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91.
A high degradation extent of benzo[a]pyrene (BaP) should not be considered as the sole desirable criterion for the bioremediation of BaP-contaminated soils because some of its accumulated metabolites still have severe health risks to human. Two main metabolites of BaP, benzo[a]pyrene-1,6-quinone (BP1,6-quinone) and 3-hydroxybenzo[a]pyrene (3-OHBP) were identified by high performance liquid chromatography (HPLC) with standards. This study was the first time that degradation of both BaP and the two metabolites was carried out by chemical oxidation and biodegradation. Three main phases during the whole degradation process were proposed. Hydrogen peroxide-zinc (H(2)O(2)-Zn), the fungus - Aspergillus niger and the bacteria - Zoogloea sp. played an important role in the different phases. The degradation parameters of the system were also optimized, and the results showed that the effect of degradation was the best when fungus-bacteria combined with H(2)O(2)-Zn, the concentration range of BaP in the cultures was 30-120mg/l, the initial pH of the cultures was 6.0. However, as co-metabolites, phenanthrene significant inhibited the degradation of BaP. This combined degradation system compared with the conventional method of degradation by domestic fungus only, enhanced the degradation extent of BaP by more than 20% on the 12d. The highest accumulation of BP1,6-quinone and 3-OHBP were reduced by nearly 10% in the degradation experiments, which further proved that the combined degradation system was more effective as far as joint toxicity of BaP and its metabolites are concerned. 相似文献
92.
Hongkuan ZANG Yi XU Wei LI Guohe HUANG Dan LIU 《Frontiers of Environmental Science & Engineering》2012,6(4):549-558
In this study, an interval fuzzy mixed-integer energy planning model (IFMI-EPM) is developed under considering the carbon tax policy. The developed IFMIEPM incorporates techniques of interval-parameter programming, fuzzy planning and mixed-integer programming within a general energy planning model. The IFMIEPM can not only be used for quantitatively analyzing a variety of policy scenarios that are associated with different levels of carbon tax policy, but also tackle uncertainties expressed as discrete intervals and fuzzy sets in energy and environment systems. Considering low, medium and high carbon tax rates, the model is applied to an ideal energy and environment system. The results indicate that reasonable solutions have been generated. They can be used for generating decision alternatives and thus help decision makers identify desired carbon tax policy. 相似文献
93.
电梯门区故障是电梯整体主要故障之一。基于目前电梯门区常见故障或者已经发生的事故,本文系统性地建立电梯门区故障案例库并进行其软件研发;根据故障案例库中已知的案例信息得到故障类型风险的相关信息,进行风险分析;将故障案例中实际出现的故障类型组合种类归纳后,计算出每种组合的危害程度,按照危害程度值进行降序排列;软件系统根据用户输入的设备信息给出风险较高的故障组合和相应的预防措施。 相似文献
94.
95.
To explore biodegradation of 2-naphthol and its metabolites accumulated in wastewater treatment, a series of bio-degradation
experiments were conducted. Two main metabolites of 2-naphthol, 1,2-naphthalene-diol and 1,2-naphthoquinone, were identified by
high-performance liquid chromatography with standards. Combining fungus Aspergillus niger with bacterium Bacillus subtilis in the
treatment enhanced 2-naphthol degradation e ciency, lowered the accumulation of the two toxic metabolites. There were two main
phases during the degradation process by the kinetic analysis: 2-naphthol was first partly degraded by the fungus, producing labile
and easily accumulated metabolites, and then the metabolites were mainly degraded by the bacterium, attested by the degradation
processes of 1,2-naphthalene-diol and 1,2-naphthoquinone as sole source of carbon and energy. Sodium succinate, as a co-metabolic
substrate, was the most suitable compound for the continuous degradation. The optimum concentration of 2-naphthol was 50 mg/L.
The overall 2-naphthol degradation rate was 92%, and the CODCr removal rate was 80% on day 10. These results indicated that
high degradation rate of 2-naphthol should not be considered as the sole desirable criterion for the bioremediation of 2-naphtholcontaminated
soils/wastewater. 相似文献
96.
97.
Using a liquid–solid phase inversion method, a hybrid matrix poly(vinylidene fluoride)(PVDF) membrane was prepared with alumina(Al2O3) nanoparticle addition. Pd/Fe nanoparticles(NPs) were successfully immobilized on the Al2O3/PVDF membrane, which was characterized by Scanning Electron Microscopy(SEM) and Transmission Electron Microscopy(TEM). The micrographs showed that the Pd/Fe NPs were dispersed homogeneously. Several important experimental parameters were optimized, including the mechanical properties, contact angle and surface area of Al2O3/PVDF composite membranes with different Al2O3 contents. At the same time, the ferrous ion concentration and the effect of hydrophilization were studied. The results showed that the modified Al2O3/PVDF membrane functioned well as a support. The Al2O3/PVDF membrane with immobilized Pd/Fe NPs exhibited high efficiency in terms of dichloroacetic acid(DCAA) dechlorination. Additionally, a reaction pathway for DCAA dechlorination by Pd/Fe NPs immobilized on the Al2O3/PVDF membrane system was proposed. 相似文献
98.
Shuangyang Zhao Chengxin Chen Jie Ding Shanshan Yang Yani Zang Nanqi Ren 《Frontiers of Environmental Science & Engineering》2022,16(3):36
99.
本文探讨了碲化镉量子点(CdTe QDs)对肝细胞的毒性效应及其影响因素,为探索量子点的肝毒性机制提供一定依据。采用人肝癌细胞(Hep G2)和人正常肝细胞(L02)为细胞模型,设置0、25、50和100μmol·L-14个浓度组,采用CCK-8法检测细胞生存率,石墨炉法检测细胞内镉元素含量,采用流式细胞术,装载荧光探针DCFH-DA检测细胞内活性氧水平,采用FITC/PI检测细胞凋亡以及JC-1检测细胞ATP水平。研究结果显示:CdTe QDs诱导2种肝细胞生存率降低,细胞凋亡率升高,细胞对QDs的摄入水平具有时间依赖性,细胞内活性氧水平显著升高,线粒体膜电位降低和ATP含量显著减少,且2种肝细胞比较发现L02细胞损伤程度更为严重。CdTe QDs对2种肝细胞造成损伤,对L02细胞损伤更明显,其原因是L02细胞对CdTe QDs摄取更多,导致进入细胞的QDs引发更为严重的损伤效应。 相似文献
100.