全文获取类型
收费全文 | 10072篇 |
免费 | 1155篇 |
国内免费 | 4921篇 |
专业分类
安全科学 | 640篇 |
废物处理 | 1057篇 |
环保管理 | 956篇 |
综合类 | 8915篇 |
基础理论 | 1458篇 |
环境理论 | 1篇 |
污染及防治 | 2584篇 |
评价与监测 | 389篇 |
社会与环境 | 129篇 |
灾害及防治 | 19篇 |
出版年
2024年 | 12篇 |
2023年 | 111篇 |
2022年 | 226篇 |
2021年 | 306篇 |
2020年 | 269篇 |
2019年 | 331篇 |
2018年 | 355篇 |
2017年 | 382篇 |
2016年 | 468篇 |
2015年 | 586篇 |
2014年 | 750篇 |
2013年 | 864篇 |
2012年 | 1082篇 |
2011年 | 1041篇 |
2010年 | 853篇 |
2009年 | 956篇 |
2008年 | 649篇 |
2007年 | 953篇 |
2006年 | 1088篇 |
2005年 | 787篇 |
2004年 | 609篇 |
2003年 | 640篇 |
2002年 | 561篇 |
2001年 | 433篇 |
2000年 | 373篇 |
1999年 | 313篇 |
1998年 | 240篇 |
1997年 | 193篇 |
1996年 | 179篇 |
1995年 | 163篇 |
1994年 | 97篇 |
1993年 | 98篇 |
1992年 | 59篇 |
1991年 | 38篇 |
1990年 | 29篇 |
1989年 | 6篇 |
1988年 | 11篇 |
1987年 | 7篇 |
1986年 | 8篇 |
1982年 | 2篇 |
1981年 | 1篇 |
1980年 | 1篇 |
1978年 | 4篇 |
1977年 | 1篇 |
1976年 | 1篇 |
1974年 | 2篇 |
1973年 | 2篇 |
1972年 | 3篇 |
1971年 | 1篇 |
1970年 | 1篇 |
排序方式: 共有10000条查询结果,搜索用时 203 毫秒
1.
以实际中药废水作为阳极基质、实际含镉废水作为阴极电解液,构建了连续流双室微生物燃料电池(MFC),考察了其产电性能及对两种废水的处理效果。78 d的运行数据表明:系统可实现最大输出电压417mV、最大体积功率密度11.8 W/m3,最大体积功率密度运行条件下的库伦效率为18.5%;在阳极进水有机物浓度变化较大的情况下,实现了阳极对中药废水中有机物的有效去除,平均COD去除率为81.5%;阴极对含镉废水中Cd2+的去除率为79.4%~84.8%。这表明MFC同步处理中药废水及重金属废水具有一定的可行性。 相似文献
2.
Afshin Shabani Xiaodong Zhang Xuefeng Chu Timothy P. Dodd Haochi Zheng 《Journal of the American Water Resources Association》2020,56(2):297-309
Devils Lake is a terminal lake located in northeast North Dakota. Because of its glacial origin and accumulated salts from evaporation, the lake has a high concentration of sulfate compared to the surrounding water bodies. From 1993 to 2011, Devils Lake water levels rose by ~10 m, which flooded surrounding communities and increased the chance of an overspill to the Sheyenne River. To control the flooding, the State of North Dakota constructed two outlets to pump the lake water to the river. However, the pumped water has raised concerns about of water quality degradation and potential flooding risk of the Sheyenne River. To investigate these perceived impacts, a Soil and Water Assessment Tool (SWAT) model was developed for the Sheyenne River and it was linked to a coupled SWAT and CE‐QUAL‐W2 model that was developed for Devils Lake in a previous study. While the current outlet schedule has attempted to maintain the total river discharge within the confines of a two‐year flood (36 m3/s), our simulation from 2012 to 2018 revealed that the diversion increased the Sheyenne River sulfate concentration from an average of 125 to >750 mg/L. Furthermore, a conceptual optimization model was developed with a goal of better preserving the water quality of the Sheyenne River while effectively mitigating the flooding of Devils Lake. The optimal solution provides a “win–win” outlet management that maintains the efficiency of the outlets while reducing the Sheyenne River sulfate concentration to ≤600 mg/L. 相似文献
3.
4.
以Ti3AlC2为原料,采用HF刻蚀工艺制备出12种Ti3C2纳米层状材料,对其形貌进行了表征,并考察了以其作为光催化剂对废水中Cr(Ⅵ)的处理效果。实验结果表明:HF体积分数为80%、刻蚀时间为48 h时得到的MX-80-48的形貌较好;MX-80-48具有类似石墨烯的二维层状结构,纳米层厚度约20~50 nm,孔径2~10 nm,比表面积14.8 m2/g,在400~700 nm可见光范围内表现出强烈的吸光性;当Cr(Ⅵ)的初始质量浓度为40.00 mg/L、MX-80-48投加量为200 mg/L、pH=2、反应时间4 h(暗反应1 h+光照3 h)时,Cr(Ⅵ)去除率可达100%。 相似文献
5.
