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81.
Sommar J Feng X Gårdfeldt K Lindqvist O 《Journal of environmental monitoring : JEM》1999,1(5):435-439
Although it makes up only a few per cent. of total gaseous mercury (TGM) in the atmosphere, the fraction of oxidised (divalent) mercury plays a major role in the biogeochemical cycle of mercury due to its high affinity for water and surfaces. Quantitative knowledge of this fraction present in mixing ratios in the parts-per-10(15) (ppq) range is currently very scarce. This work is based on approximately 220 data for divalent gaseous mercury (DGM) collected during 1995-99 in ambient air. Over the course of the measurements, the sampling and analytical methods were modified and improved. This is described here in detail and includes transition from wet leaching and reduction procedures to thermo-reductive desorption, the use of annular as well as tubular denuders and adoption of an automated sampling system. The concentration of DGM exhibited a strong seasonal behaviour in contrast to atomic gaseous mercury, with low values in winter and maximum values in summer. The DGM/TGM ratios were frequently found to be below the detection limit (< or = 1%) and in the range 1-5%. A trend of diurnal DGM patterns was observed and implies photolytically induced sources. Scavenging of DGM during rain events was also noticed. 相似文献
82.
Degradation of Pesticides on Plant Surfaces and its Prediction - A Case Study on Tea Plant 总被引:4,自引:0,他引:4
The degradative kinetics of pesticides on plant surface are characterized by an initial rapid degradation which follows a first-order kinetics, then transferred to a more slower degradative rate. The degradative process mainly consists of photodegradation, evaporation, rainfall elution and growth dilution. The influencing parameters of these processes were investigated by using the tea plant as a case study. The predictive model of the initial concentration, photodegradation rate constant, evaporation rate constant, rainfall elution rate, growth dilution rate and the total degradation rate was discussed and verified in four locations situated in the range of 25°-30°N latitude, and acceptable results were obtained. 相似文献
83.
Thin-film technique is becoming an industry standard for the preparation of TiO2-based photocatalyst for organic destruction. The catalyst provides several advantages over the conventional powder TiO2 in the treatment of wastewater and groundwater. In this study, a continuous stir flow reactor model is developed capable of describing the photocatalytic process. The model incorporates the following fundamental mechanisms: adsorption, diffusion, liquid-film transfer, UV attenuation, and photocatalytic reaction. All of the simulation results indicate that there exists a highly nonlinear relation between each of these parameters and the destruction rate. Various incident light intensities also are incorporated to simulate the energy efficiency. The simulations illustrate that the photocatalytic model can be used to elucidate the effect of process variables. It is also possible to “custom-design” a catalyst for the treatment of a particular waste stream. 相似文献
84.
Spatial structure analysis and kriging analysis have been identified to be useful tools in illustrating the spatial patterns of variables. Taihu Lake is one of the largest fresh water lakes in China, and has suffered serious eutrophication in recent years due to the rapid economic development and growing environmental pollution in the Taihu Catchment. In this paper, spatial structural analysis, kriging interpolation and eutrophication assessment were carried out for chlorophyll a in the lake. Studies show that spherical model could be applied to fit all experimental variograms. Positive nuggets were observed for three directions except NE–SW direction. The variograms show some anisotropy with anisotropic ratio falling within 1.76. The spatial structural patterns of chlorophyll a in the lake were affected by factors such as distribution of pollution sources, water flow and wind. Two-dimensional ordinary block kriging was applied for interpolation process. An eutrophication assessment map was also made based on a water-quality evaluation standard. Results show that the content of chlorophyll a in Taihu Lake was quite high. The whole lake has suffered serious eutrophication. However, the eutrophic situation varied in space. Higher contents of chlorophyll a appeared mainly in the northern part of the lake. 相似文献
85.
Advances in polymerase chain reaction (PCR) have permitted accurate, rapid and quantitative identification of microorganisms in pure cultures regardless of viability or culturability. In this study, a simple sample processing method was investigated for rapid identification and quantification of fungal spores from dust samples using both conventional and real-time PCR. The proposed method was evaluated for susceptibility to interference from environmental dust samples. Stachybotrys chartarum and Aspergillus fumigatus were used as test organisms. The sensitivity of detection in pure culture was 0.1 spore DNA equivalents per PCR reaction corresponding to 20 spores ml(-1) in the sample. However, 1 spore DNA equivalent per PCR reaction corresponding to 200 spores ml(-1) in the sample was the lowest amount of spores tested without interference in dust samples spiked with spores of either fungal species. The extent of inhibition was calculated using conventional and real-time PCR reactions containing fungal spores, specific primers, specific probes (for real-time PCR) and various amounts of dust. The results indicate that the extent of inhibition by dust on PCR varies with the type and amount of dust, and number of spores. No interference in the analysis of spiked samples was detected from 0.2 mg ml(-1) of four real-life dust samples at p-value >0.05 using 2 x 10(4) spores for conventional PCR and 2 x 10(5) spores for real-time PCR. However, samples containing >0.2 mg ml(-1) real-life dust compromised the PCR assay. These results suggest the potential usefulness of a simple sample processing method in conjunction with PCR for monitoring the fungal content of aerosols collected from indoor environments. 相似文献
86.
中国土壤中溴,碘的背景含量 总被引:1,自引:0,他引:1
通过对全国八百余个表层土样的分析测试,获得了中国土壤中溴、碘背景含量的总体水平及在各土类中的含量,相对于地壳丰度,中国土壤中溴、碘普遍得到了富集,溴、碘含量分异变化较大,并具有明显的地域分异特征,影响中国土壤中溴、碘含量的主要因素是降水量、土壤吸附体的含量以及某些特殊母质。 相似文献
87.
浅析生态园林城市的建设--以重庆市为例 总被引:3,自引:0,他引:3
随着社会、经济的快速发展,城市生态环境问题越来越突出,由此人们提出了建设生态园林城市的构想,即实现了人与自然、人与社会的和谐统一,实现了可持续发展的人类聚居地。山水园林城市与生态城市在本质上是一致的。本文以重庆市为例,从自然、经济、社会三个生态亚系统入手,分析了重庆市生态系统的现状,主要是提出目前面临的问题和矛盾,并在此基础上提出重庆市建设山水园林城市的5条途径。 相似文献
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90.
IntroductionHeavymetalsinwaterbodiesaresignificantlydifferentfromorganicpollutantsthatcanbemicrobiologicallydegradedordecomposed .Generally ,theyarepurifiedthroughtheiradsorptionontosuspendedsubstratesinrivers.Adsorptionofheavymetalsonriversuspendedsub… 相似文献