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121.
122.
The concentrations of ambient total suspended particulates (TSP) and PM2.5, and the dry depositions at a sample site at Luliao Junior High School (Luliao) in central Taiwan were measured during smog and non-smog days between December 2017 and July 2018. The results are compared to those obtained during non-smog periods in the years 2015–2017. The mean TSP and PM2.5 concentrations and dry deposition flux were 72.41?±?26.40, 41.88?±?23.51?μg/m3, and 797.57?±?731.46?μg/m2 min, respectively, on the smog days. The mean TSP and PM2.5 concentrations and dry deposition flux on the non-smog days were 56.39?±?18.08, 34.81?±?12.59?μg/m3 and 468.93?±?600.57?μg/m2 min, respectively. The mean TSP concentration in the smog period was 28% greater than that in the non-smog period, and the mean PM2.5 concentration was 20% higher. The mean dry deposition flux in the smog period was 70% higher than that in the non-smog period at Luliao. The PM2.5 concentrations exceeded the standards set by the Taiwan EPA (35?μg/m3 daily, and 15?μg/m3 annually). Therefore, the TSP and PM2.5 concentrations and dry deposition must be reduced in central Taiwan on smog days. In addition, atmospheric TSP and PM2.5 concentrations at various sampling sites were compared, and those herein were not higher than those measured in other countries. Finally, apart from the local traffic emissions, during smog periods, the other pollution source originated from the transportation process of traffic pollutants emitted in the northwest side of Taiwan. 相似文献
123.
将MODIS数据反演得出的气溶胶光学厚度与无锡市区实测得到的PM2.5质量浓度进行相关性分析,结果两者的直接相关性较低,相关系数为0.283 4。气溶胶光学厚度经垂直分布和湿度修正后,两者相关性显著提高,相关系数为0.565 9。虽然修正过程存在误差,相关性未达预期程度,但该方法得到的气溶胶光学厚度可作为PM2.5监测的有效补充。 相似文献
124.
Tianzeng Chen Yongchun Liu Biwu Chu Changgeng Liu Jun Liu Yanli Ge Qingxin M Jinzhu M Hong He 《环境科学学报(英文版)》2019,31(5):256-263
Current atmospheric quality models usually underestimate the level of ambient secondary organic aerosol(SOA), one of the possible reasons is that the precursors at different concentrations may undergo different oxidation processes and further affect SOA formation. Therefore, there is a need to perform more chamber studies to disclose the influence. In this work, SOA formation over a wide range of initial precursor concentrations(tens of ppb to hundreds of ppb levels) was investigated in a 30 m3 indoor smog chamber,and mainly through the analysis of multiple generations of VOCs detected from HR-To FPTRMS to expound the difference in the oxidation process between low and high precursor concentrations. Compared to high initial concentrations, gas-phase intermediates formed at low concentrations had a higher intensity by about one order of magnitude, and the lowvolatility compounds also had a higher formation potential due to the competition between semi-volatile intermediates and precursors with oxidants. In addition, the formed SOA was more oxidized with higher f44 value(0.14 ± 0.02) and more relevant to real atmosphere than that formed at high concentrations. This work should help to deeply understand SOA formation and improve the performance of air quality models for SOA simulation. 相似文献
125.
自然通风对办公室内气溶胶的影响 总被引:2,自引:0,他引:2
办公室间歇开窗自然通风可降低空内颗粒物和微生物的浓度,用TSI公司的气溶胶自动分析仪和FA-1型空气微生物采样器对样品测定结果表明,上午9:00室外大气颗粒物浓度高于室内,不宜开窗;10:30左右,室内颗粒物浓度增高,开窗自然通风效果好。 相似文献
126.
重庆城区气溶胶的理化特性 总被引:1,自引:0,他引:1
用大流量采样器在重庆市区内采集可吸入颗粒物(IP),对样品进行了多种分析,结果表明,IP的质量分布主要集中在3.0μm以下,占93.4%;IP中水溶物占53.4%,硫酸盐又占水溶物的60%;燃煤及汽车污染对IP的贡献为54%. 相似文献
127.
利用美国PC—2型气溶胶粒度分析仪,对淮南市的气溶胶现状进行厂流动监测,并研究其分布特征。结果表明,淮南市的气溶胶从西北向东南有明显的扩散趋势,最大浓度出现在早晨7~8时。大于1.0μm粒径的颗粒对气溶胶污染贡献较大。 相似文献
128.
129.
Georgiy Stenchikov Nilesh Lahoti David J. Diner Ralph Kahn Paul J. Lioy Panos G. Georgopoulos 《Environmental Fluid Mechanics》2006,6(5):425-450
The collapse of the world trade center (WTC) produced enhanced levels of airborne contaminants in New York City and nearby areas on September 11, 2001 through December, 2001. This catastrophic event revealed the vulnerability of the urban environment, and the inability of many existing air monitoring systems to operate efficiently in a crisis. The contaminants released circulated within the street canyons, but were also lifted above the urban canopy and transported over large distances, reflecting the fact that pollutant transport affects multiple scales, from single buildings through city blocks to mesoscales. In this study, ground-and space-based observations were combined with numerical weather forecast fields to initialize fine-scale numerical simulations. The effort is aimed at reconstructing pollutant dispersion from the WTC in New York City to surrounding areas, to provide means for eventually evaluating its effect on population and environment. Atmospheric dynamics were calculated with the multi-grid Regional Atmospheric Modeling System (RAMS), covering scales from 250 m to 300 km and contaminant transport was studied using the Hybrid Particle and Concentration Transport (HYPACT) model that accepts RAMS meteorological output. The RAMS/HYPACT results were tested against PM2.5 observations from the roofs of public schools in New York City (NYC), Landsat images, and Multi-angle Imaging SpectroRadiometer (MISR) retrievals. Calculations accurately reproduced locations and timing of PM2.5 peak aerosol concentrations, as well as plume directionality. By comparing calculated and observed concentrations, the effective magnitude of the aerosol source was estimated. The simulated pollutant distributions are being used to characterize levels of human exposure and associated environmental health impacts. 相似文献
130.
Tatu Anttila Veli-Matti Kerminen Markku Kulmala 《Atmospheric environment (Oxford, England : 1994)》2002,36(39-40)
In this theoretical investigation, we elucidated several factors governing the ability of organic, water-soluble vapours to participate into either the secondary organic aerosol formation or particle condensational growth in the atmosphere. The corresponding requirements for physico-chemical properties of the vapour were estimated. These estimates were also compared with the properties of several difunctional carboxylic acids identified in the atmosphere. Our analysis indicates that while many of the considered compounds are expected to contribute to the total particle mass in the atmosphere, their role in particle condensational growth process remains uncertain. This uncertainty emerges from the fact that the saturation ratio of an organic vapour does not alone determine its ability to act as a “nonvolatile” compound. Instead, the hygroscopic and chemical properties of the vapour, as well as the particle pH and size, have also to be taken into account. 相似文献