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81.
82.
Lance Wallace Cynthia Howard-Reed 《Journal of the Air & Waste Management Association (1995)》2013,63(7):828-844
Abstract Continuous monitors were employed for 18 months in an occupied townhouse to measure ultrafine, fine, and coarse particles; air change rates; wind speed and direction; temperature; and relative humidity (RH). A main objective was to document short-term and long-term variation in indoor air concentrations of size-resolved particles (0.01-20 μm) caused by (1) diurnal and seasonal variation of outdoor air concentrations and meteorological variables, (2) indoor sources such as cooking and using candles, and (3) activities affecting air change rates such as opening windows and using fans. A second objective was to test and compare available instruments for their suitability in providing real-time estimates of particle levels and ancillary variables. Despite different measuring principles, the instruments employed in this study agreed reasonably well for particles less than 10 μm in diameter. The three instruments measuring fine and coarse particles (aerodynamic diameter between 0.3 and 20 μm) agreed to within 30% in their overall estimates of total volume. Two of these instruments employed optical scattering, and the third used an aerodynamic acceleration principle. However, several lines of evidence indicated that the instrument employing aerodynamic acceleration overestimated concentrations for particle diameters greater than 10 μm. A fourth instrument measuring ultrafine and accumulation-mode particles (0.01-1 μm) was operated with two different inlets providing somewhat different particle size ranges. The two inlets agreed in the ultrafine region (<0.1 μm) but diverged increasingly for larger particles (up to 0.445 μm). Indoor sources affecting ultrafine particle concentrations were observed 22% of the time, and sources affecting fine and coarse particle concentrations were observed 12 and 15% of the time, respectively. When an indoor source was operating, particle concentrations for different sizes ranged from 2 to 20 times the average concentrations when no indoor source was apparent. Indoor sources, such as cooking with natural gas, and simple physical activities, such as walking, accounted for a majority (50-90%) of the ultrafine and coarse particle concentrations, whereas outdoor sources were more important for accumulation-mode particles between 0.1 and 1 um in diameter. Averaged for the entire year and including no periods when indoor sources were apparent, the number distribution was bimodal, with a peak at ~10 nm (possibly smaller), a shallow minimum at ~14 nm, and a second broad peak at ~68 nm. The volume distribution was also bimodal, with a broad peak at ~200 nm, a minimum at ~1.2 μm, and then an upward slope again through the remaining size fractions. A database was created on a 5-min averaging time basis. It contains more than 90,000 measurements by two of the instruments and approximately 30,000 by the two optical scattering instruments. About 4500 hour-long average air change rates were also calculated throughout the year using a dedicated gas chromatograph with electron capture detection (GC/ECD). At high air change rates [>0.8 air changes per hour (hr?1)], particle concentrations were either elevated (when no source was present) or depressed (when an indoor source was operating) by factors of up to 2 compared with low air change rates. 相似文献
83.
Robert C. Carr Wallace B. Smith 《Journal of the Air & Waste Management Association (1995)》2013,63(5):584-599
This is the fifth in a series of papers discussing the experience of electric utilities in applying baghouse technology for the collection of particulate matter at coal-fired electric power generating plants. The series presents new data obtained in research sponsored by the Electric Power Research Institute (EPRI) on reverse-gas and shake/deflate cleaned baghouses, and specifically addresses a number of unresolved issues in the design and operation of these units. This paper describes research to improve reverse-gas cleaning technology, and to characterize reverse-gas sonic assisted and shake/deflate cleaning. 相似文献
84.