Understanding implications of consumer behavior for wildlife farming and sustainable wildlife trade 下载免费PDF全文
A. Nuno J. M. Blumenthal T. J. Austin J. Bothwell G. Ebanks‐Petrie B. J. Godley A. C. Broderick 《Conservation biology》2018,32(2):390-400
Unsustainable wildlife trade affects biodiversity and the livelihoods of communities dependent upon those resources. Wildlife farming has been proposed to promote sustainable trade, but characterizing markets and understanding consumer behavior remain neglected but essential steps in the design and evaluation of such operations. We used sea turtle trade in the Cayman Islands, where turtles have been farm raised for human consumption for almost 50 years, as a case study to explore consumer preferences toward wild‐sourced (illegal) and farmed (legal) products and potential conservation implications. Combining methods innovatively (including indirect questioning and choice experiments), we conducted a nationwide trade assessment through in‐person interviews from September to December 2014. Households were randomly selected using disproportionate stratified sampling, and responses were weighted based on district population size. We approached 597 individuals, of which 37 (6.2%) refused to participate. Although 30% of households had consumed turtle in the previous 12 months, the purchase and consumption of wild products was rare (e.g., 64–742 resident households consumed wild turtle meat [i.e., 0.3–3.5% of households] but represented a large threat to wild turtles in the area due to their reduced populations). Differences among groups of consumers were marked, as identified through choice experiments, and price and source of product played important roles in their decisions. Despite the long‐term practice of farming turtles, 13.5% of consumers showed a strong preference for wild products, which demonstrates the limitations of wildlife farming as a single tool for sustainable wildlife trade. By using a combination of indirect questioning, choice experiments, and sales data to investigate demand for wildlife products, we obtained insights about consumer behavior that can be used to develop conservation‐demand‐focused initiatives. Lack of data from long‐term social–ecological assessments hinders the evaluation of and learning from wildlife farming. This information is key to understanding under which conditions different interventions (e.g., bans, wildlife farming, social marketing) are likely to succeed. 相似文献
6.
采用特异性移动床生物膜反应器(SMBBR)和厌氧生物滤池(AF)组合工艺处理高氨氮农药废水。考察了HRT、pH和DO等工艺条件对SMBBR-AF-SMBBR组合工艺运行稳定期COD和氨氮去除率的影响。试验结果表明,在进水COD为2 408~7 440 mg/L、ρ(NH_4~+-N)为160.21~433.84 mg/L、TN为208.27~537.65 mg/L、HRT为8d、pH为8.0、DO为4 mg/L的条件下,处理后出水平均COD为342 mg/L,COD去除率达92.3%;ρ(NH_4~+-N)小于4.0mg/L,氨氮平均去除率为89.2%;TN小于50 mg/L,平均TN去除达83.0%。出水各指标均优于原A2O工艺出水。 相似文献
7.
8.
针对煤制乙二醇废水含高浓度硝酸盐氮的特点,设计了缺氧膨胀床(AEB)反应器预处理装置,并进行了工业化启动和调试运行,考察了其在反硝化连续流运行条件下的处理效果及工艺参数变化。结果表明,AEB反应器启动后,填料层生物膜挂膜快速且生长稳定。反应器在工业化调试阶段运行稳定,COD和TN的去除率和去除负荷较为稳定。在受到来水冲击后,AEB反应器处理效果稳定,出水可在短期内恢复正常。该技术的系统操控参数范围较广,易于工业化操控运行,在煤制乙二醇废水和其他含高浓度硝酸盐氮废水的处理中具有较大的推广价值。 相似文献
9.
A sequencing batch reactor was modeled using multi-layer perceptron and radial basis function artificial neural networks (MLPANN and RBFANN). Then, the effects of influent concentration (IC), filling time (FT), reaction time (RT), aeration intensity (AI), SRT and MLVSS concentration were examined on the effluent concentrations of TSS, TP, COD and NH4+-N. The results showed that the optimal removal efficiencies would be obtained at FT of 1 h, RT of 6 h, aeration intensity of 0.88 m3/min and SRT of 30 days. In addition, COD and TSS removal efficiencies decreased and TP and NH4+-N removal efficiencies did not change significantly with increases of influent concentration. The TSS, TP, COD and NH4+-N removal efficiencies were 86%, 79%, 94% and 93%, respectively. The training procedures of all contaminants were highly collaborated for both RBFANN and MLPANN models. The results of training and testing data sets showed an almost perfect match between the experimental and the simulated effluent of TSS, TP, COD and NH4+-N. The results indicated that with low experimental values of input data to train ANNs the MLPANN models compared to RBFANN models are more precise due to their higher coefficient of determination (R2) and lower root mean squared errors (RMSE) values. 相似文献
10.
采用固相烧结法制备了NaCo_2O_4催化剂,构建了NaCo_2O_4-H_2O_2热催化体系降解亚甲基蓝(MB)。XRD和SEM表征结果显示,合成的NaCo_2O_4催化剂具有良好的稳定性。NaCo_2O_4对H_2O_2具有良好的热催化性能,反应温度越高,反应速率常数k越大,该催化反应符合一级动力学方程。NaCo_2O_4-H_2O_2体系对MB具有较好的降解效果,在反应温度为50℃、NaCo_2O_4加入量为50 mg、MB溶液加入量为100 mL、MB初始质量浓度为30 mg/L、H_2O_2加入量为1.00 mL的最优条件下,反应340 min时,MB降解率达87.00%;催化剂重复使用三次,MB降解率仍可达85%以上;经捕获剂效果对比实验发现,催化反应体系中存在h~+、·OH等催化活性物种。 相似文献