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11.
Syam S. Andra Konstantinos C. Makris Shahida Quazi Dibyendu Sarkar Rupali Datta Stephan B. H. Bach 《Environmental science and pollution research international》2010,17(5):1167-1173
Background, aim, and scope
Organoarsenical-containing animal feeds that promote growth and resistance to parasites are mostly excreted unchanged, ending up in nearby wastewater storage lagoons. Earlier work documented the partial transformation of organoarsenicals, such as, 3-nitro-4-hydroxyphenylarsonic acid (roxarsone) to the more toxic inorganic arsenate [As(V)] and 3-amino-4-hydroxyphenylarsonic acid (3-AHPAA). Unidentified roxarsone metabolites using liquid chromatography coupled to inductively coupled plasma mass spectrometry (LC/ICP-MS) were also inferred from the corresponding As mass balance. Earlier batch experiments in our laboratory suggested the presence of organometallic (Cu) complexes during relevant roxarsone degradation experiments. We hypothesized that organocopper compounds were complexed to roxarsone, mediating its degradation in field-collected swine wastewater samples from storage lagoons. The objective of this study was to investigate the role of organometallic (Cu) complexes during roxarsone degradation under aerobic conditions in swine wastewater suspensions, using electrospray ionization mass spectrometry (ES-MS). 相似文献12.
Makris KC Shakya KM Datta R Sarkar D Pachanoor D 《Environmental pollution (Barking, Essex : 1987)》2007,148(1):101-106
The efficiency of vetiver grass (Vetiveria zizanioides) in removing 2,4,6-trinitrotoluene (TNT) from aqueous media was explored in the presence of a common agrochemical, urea, used as a chaotropic agent. Chaotropic agents disrupt water structure, increasing solubilization of hydrophobic compounds (TNT), thus, enhancing plant TNT uptake. The primary objectives of this study were to: (i) characterize TNT absorption by vetiver in hydroponic media, and (ii) determine the effect of urea on chemically catalyzing TNT uptake by vetiver grass in hydroponic media. Results showed that vetiver exhibited a high TNT uptake capacity (1.026 mgg(-1)), but kinetics were slow. Uptake was considerably enhanced in the presence of urea, which significantly (p<0.001) increased the 2nd-order reaction rate constant over that of the untreated (no urea) control. Three major TNT metabolites were detected in the roots, but not in the shoot, namely 1,3,5-trinitrobenzene, 4-amino 2,6-dinitrotoluene, and 2-amino 4,6-dinitrotoluene, indicating TNT degradation by vetiver grass. 相似文献
13.
Konstantinos Ganias 《Marine Biology》2008,155(3):293-301
Using previously published histological data on multiple, monthly samples of Sardina pilchardus collected in the central Aegean and Ionian Seas (September 1999–August 2000, and November 2000–February 2001), the Mediterranean
sardine was treated as a case study to investigate the biological characteristics of ephemeral spawning aggregations in multiple-spawning
clupeoids. Actively spawning (Day0) females in the Mediterranean sardine, i.e., the daily class of spawners caught a few hours prior, during, or after the spawning
act, were shown to separate spatially from late (Day1+) spawners and non-spawning females, taking with them a large proportion of conspecific males which were also in advanced
spawning condition and in better somatic condition compared to the remaining population. In addition, information from 28
stocks of multiple-spawning clupeoids from a wide range of geographic locations, belonging to 14 species and 2 families (Engraulidae
and Clupeidae), was reviewed and analyzed pertinent to the formation of ephemeral spawning aggregations. Results from the
latter analysis indicated similar patterns of spatial segregation of Day0 spawners in the reviewed clupeoid stocks as in the Mediterranean Sardine, which strongly suggested that the formation of
ephemeral spawning aggregations is a common behavioral trait among multiple-spawning clupeoids.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
14.
