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121.
122.
河岸缓冲区氮素截留研究进展 总被引:1,自引:0,他引:1
河岸缓冲区对氮素的有效截留以阻止其进入河流已得到广泛的认可,是美国资源局所认可的一种最佳管理措施。总结河岸缓冲区中氮素截留的主要机制、影响因素及缓冲区的管理原则。最主要截留机制为反硝化作用与植物吸收,相应的最主要影响因素是缓冲区的水文特征。为达到较好的氮素截留效率,必须重建退化的缓冲区、保护缓冲区的完整性与不受干扰,并与其他流域管理措施相结合。 相似文献
123.
Cook KL Rothrock MJ Eiteman MA Lovanh N Sistani K 《Journal of environmental management》2011,92(7):1760-1766
Poultry litter is a valuable nutrient source for crop production. Successful management to reduce ammonia and its harmful side-effects on poultry and the environment can be aided by the use of litter amendments. In this study, three acidifiers, two biological treatments, one chemical urease inhibitor and two adsorber amendments were added to poultry litter. Chemical, physical and microbiological properties of the litters were assessed at the beginning and the end of the experiment. Application of litter amendments consistently reduced organic N loss (0-15%) as compared to unamended litter (20%). Acidifiers reduced nitrogen loss through both chemical and microbiological processes. Adsorbent amendments (water treatment residuals and chitosan) reduced nitrogen loss and concentrations of ammonia-producing bacteria and fungi. The use of efficient, cost-effective litter amendments to maximum agronomic, environmental and financial benefits is essential for the future of sustainable poultry production. 相似文献
124.
This article focuses on modelling above and below-ground mass loss and nitrogen (N) dynamics based on the wooden dowels (Gonystylus bancanus [Miq.] Kurz) of the decadal Long-term Intersite Decomposition Experiment (LIDET) data. These dowels were placed at 27 locations across North and Central America, involving tropical, temperate and boreal forests, grasslands, wetlands and the tundra. The dowel, inserted vertically into the soil with one half remaining exposed to the air, revealed fast mass and N losses under warm to humid conditions, and slow losses under wet as well as cold to dry conditions. The model formulation, referred to as the Wood Decomposition Model, or WDM, related these losses to (i) mean annual precipitation, mean monthly January and July air temperatures, and (ii) mean annual actual evapotranspiration (AET) at each location. The resulting calibrations conformed well to the time-in-field averages for mass remaining by location: R2 = 0.83 and 0.90 for the lower and upper parts, respectively. These values dropped, respectively, to 0.41 and 0.55 for the N concentrations, and to 0.28 and 0.43 for N remaining. These reductions likely refer to error propagation and to as yet unresolved variations in N transference into and out of the wood specific to each individual dowel location. Recalibrating the model parameters by ecosystem type reduced the R2 values for actual versus best-fitted mass loss by about 0.15. Doing the same without location- or ecosystem-specific adjustments reduced the R2 values further, by about 0.3. 相似文献
125.
Modelling N mineralization from green manure and farmyard manure from a laboratory incubation study 总被引:1,自引:0,他引:1
M. Mohanty K. Sammi ReddyM.E. Probert R.C. Dalal A. Subba RaoN.W. Menzies 《Ecological modelling》2011,222(3):719-726
Predicting N mineralization from organic manures like farmyard manure (FYM) is more difficult than from fresh organic materials like crop residues, as the manures vary greatly in composition. A laboratory incubation experiment was carried out for 98 days at 30 °C under aerobic conditions to study the effects on N dynamics of Gliricidia (Gliricidia sepium, Jacquin) and FYM application to soil at 5 and 10 g kg−1. Application of Gliricidia induced N mineralization from the start of incubation period, with the amount of N mineralized increasing with rate of application. In contrast, application of FYM resulted in immobilization of mineral N in soil, irrespective of the rate of application. The initial net immobilization from FYM was limited by availability of N in the soil for the higher rate of application.We used the APSIM SoilN module to simulate these contrasting patterns of mineralization of N from Gliricidia and from FYM. The prediction of N mineralized from Gliricidia was better than FYM. The default model parameters specify that the fresh organic matter pools (FPOOL1, FPOOL2 and FPOOL3) have the same C:N ratio and this assumption was ineffective in predicting N mineralized from FYM. The predictive ability of the model improved when this default assumption was modified based on the size of the individual pools (FPOOL1, FPOOL2 and FPOOL3), and the pool's C:N ratios. The modelling efficiency, a measure of goodness of fit between the simulated and observed data, improved markedly for the modified model. The discrepancy between the modelled and observed data was a tendency for the model to underestimate the rate of re-mineralization at the lower rate of application of FYM in the later part of incubation. Unfortunately the appropriate modification to the size and C:N ratios of the FPOOLs could not be determined on the basis of chemical analysis alone. Thus, a true predictive application of the model to a new FYM material is not yet possible. 相似文献
126.
Zhenming Zhou Canyang Lin Shuwen Li Shupo Liu Fei Li Baoling Yuan 《Frontiers of Environmental Science & Engineering》2022,16(3):29
127.