Wheeler AJ Xu X Kulka R You H Wallace L Mallach G Van Ryswyk K MacNeill M Kearney J Dabek-Zlotorzynska E Wang D Poon R Williams R Stocco C Anastassopoulos A Miller JD Dales R Brook JR 《Journal of the Air & Waste Management Association (1995)》2011,61(2):142-156
The Windsor, Ontario Exposure Assessment Study evaluated the contribution of ambient air pollutants to personal and indoor exposures of adults and asthmatic children living in Windsor, Ontario, Canada. In addition, the role of personal, indoor, and outdoor air pollution exposures upon asthmatic children's respiratory health was assessed. Several active and passive sampling methods were applied, or adapted, for personal, indoor, and outdoor residential monitoring of nitrogen dioxide, volatile organic compounds, particulate matter (PM; PM < or = 2.5 microm [PM2.5] and < or = 10 microm [PM10] in aerodynamic diameter), elemental carbon, ultrafine particles, ozone, air exchange rates, allergens in settled dust, and particulate-associated metals. Participants completed five consecutive days of monitoring during the winter and summer of 2005 and 2006. During 2006, in addition to undertaking the air pollution measurements, asthmatic children completed respiratory health measurements (including peak flow meter tests and exhaled breath condensate) and tracked respiratory symptoms in a diary. Extensive quality assurance and quality control steps were implemented, including the collocation of instruments at the National Air Pollution Surveillance site operated by Environment Canada and at the Michigan Department of Environmental Quality site in Allen Park, Detroit, MI. During field sampling, duplicate and blank samples were also completed and these data are reported. In total, 50 adults and 51 asthmatic children were recruited to participate, resulting in 922 participant days of data. When comparing the methods used in the study with standard reference methods, field blanks were low and bias was acceptable, with most methods being within 20% of reference methods. Duplicates were typically within less than 10% of each other, indicating that study results can be used with confidence. This paper covers study design, recruitment, methodology, time activity diary, surveys, and quality assurance and control results for the different methods used. 相似文献
85.
Wayne Ott Lance Wallace David Mage 《Journal of the Air & Waste Management Association (1995)》2013,63(8):1390-1406
ABSTRACT This paper presents a new statistical model designed to extend our understanding from prior personal exposure field measurements of urban populations to other cities where ambient monitoring data, but no personal exposure measurements, exist. The model partitions personal exposure into two distinct components: ambient concentration and nonambient concentration. It is assumed the ambient and nonambient concentration components are uncorrelated and add together; therefore, the model is called a random component superposition (RCS) model. The 24-hr ambient outdoor concentration is multiplied by a dimensionless “attenuation factor” between 0 and 1 to account for deposition of particles as the ambient air infiltrates indoors. The RCS model is applied to field PM10 measurement data from three large-scale personal exposure field studies: THEES (Total Human Environmental Exposure Study) in Phillipsburg, NJ; PTEAM (Particle Total Exposure Assessment Methodology) in Riverside, CA; and the Ethyl Corporation study in Toronto, Canada. Because indoor sources and activities (smoking, cooking, cleaning, the personal cloud, etc.) may be similar in similar populations, it was hypothesized that the statistical distribution of nonambient personal exposure is invariant across cities. 相似文献
86.
Sigurdur Reynir Gislason Domenik Wolff-Boenisch Andri Stefansson Eric H. Oelkers Einar Gunnlaugsson Hólmfridur Sigurdardottir Bergur Sigfusson Wallace S. Broecker Juerg M. Matter Martin Stute Gudni Axelsson Thrainn Fridriksson 《International Journal of Greenhouse Gas Control》2010,4(3):537-545
In this paper we describe the thermodynamic and kinetic basis for mineral storage of carbon dioxide in basaltic rock, and how this storage can be optimized. Mineral storage is facilitated by the dissolution of CO2 into the aqueous phase. The amount of water required for this dissolution decreases with decreased temperature, decreased salinity, and increased pressure. Experimental and field evidence suggest that the factor limiting the rate of mineral fixation of carbon in silicate rocks is the release rate of divalent cations from silicate minerals and glasses. Ultramafic rocks and basalts, in glassy state, are the most promising rock types for the mineral sequestration of CO2 because of their relatively fast dissolution rate, high concentration of divalent cations, and abundance at the Earth's surface. Admixture of flue gases, such as SO2 and HF, will enhance the dissolution rates of silicate minerals and glasses. Elevated temperature increases dissolution rates but porosity of reactive rock formations decreases rapidly with increasing temperature. Reduced conditions enhance mineral carbonation as reduced iron can precipitate in carbonate minerals. Elevated CO2 partial pressure increases the relative amount of carbonate minerals over other secondary minerals formed. The feasibility to fix CO2 by carbonation in basaltic rocks will be tested in the CarbFix project by: (1) injection of CO2 charged waters into basaltic rocks in SW Iceland, (2) laboratory experiments, (3) studies of natural analogues, and (4) geochemical modelling. 相似文献
87.