Development of a black carbon-inclusive multi-media model: application for PAHs in Stockholm 总被引:1,自引:0,他引:1
A multi-media model was developed for predicting the fate of organic chemicals in the Greater Stockholm Area, Sweden, and applied to selected polycyclic aromatic hydrocarbons (PAHs). Although urban models have been previously developed, this model is novel in that it includes sorption to pyrogenically-derived particles, commonly termed "black carbon" (BC), within the model structure. To examine the influence of BC sorption on environmental fate of PAHs, two versions of the model were generated and run: one in which sorption to BC was included and one in which BC sorption was excluded. The inclusion of BC sorption did not cause any significant variations to air levels, but it did cause an average 20-30% increase in sediment concentrations related to increased sediment solids partitioning. The model also predicted reduced advective losses out of the model domain, as well as chemical potential to diffuse from sediments, whilst total chemical inventory increased. In all cases, the lighter PAHs were more affected by BC inclusion than their heavier counterparts. We advocate the addition of sorption to BC in future multi-media fate and exposure models, which as well as influencing fate will also alter (lower) chemical availability and, thus, wildlife exposure to hydrophobic chemicals. A quantification of the latter was derived with the help of the soot-inclusive model version, which estimated a lowering of dissolved water concentrations between five and >200 times for the different PAHs of this study. 相似文献
15.
Methane and carbon dioxide emission in a two-phase olive oil mill sludge windrow pile during composting 总被引:1,自引:0,他引:1
Manios T Maniadakis K Boutzakis P Naziridis Y Lasaridi K Markakis G Stentiford EI 《Waste management (New York, N.Y.)》2007,27(9):1092-1098
The aim of this work was to make some preliminary evaluations on CO(2) and CH(4) emissions during composting of two-phase olive oil mill sludge (OOMS). OOMS, olive tree leaves (OTL) and shredded olive tree branches (OTB) were used as feedstock for Pile I and Pile II with a 1:1:1 and 1:1:2v/v ratio, respectively. Each pile was originally 1.2m high, 2.0m wide and approximately 15.0m long. Four 500 ml volume glass funnels were inverted and introduced in each pile, two in the core (buried 50-60 cm from the surface) and two near the surface under a thin 10-15 cm layer of the mixture. Thin (0.5 cm diameter) plastic, 80 cm long tubes were connected to the funnels. A mobile gas analyser (GA2000) was used to measure the composition (by volume) of O2, CO2 and CH4 on a daily basis. The funnels were removed prior to each turning and reinserted afterwards. From each pair of funnels (core and surface) of both piles, one was kept closed between samplings. Two way ANOVA was used to test differences between piles and among the tubes. Post hoc Tukey tests were also used to further investigate these differences. There was a significant difference (at p<0.001) in the two piles for all three gases. The average concentrations of O2, CO2 and CH4 in Pile I, from all four funnels was 16.86%, 3.89% and 0.25%, respectively, where for Pile II the average values were 18.07%, 2.38% and 0.04%, respectively. The presence of OOMS in larger amounts in Pile I (resulting in more intense decomposing phenomena), and the larger particle size of OTB in Pile II (resulting in increasing porosity) are the probable causes of these significant differences. Samples from open funnels presented lower, but not significantly lower, O2 composition (higher for CO2 and CH4) in comparison with closed funnels in both depths and both piles. Not significant were also the different mean gas compositions between core and surface funnels in the same pile. 相似文献
16.
The efficiency of water rinsing for removing fenthion from non-combustible used pesticide containers was investigated. Four hundred empty containers from four olive oil producing areas in Greece were studied. Following triple rinsing cleaning procedures, the amount of fenthion retained in the container ranged from 0.01% to 0.1% w/w of its initial concentration. Extraction was accomplished with acetone, and the extracts were analyzed with a capillary gas chromatographic system coupled with flame ionization detector. The results obtained showed that triple rinsing is an effective procedure for removing fenthion from used pesticide containers, since the remaining pesticide concentration was below the legislated threshold value. Consequently, the containers can be handled as non-hazardous solid wastes. 相似文献
17.