Chen Xing Daihui Yang Yan Zhang Tian Sun Junfei Duan Hussein A.Younus Shiguo Zhang 《绿色能源与环境(英文)》2022,7(1):43-52
Heteroatom-doped meso/micro-porous carbon materials are conventionally produced by harsh carbonization under an inert atmosphere involving specific precursors, hard/soft templates, and heteroatom-containing agents. Herein, we report a facile synthesis of N and O co-doped meso/micro-porous carbon (NOMC) by template-free carbonization of a small-molecule precursor in a semi-closed system. The semi-closed carbonizaiton process yields hydrophilic NOMCs with large surface area in a high yield. The porous structure as well as the elemental composition of NOMCs can be modulated by changing the holding time at a particular temperature. NOMCs as metal-free heterogeneous catalysts can selectively oxidize benzyl alcohol and its derivatives into aldehydes/ketones with>85%conversion in aqueous solution, which is much higher than that of the control sample obtained in tube furnace (21%conversion), mainly due to their high N content, high percentage of pyridinic N, and large surface area. The presence of O-containing moieties also helps to improve the hydrophilicity and dispersion ability of catalysts and thus facilitates the mass transfer process during aqueous oxidation. The NOMC catalysts also dispayed excellent activity for a wide range of substrates with a selectivity of>99%. 相似文献
128.
Analysis of the relationship between ambient levels of O3, NO2 and NO as a function of NOx in the UK
Monitoring data from the UK Automatic Urban and Rural Network are used to investigate the relationships between ambient levels of ozone (O3), nitric oxide (NO) and nitrogen dioxide (NO2) as a function of NOx, for levels ranging from those typical of UK rural sites to those observed at polluted urban kerbside sites. Particular emphasis is placed on establishing how the level of ‘oxidant’, OX (taken to be the sum of O3 and NO2) varies with the level of NOx, and therefore to gain some insight into the atmospheric sources of OX, particularly at polluted urban locations. The analyses indicate that the level of OX at a given location is made up of NOx-independent and NOx-dependent contributions. The former is effectively a regional contribution which equates to the regional background O3 level, whereas the latter is effectively a local contribution which correlates with the level of primary pollution. The local oxidant source has probable contributions from (i) direct NO2 emissions, (ii) the thermal reaction of NO with O2 at high NOx, and (iii) common-source emission of species which promote NO to NO2 conversion. The final category may include nitrous acid (HONO), which appears to be emitted directly in vehicle exhaust, and is potentially photolysed to generate HOx radicals on a short timescale throughout the year at southern UK latitudes. The analyses also show that the local oxidant source has significant site-to-site variations, and possible reasons for these variations are discussed. Relationships between OX and NOx, based on annual mean data, and fitted functions describing the relative contributions to OX made by NO2 and O3, are used to define expressions which describe the likely variation of annual mean NO2 as a function of NOx at 14 urban and suburban sites, and which can take account of possible changes in the regional background of O3. 相似文献
129.
The HBV-N model was used for a scenario analysis of changes in nitrogen retention and transport caused by alterations of
wetness due to land drainage, lowering of lakes, building of dams and climatic variability in a river basin in south-central
Sweden (1885–1994). In general, dams were situated in locations more favourable for retention, compared to the lowered lakes.
Rather modest conversions of water bodies only changed nitrogen transport by about 3%. The 180-times-larger increase of (mainly)
tile-drained agricultural land had, according to simulations, increased the nitrogen transport by 17%, due to reduced retention.
However, compared to human-induced alteration of the landscape N retention, the choice of 10-year periods of climatological
data had the overriding effect on the calculated nitrogen transport. Weather-induced variations resulted in a 13% difference
in nitrogen retention between various 10-year periods. When the model was driven by climatological data from the driest 10-year
period (1905–1914), the estimated average annual load was only half of that obtained with climatological data from the wettest
10-year period (1975–1984).
Electronic Publication 相似文献
130.
Zhenyan Zhang Xiaoji Fan W.J.G.M. Peijnenburg Meng Zhang Liwei Sun Yujia Zhai Qi Yu Juan Wu Tao Lu Haifeng Qian 《环境科学学报(英文版)》2021,33(1):1-9
Freshwater cyanobacterial blooms have drawn public attention because they threaten the safety of water resources and human health worldwide. Heavy cyanobacterial blooms outbreak in Lake Taihu in summer annually and vanish in other months. To find out the factors impacting the cyanobacterial blooms, the present study measured the physicochemical parameters of water and investigated the composition of microbial community using the 16S rRNA gene and internal transcribed spacer amplicon sequencing in the months with or without bloom. The most interesting finding is that two major cyanobacteria, Planktothrix and Microcystis, dramatically alternated during a cyanobacterial bloom in 2016, which is less mentioned in previous studies. When the temperature of the water began increasing in July, Planktothrix appeared first and showed as a superior competitor for M. aeruginosa in NO3?-rich conditions. Microcystis became the dominant genus when the water temperature increased further in August. Laboratory experiments confirmed the influence of temperature and the total dissolved nitrogen (TDN) form on the growth of Planktothrix and Microcystis in a co-culture system. Besides, species interactions between cyanobacteria and non-cyanobacterial microorganisms, especially the prokaryotes, also played a key role in the alteration of Planktothrix and Microcystis. The present study exhibited the alteration of two dominant cyanobacteria in the different bloom periods caused by the temperature, TDN forms as well as the species interactions. These results helped the better understanding of cyanobacterial blooms and the factors which contribute to them. 相似文献