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Wei Que Luhua Jiang Chen Wang Yunguo Liu Zhiwei Zeng Xiaohua Wang Qimeng Ning Shaoheng Liu Peng Zhang Shaobo Liu 《环境科学学报(英文版)》2018,30(8):166-174
Biochar is regarded as a promising new class of materials due to its multifunctional character and the possibility of effectively coupling different properties. With increasing introduction into the environment, environmental chemicals such as surfactants will load onto the released biochar and change its physicochemical characteristics and adsorption behavior toward pollutants. In this study, sodium dodecyl sulfate(SDS), as one type of anionic surfactant, was coated onto biochar with different loading amounts. The influence of SDS loading onto biochar's physicochemical properties were investigated by Fourier transform infrared(FT-IR) spectroscopy, elemental analysis, zeta potential and Brunauer–Emmett–Teller(BET) surface area and pore size distribution analysis. Results showed that the pore size of the biochar decreased gradually with the increase of SDS loading because of the surface-adsorption and pore-blocking processes; the p H of the point of zero charge(pHPZC) decreased with increasing SDS loading. Although surface-coating with SDS decreased the pore size of the biochar, its adsorption capacity toward Methylene Blue(MB) significantly increased. The biochar-bound SDS introduced functional groups and negative charges to the biochar surface, which could thus enhance the adsorption of MB via hydrogen bonding and electrostatic interaction. The results can shed light on the underlying mechanism of the influence of anionic surfactants on the adsorption of MB by biochar. 相似文献
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The study of operating variables in soil washing with EDTA 总被引:7,自引:0,他引:7
Zou Z Qiu R Zhang W Dong H Zhao Z Zhang T Wei X Cai X 《Environmental pollution (Barking, Essex : 1987)》2009,157(1):229-236
This study discusses the operating variables for removal of metals from soils using EDTA, including the type of EDTA, reaction time, solution pH, dose, temperature, agitation, ultrasound and number of extractions. For As, Cd, Cu, Pb and Zn, the removal efficiency order was: H4-EDTA > Na2EDTA > (NH4)2EDTA. At low EDTA concentrations the removal increased progressively with increasing dose while above 0.4 mmol/g only small increases in extraction efficiency were observed. EDTA induced a two-step process including a rapid desorption within the first hour, and a gradual release in the following hours. The extraction efficiency of metals decreased with increasing pH in the range of 2-10. Consecutive extractions using low concentrations were more effective than a single extraction with concentrated EDTA if the same dose of EDTA was used. 相似文献
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Xiao X.Huang L.Huang N.Zhang Y.Ling H.Liu F.Su W.Que Y. 《应用与环境生物学报》2015,(5):872-881
Alternative splicing (AS) is an important part of regulation of eukaryotic gene expression. BAK1 (Brassinosteroid insensitive1-associated receptor kinase 1) is a specific type of plant serine/threonine protein kinases, and can regulate growth and development and natural immunization. To reveal the responses of sugarcane BAK1 gene to the adverse environment, a ScBAK1 gene and its alternative spliceosome, termed ScBAK1 (GenBank accession number: KP032226) and ScBAK1 S1 (GenBank accession number: KP032227), were cloned from leaf cDNA of Yacheng 05-179 utilizing the methods of electronic cloning and RT-PCR. The open reading frame (ORF) length of ScBAK1/ScBAK1 S1 gene was 1 860bp/1 770bp, encoding 619/589 amino acids residues. The predicted molecular weight of the protein was 69.28 kDa/ 65.76 kDa. Both proteins were located in plasma membrane, estimated as acid, hydrophikic and secretive proteins. Random coil and alpha helix gave priority to extended strand in their secondary structure without beta turn. The most important protein function