Christos Giannakopoulos Effie Kostopoulou Konstantinos V. Varotsos Kostas Tziotziou Achilleas Plitharas 《Regional Environmental Change》2011,11(4):829-843
Climate changes in the Mediterranean region, related to a significant increase in temperature and changes in precipitation
patterns, can potentially affect local economies. Agriculture and tourism are undoubtedly the most important economic sources
for Greece and these may be more strongly affected by changing future climate conditions. Climate change and their various
negative impacts on human life are also detected in their environment; hence this study deals with implications, caused by
changing climate, in urban and forest areas. Potential changes for the mid-twenty-first century (2021–2050) are analysed using
a high-resolution regional climate model. This paper presents relevant climatic indices, indicative for potential implications
which may jeopardise vital economic/environmental sectors of the country. The results provide insights into particular regions
of the Greek territory that may undergo substantial impacts due to climate change. It is concluded that the duration of dry
days is expected to increase in most of the studied agricultural regions. Winter precipitation generally decreases, whereas
an increase in autumn precipitation is projected in most areas. Changing climate conditions associated with increased minimum
temperatures (approximately 1.3°C) and decreased winter precipitation by 15% on average suggest that the risk for forest fires
is intensified in the future. In urban areas, unpleasantly high temperatures during day and night will increase the feeling
of discomfort in the citizens, while flash floods events are expected to occur more frequently. Another impact of climate
change in urban regions is the increasing energy demand for cooling in summer. Finally, it was found that continental tourist
areas of the Greek mainland will more often face heatwave episodes. In coastal regions, increased temperatures especially
at night in combination with high levels of relative humidity can lead to conditions that are nothing less than uncomfortable
for foreigners and the local population. In general, projected changes associated with temperature have a higher degree of
confidence than those associated with precipitation. 相似文献
18.
Valavanidis A Fiotakis K Vlahogianni T Bakeas EB Triantafillaki S Paraskevopoulou V Dassenakis M 《Chemosphere》2006,65(5):760-768
The concentrations of trace metals and polycyclic aromatic hydrocarbons (PAHs) adsorbed to total suspended particulate (TSP) and finer fractions of airborne particulate matter (PM) were determined from a site in the centre of Athens (Greece), which is characterized by heavy local traffic and is densely populated, during the winter and summer periods in 2003-2004. Also, we collected and analyzed samples of diesel and gasoline exhaust particles from local vehicles (buses, taxis and private cars) and from chimney exhaust of residential central heating appliances. A seasonal effect was observed for the size distribution of aerosol mass, with a shift to larger fine fractions in winter. The most commonly detected trace metals in the TSP and PM fractions were Fe, Pb, Zn, Cu, Cr, V, Ni and Cd and their concentrations were similar to levels observed in heavily polluted urban areas from local traffic and other anthropogenic emissions. Analysis of 16 PAHs bound to PM showed that they are mostly traffic related. In general, the fine particulate PAHs concentrations were higher than coarse particles. The most common PAHs in PM(10.2) and PM(2.1) were pyrene, phenanthrene, acenapthylene and fluoranthene, which are associated with diesel and gasoline exhaust particles. The results of this study underlined the importance of local emission sources, especially vehicular traffic, central heating and other local anthropogenic emissions. Compared with other big cities, Athens has much higher levels of airborne particles, especially of the finer fractions PM(10) and PM(2.5), correlated with traffic-related air pollution. 相似文献
19.
Shakoor Adeel Khan Asim Laeeq Akhter Parveen Aslam Muhammad Bilad Muhammad Roil Maafa Ibrahim M. Moustakas Konstantinos Nizami Abdul-Sattar Hussain Murid 《Environmental science and pollution research international》2021,28(10):12397-12405
Environmental Science and Pollution Research - Mixed matrix membranes (MMMs) were fabricated by the hydrothermal synthesis of ordered mesoporous KIT-6 type silica and incorporating in polyimide... 相似文献
20.