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11.
Larisse Montero Matthew Duane Urbano Manfredi Covadonga Astorga Giorgio Martini Massimo Carriero Alois Krasenbrink B.R. Larsen 《Atmospheric environment (Oxford, England : 1994)》2010,44(18):2167-2175
The present paper presents results from the analysis of 29 individual C2–C9 hydrocarbons (HCs) specified in the European Commission Ozone Directive. The 29 HCs are measured in exhaust from common, contemporary vehicle/engine/fuel technologies for which very little or no data is available in the literature. The obtained HC emission fingerprints are compared with fingerprints deriving from technologies that are being phased out in Europe. Based on the total of 138 emission tests, thirteen type-specific fingerprints are extracted (Mean ± SD percentage contributions from individual HCs to the total mass of the 29 HCs), essential for receptor modelling source apportionment. The different types represent exhaust from Euro3 and Euro4 light-duty (LD) diesel and petrol-vehicles, Euro3 heavy-duty (HD) diesel exhaust, and exhaust from 2-stroke preEuro, Euro1 and Euro2 mopeds. The fuels comprise liquefied petroleum gas, petrol/ethanol blends (0–85% ethanol), and mineral diesel in various blends (0–100%) with fatty acid methyl esters, rapeseed methyl esters palm oil methyl esters, soybean oil methyl or sunflower oil methyl esters. Type-specific tracer compounds (markers) are identified for the various vehicle/engine/fuel technologies.An important finding is an insignificant effect on the HC fingerprints of varying the test driving cycle, indicating that combining HC fingerprints from different emission studies for receptor modelling purposes would be a robust approach.The obtained results are discussed in the context of atmospheric ozone formation and health implications from emissions (mg km?1 for LD and mopeds and mg kW h?1 for HD, all normalised to fuel consumption: mg dm?3 fuel) of the harmful HCs, benzene and 1,3-butadiene.Another important finding is a strong linear correlation of the regulated “total” hydrocarbon emissions (tot-HC) with the ozone formation potential of the 29 HCs (ΣPO3 = (1.66 ± 0.04) × tot-RH; r2 = 0.93). Tot-HC is routinely monitored in emission control laboratories, whereas C2–C9 are not. The revealed strong correlations broadens the usability of data from vehicle emission control laboratories and facilitates the comparison of the ozone formation potential of HCs in exhaust from of old and new vehicle/engine/fuel technologies. 相似文献
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Riparian Bird Communities as Indicators of Human Impacts Along Mediterranean Streams 总被引:1,自引:0,他引:1
Riparian areas link aquatic and terrestrial habitats, supporting species-rich bird communities, which integrate both terrestrial
and aquatic processes. For this reason, inclusion of riparian birds in stream bioassessment could add to the information currently
provided by existing programs that monitor aquatic organisms. To assess if bird community metrics could indicate stream conditions,
we sampled breeding birds in the riparian zone of 37 reaches in 5 streams draining watersheds representing a gradient of agricultural
intensity in central Italy. As a more direct indicator of water quality, stream macroinvertebrates were also sampled for computation
of the Italian Extended Biotic Index (IBE). An anthropogenic index was calculated within 1 km of sampled reaches based on
satellite-derived land-use classifications. Predictive models of macroinvertebrate integrity based on land-use and avian metrics
were compared using an information-theoretic approach (AIC). We also determined if stream quality related to the detection
of riverine species. Apparent bird species diversity and richness peaked at intermediate levels of land-use modification,
but increased with IBE values. Water quality did not relate to the detection of riverine species as a guild, but two species,
the dipper Cinclus cinclus and the grey wagtail Motacilla cinerea, were only observed in reaches with the highest IBE values. Small-bodied insectivorous birds and arboreal species were detected
more often in reaches with better water quality and in less modified landscapes. In contrast, larger and granivorous species
were more common in disturbed reaches. According to the information-theoretic approach, the best model for predicting water
quality included the anthropogenic index, bird species diversity, and an index summarizing the trophic structure of the bird
community. We conclude that, in combination with landscape-level information, the diversity and trophic structure of riparian
bird communities could serve as a rapid indicator of stream-dwelling macroinvertebrates and, therefore, degradation of in-stream
biotic integrity. 相似文献
14.