James K. Sheppard Matthew Walenski Michael P. Wallace Juan J. Vargas Velazco Catalina Porras Ronald R. Swaisgood 《Behavioral ecology and sociobiology》2013,67(8):1227-1238
Populations of reintroduced California condors (Gymnogyps californianus) develop complex social structures and dynamics to maintain stable group cohesion, and birds that do not successfully integrate into group hierarchies have highly impaired survivability. Consequently, improved understanding of condor socioecology is needed to inform conservation management strategies. We report on the dominance structure of free-ranging condors and identify the causes and consequences of rank in condor populations by matching social status with the behavioral and physical correlates of individual birds. We characterized the hierarchical social structure of wild condor populations as mildly linear, despotic, and dynamic. Condor social groups were not egalitarian and dominance hierarchies regulated competitive access to food resources. Absence of kin-based social groups also indicated that condor social structure is individualistic. Agonistic interactions among condors were strongly unidirectional, but the overall linearity and steepness of their hierarchies was low. Although one aggressive male maintained the highest dominance rank across the 3-year observation period, there was considerable fluidity in social status among condors within middle and lower rank orders. Older condors were more dominant than younger birds and younger males supplanted older females over time to achieve higher status. Dominance rank did not predict the amount of time that a bird spent feeding at a carcass or the frequency that a bird was interrupted while feeding. Thus, younger, less dominant birds are able to obtain sufficient nutrition in wild social populations. 相似文献
88.
Judy L. Meyer David L. Strayer J. Bruce Wallace Sue L. Eggert Gene S. Helfman Norman E. Leonard 《Journal of the American Water Resources Association》2007,43(1):86-103
Abstract: The diversity of life in headwater streams (intermittent, first and second order) contributes to the biodiversity of a river system and its riparian network. Small streams differ widely in physical, chemical, and biotic attributes, thus providing habitats for a range of unique species. Headwater species include permanent residents as well as migrants that travel to headwaters at particular seasons or life stages. Movement by migrants links headwaters with downstream and terrestrial ecosystems, as do exports such as emerging and drifting insects. We review the diversity of taxa dependent on headwaters. Exemplifying this diversity are three unmapped headwaters that support over 290 taxa. Even intermittent streams may support rich and distinctive biological communities, in part because of the predictability of dry periods. The influence of headwaters on downstream systems emerges from their attributes that meet unique habitat requirements of residents and migrants by: offering a refuge from temperature and flow extremes, competitors, predators, and introduced species; serving as a source of colonists; providing spawning sites and rearing areas; being a rich source of food; and creating migration corridors throughout the landscape. Degradation and loss of headwaters and their connectivity to ecosystems downstream threaten the biological integrity of entire river networks. 相似文献
89.
While second-trimester prenatal screening programmes for Down's syndrome have become established in prenatal care, it would be advantageous to be able to offer screening in earlier preganancy. To this end, we have evaluated a new potential maternal serum marker, dimeric inhibin A, as a possible first-trimester marker. Dimeric inhibin A was measured in propsectively collected maternal serum from 23 cases of Down's syndrome and matched chromosomally normal controls, at 11–13 weeks' gestation. Levels of this protein were significantly elevated in the Down's pregnancies compared with the control pregnancies. The median multiple of the normal median (MOM) for the Down's samples was 2.46 (95 per cent confidence interval: 2.11–3.26, P<0.0001 vs. controls). These results suggest that dimeric inhibin A is a useful discriminator of Down's-affected pregnancies from normal pregnancies in the first trimester and that sensitive screening in combination with maternal age and other possible markers may be practicable in the first trimester. 相似文献
90.