy for treatment of cancer and other health problems. It is shown that EMF therapy provides a safe alternative and adjunct modality for the treatment of cancer and other health problems, and therefore, research in this field deserves more support. The paper also discusses some reports and hypothesis of potential risk of human exposure to low frequency EMF, mainly to the power line frequency of 60 Hz.  相似文献   

19.
Pesticide Risk Indicators (PRIs) are widely used to evaluate and compare the potential health and environmental risks of pesticide use and to guide pest control policies and practices. They are applied to agricultural, landscape and structural pest management by governmental agencies, private institutions and individuals. PRIs typically assess only the potential risks associated with the active ingredients because, with few exceptions, pesticide manufacturers disclose only the identity of the active ingredients which generally comprise only a minor portion of pesticide products. We show that when inert ingredients are identified and assessed by the same process as the active ingredient, the product specific risk can be much greater than that calculated for the active ingredient alone. To maintain transparency in risk assessment, all those who develop and apply PRIs or make decisions based on their output, should clearly disclose and discuss the limitations of the method.  相似文献   

20.
Pesticides, regardless of their known toxic impacts to human health and environment, are widely used in the rapid growing agricultural sectors of developing countries. As an agricultural country with small lands and enormous population to feed, a developing country like Bangladesh rely heavily on the uses of pesticides to increase crop yields. Nevertheless, during the past decades, Peoples’ Republic of Bangladesh has experienced 26.46% decrease in total pesticide consumption. However, the presence of unregistered pesticides in the environmental samples and agricultural products has pointed out the weakness in the existing legal regime of the pesticide governance. This, in turn, is threatening the livelihood and health of the farmers, food safety and consumer health. This paper reviews the antiquity of the status of pesticide consumption, evolution and drawbacks of pesticide in the context of existing socio-economic position of Bangladesh. A consolidated uniform system is lacking to project pesticide management in the country. Existing legal policy, rules and regulations in the context of international agreements regarding pesticide management have been reviewed and suggested for further amendment. Moreover, role of green microfinance in sustainable management of pesticides and food safety were recommended. A framework is proposed for pesticide governance with a stronger pesticide surveillance program and coordination of ministries interlinking environmental, occupational health and food safety.  相似文献   

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