Robust monitoring of carbon sequestration by forests requires the use of multiple data sources analyzed at a common scale. To that end, model-based Moderate Resolution Imaging Spectroradiometer (MODIS) and field-based Forest Inventory and Analysis (FIA) data of net primary productivity (NPP) were compared at increasing levels of spatial aggregation across the eastern USA. A total of 52,167 FIA plots and colocated MODIS forest cover NPP pixels were analyzed using a hexagonal tiling system. A protocol was developed to assess the optimal scale as an optimal size of landscape patches at which to map spatially explicit estimates of MODIS and FIA NPP. The optimal mapping resolution (hereafter referred to as optimal scale) is determined using spatially scaled z-statistics as the tradeoff between increased spatial agreement as measured by Pearson’s correlation coefficient and decreased details of coverage as measured by the number of hexagons. Spatial sensitivity was also assessed using land cover assessment and forest homogeneity using spatially scaled z-statistics. Pearson correlations indicate that MODIS and FIA NPP are most highly correlated when using large hexagons, while z-statistics indicate an optimal scale at an intermediate hexagon size of 390 km2. This optimal scale had more spatial detail than was obtained for larger hexagons and greater spatial agreement than was obtained for smaller hexagons. The z-statistics for land cover assessment and forest homogeneity also indicated an optimal scale of 390 km2. 相似文献
15.
Ralph I. Larsen 《Journal of the Air & Waste Management Association (1995)》2013,63(11):1326-1339
Abstract The Clean Air Act Amendments of 1990 (CAAA-90) list 189 hazardous air pollutants (HAPs) for which “safe” ambient concentrations are to be determined. The primary purpose of this paper is to develop two mathematical models, lognormal and logarithmic, that effectively express excess lung cancer mortality as a function of asbestos concentration for an example set of data and also to suggest using these two models for additional HAPs. The secondary purpose of this paper is to calculate a “safe” asbestos concentration by first assuming a default linear extrapolation (to one excess death per million people, as specified for carcinogenic HAPs). The resulting “safe” concentration is an impossible-to-achieve 1/1000 of present background asbestos concentrations. A letter to the editor and a response in this Journal issue use additional asbestos data that suggest that the “safe” concentration should be about 730 times higher than first calculated here and that a default nonlinear extrapolation should be used instead, with the “safe” concentration proportional to the desired mortality level raised to the 0.39 power. These results suggest that the most important problem in setting a “safe” concentration for each carcinogenic HAP is to determine the correct nonlinear extrapolation to use for each HAP. 相似文献
16.
Miller JL Miller MJ de Vlaming V Larsen K Smith E Reece K 《Environmental monitoring and assessment》2009,150(1-4):333-349
A number of procedures have been developed to assess toxic effects on the early life stages of salmonid fish. In this study 13 rainbow trout embryo development relatively short-term (7 to 90 day) procedures were reviewed. Three 7-day methods from the published literature and three modifications developed at AQUA-Science (A-S) were evaluated in the laboratory. Based on that evaluation, A-S methods were selected for screening surface water samples (A-S 1) collected in the Sacramento River watershed (California) and for conducting toxicity identification evaluations (TIE) to identify cause(s) of toxicity. Test control performance, test sensitivity, and reference toxicant response variability in the A-S 1 were superior to those in commonly used freshwater toxicity testing methods. The incidence of Sacramento River watershed samples resulting in a notable decrease in embryo development was very low. Of 260 samples screened only 16 (6%) resulted in statistically significant inhibition of embryo development. Of the 16 toxic samples, nine caused minimal (less than 20% abnormal development) and four marginal (less than 30%) toxicity. Samples collected from the agriculture-dominated Colusa Basin Drain and rangeland/forest-dominated Battle Creek on June 16, 2005 caused significant toxicity. TIE procedures indicated that cationic chemicals were the primary cause of toxicity. Metals analysis did not reveal concentrations sufficient to inhibit embryo development, so the most probable cause of toxicity in the two samples was cationic chemicals (perhaps surfactants?) or metals that were not included in the analytical screening. 相似文献
17.
Understanding how hydraulic factors control alluvial river meander migration can help resource managers evaluate the long-term
effects of floodplain management and bank stabilization measures. Using a numerical model based on the mechanics of flow and
sediment transport in curved river channels, we predict 50 years of channel migration and suggest the planning and ecological
implications of that migration for a 6.4-km reach (river miles 218–222) of the Sacramento River near the Woodson Bridge State
Recreation Area, California, USA.
Using four different channel management scenarios, our channel migration simulations suggest that: (1) channel stabilization
alters the future channel planform locally and downstream from the stabilization; (2) rock revetment currently on the bank
upstream from the Woodson Bridge recreation area causes more erosion of the channel bank at the recreation area than if the
revetment were not present; (3) relocating the channel to the west and allowing subsequent unconstrained river migration relieves
the erosion pressure in the Woodson Bridge area; (4) the subsequent migration reworks (erodes along one river bank and replaces
new floodplain along the other) 26.5 ha of land; and (5) the river will rework between 8.5 and 48.5 ha of land in the study
reach (over the course of 50 years), depending on the bank stabilization plan used. The reworking of floodplain lands is an
important riparian ecosystem function that maintains habitat heterogeneity, an essential factor for the long-term survival
of several threatened and endangered animal species in the Sacramento River area. 相似文献
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