was cell envelope, secondly biosynthesis of amino acids and cofactors. Real-time quantitative PCR analysis revealed that the expression of sugarcane ScBAK1 S1 gene exhibited the reduced expression trend under smut fungus stress and various abiotic exogenous stresses, including SA, CuCl2, PEG, ABA, NaCl and JA, while the expression of ScBAK1 gene was induced by SA, CuCl2, PEG, NaCl and smut fungus stresses. The phenomenon showed that the absent sequences or amounts of ScBAK1 S1 gene plays a key role in the response of ScBAK1 to the stress of sugarcane smut fungus, osmotic stress and cell growth. The differential expression of ScBAK1 and ScBAK1 S1 lays a foundation for further research on the function of ScBAK1 gene under biotic and abiotic stress. 相似文献
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研究了聚乙烯醇(PVA)加少量海藻酸钠及SiO2、CaCO3的方法固定高效菌处理PTA污水.结果表明,采用质量分数分别为PVA 10%、海藻酸钠0.3%、特种菌种10%、SiO2 3%、CaCO30.3%,用饱和硼酸溶液(pH为4.0)作为交联剂,制得的颗粒处理PTA废水时,废水COD负荷为2.91kg/m3·d时,CODcr、TOC、TA去除率均为85%以上;废水COD负荷为12.2kg/m3j·时,CODcr去除率仍为50%以上、TOC去除率为60%以上,当pTA废水pH从55降至35时,CODcr、TOC、TA去除率仍在86%以上. 相似文献
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Monitoring seasonal distribution of an endangered anadromous sturgeon in a large river using environmental DNA 总被引:1,自引:0,他引:1
Nian Xu Bin Zhu Fang Shi Ke Shao Yanfu Que Weitao Li Wei Li Wenjing Jiao Hua Tian Dongmei Xu Jianbo Chang 《Die Naturwissenschaften》2018,105(11-12):62
Monitoring dynamic distribution is crucial to conservation management of anadromous sturgeons, but traditional survey methods are less efficient for low-density populations in a large river. Natural propagation of Chinese sturgeon has been monitored annually mainly at the spawning ground using netting for eggs and hydroacoustics for broodstock. However, absence of spawning was observed sporadically in recent years, indicating further crises for the declining population. We analyzed eDNA of water samples collected from 24 sites across 1360 km of the migratory route of anadromous Chinese sturgeon in the middle and lower reaches of the Yangtze River. Chinese sturgeon was detected at 9 sites during the spawning season and 14 sites after the spawning season. We found that positive eDNA detection rates remained constant in the middle reaches but dramatically changed in the lower reaches, reflecting seasonal migration pattern of Chinese sturgeon. Invasive sturgeons were detected in the river, indicating their possible escape from aquaculture facilities. This study established a protocol for the use of eDNA to monitor distribution of Chinese sturgeon and could be valuable in making better policies for the conservation of this endangered species. 相似文献
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Li Qi Yu Shuili Yang Shengfa Yang Wei Que Sisi Li Wenjie Qin Yu Yu Weiwei Jiang Hui Zhao Deqiang 《Environmental science and pollution research international》2021,28(14):17417-17430
Environmental Science and Pollution Research - In this study, 18S rRNA high-throughput sequencing was applied to investigate the eukaryotic community in a full-scale drinking water treatment plant.... 相似文献
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流域模型技术应用是当前开展面源污染防治的重要工具,而水文过程的准确模拟是进行污染负荷估算的首要环节和关键步骤。为了弄清近年来于桥水库入库河流氮、磷输入负荷,选取GWLF模型对水平口子流域的水文过程进行模拟,首先利用2006—2018年气象、水文资料率定模型水文参数,然后将参数推广到整个流域,对2019—2020年3条主要入库河流流量进行模拟,最后乘以相应河流断面的总氮、总磷浓度估算氮磷输入负荷。结果显示:GWLF模型适用于研究区的水文过程模拟,校准期和验证期的纳氏系数分别为0.89和0.91,平均相对误差分别为12.2%和13.1%;2020年总氮入库负荷为3 977.0 t,其中引滦调水贡献占57.0%,3条入库河流共贡献43.0%;总磷入库负荷为48.8 t,其中引滦调水贡献占68.6%,3条入库河流共贡献31.4%。GWLF模型输入数据需求量较少,模型参数较少,模拟效果较好,适用于中小型流域的水资源和水环境管理,具有一定的推广应用前景。 相似文献
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以玉米秸秆为原料制备生物炭吸附剂,研究了生物炭对水中苯胺的吸附性能。表征结果显示:制备的生物炭的比表面积为449.7 m2/g,体积平均粒径为103μm,主要以小粒径存在;制备的生物炭表面以碱性含氧官能团为主,含量为1.31 mmol/g。实验结果表明:在溶液p H 3、生物炭加入量10 g/L、吸附温度313 K、吸附时间3.0h的最佳反应条件下处理初始苯胺质量浓度为400 mg/L的苯胺溶液,苯胺去除率为94.0%,吸附量为37 mg/g;生物炭对苯胺的吸附过程符合拟二级动力学方程,吸附等温线满足Freundlich等温吸附方程;生物炭对苯胺的吸附是自发、吸热的过程;吸附过程中存在着水分子从生物炭表面的解吸。 相似文献