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1.
Pre-concentration and separation of heavy metal ions by chemically modified waste paper gel 总被引:1,自引:0,他引:1
Iminodiacetic acid was immobilized on waste paper by chemical modification in order to develop a new type of adsorption gel for heavy metal ions. Adsorption behavior of the gel was investigated for a number of metal ions, specifically Cu(II), Pb(II), Fe(III), Ni(II), Cd(II), and Co(II) at acidic pH. From batch adsorption tests, the order of selectivity was found to be as follows: Cu(II) Fe(III) > Pb(II) > Ni(II) Co(II) > Cd(II). Column tests were carried out for pairs of metal ions to understand the separation and pre-concentration behavior of the gel. It was found that mutual separation of Ni(II) from Co(II) and that of Pb(II) from Cd(II) can be achieved at pH 3. Similarly, selective separation of Cu(II) from Cu(II)–Fe(III) and Cu(II)–Pb(II) mixtures at pH 1.5 and 2, respectively, was observed by using this new adsorption gel. In all cases, almost complete recovery of the adsorbed metal was confirmed by elution tests with HCl. 相似文献
2.
3.
Tone River supplies most of the water requirements of the Tokyo Metropolitan Area (TMA). Lowering of Tone flow and yearly
fluctuation, however, is causing water shortage along TMA nowadays. This study investigated the future water availability
scenarios under climatic changes. A state-of-the-art approach to utilize the output of several GCM has been demonstrated to
investigate the future water availability scenarios for TMA from the Tone River. An integrated modeling approach for water
balance considering several hydrological risk indices was adopted to quantify the future changes in this case. It is observed
that the future summer precipitation along the Tone basin is going to be increased considerably, while an almost constant
or decreasing trend is observed for winter season. Natural flow availability for winter or spring seasons thus can be crucial
under future scenarios. After reservoir routing, the hydrological risk indices estimated, however, were not found to be changed
significantly due to the presence of a robust reservoir system at the upstream. 相似文献
4.
A postanal tail is a major synapomorphy of the phylum Chordata, which is composed of three subphyla: Vertebrata, Cephalochordata,
and Tunicata (Urochordata). Among tunicates, appendicularians are the only group that retains the tail in the adult, and the
adult tail functions in locomotion and feeding in combination with a cellulose-based house structure. Given the phylogenetic
position of tunicates, the appendicularian adult tail may possess ancestral features of the chordate tail. We assess the ultrastructural
development of the tail epidermis of the appendicularian Oikopleura dioica. The epidermis of the larval tail is enclosed by the larval envelope, which is a thin sheet similar to the outer tunic layer
of ascidian larvae. The epidermis of the adult tail seems to bear no tunic-like cellulosic integuments, and the tail fin is
a simple folding of the epidermis. Every epidermal cell, except for the triangular cells at the edge of the tail fin, has
a conspicuous matrix layer of fibrous content in the apical cytoplasm without enclosing membranes. The epidermis of the larval
tail does not have a fibrous matrix layer, suggesting the production of the layer during larval development and metamorphosis.
Zonulae adhaerentes firmly bind the epidermal cells of the adult tail to one another, and the dense microfilaments lining
the cell borders constitute a mechanical support for the cell membranes. The intracellular matrix, cell junctions, and cytoskeletons
probably make the tail epidermis a tough, flexible shell supporting the active beating of the oikopleuran adult tail. 相似文献
5.
Minoru Ichihara Keisuke Maruyama Masayuki Yamashita Hitoshi Sawada Hidehiro Inagaki Yoshiki Ishida Motoaki Asai 《Agriculture, ecosystems & environment》2011,140(1-2):191-198
The extent of post-dispersal weed seed predation in upland wheat fields converted from paddy fields was quantified in Shizuoka Prefecture, central Japan. We investigated the temporal variability in seed predation of Italian ryegrass (Lolium multiflorum Lam.), a non-native winter annual weed in Japan, during summer after the seed shed in both the field interior areas and boundary strips, and estimated the total seed loss due to predation during the summer. Furthermore, the contribution of invertebrates and vertebrates to seed predation was estimated by using exclosures. The total seed loss due to predation during four months (from late June to late October) in the field interior areas and boundary strips was estimated to be 35–43% (the maximum proportion of seed predation per two weeks = 27%) and 42% (25%), respectively. The seed predators in the field interior areas were vertebrates (rodents or birds) and invertebrates (crickets and ground beetles). In contrast, seed predators in the boundary strips were mainly invertebrates (crickets and ground beetles). The results of this study suggest that predators make a substantial contribution in the depletion of post-dispersal seeds of Italian ryegrass in converted paddy fields. 相似文献
6.
Nina Y. Ileva Hideaki Shibata Fuyuki Satoh Kaichiro Sasa Hiroshi Ueda 《Sustainability Science》2009,4(2):189-198
The present research investigated the relationship between nitrate–nitrogen (NO3–N) in river water and the land use/land cover (hereafter, land use) in the Teshio River watershed located in northern Hokkaido
island to understand the effect of human activities such as agriculture, forestry, industry, and urbanization in the drainage
basin on the river ecosystem quality and services. River water was sampled at nine points seasonally during a 2-year period
and the nutrients concentration was measured. Land use profiles were estimated at two spatial scales, riparian and sub-catchment,
for each sampling station. The spatial pattern of water quality in the Teshio River showed increased NO3–N levels associated with agriculture and urban expansion, and forest reduction in the watershed. Land use at the riparian
scale closely reflected that at the sub-catchment scale, which masked the unique riparian buffer effect on the river water
condition. The increased agricultural and reduced forest area in the riparian zone, especially in the upper middle reach,
could be a possible reason for a decline of ecosystem service for the provisioning of clean water and habitat for aquatic
organisms. Measures towards sustainable and more nature-friendly agricultural management are necessary in the area to protect
the Teshio River ecosystem and its ecosystem services. 相似文献
7.
Dietary patterns and blood levels of PCDDs, PCDFs, and dioxin-like PCBs in 1656 Japanese individuals
Arisawa K Uemura H Hiyoshi M Kitayama A Takami H Sawachika F Nishioka Y Hasegawa M Tanto M Satoh H Shima M Sumiyoshi Y Morinaga K Kodama K Suzuki T Nagai M 《Chemosphere》2011,82(5):656-662
The association between dietary patterns and blood dioxin levels has not been fully investigated. The present study population consisted of 755 men and 901 women (aged 15-73 years) living in 90 different areas of 30 prefectures of Japan. Dietary habits were assessed by inquiring about the consumption frequency of 28 foods, food groups and beverages. In addition, the blood levels of 29 polychlorinated dibenzo-p-dioxins (PCDDs), polychlorinated dibenzo-furans (PCDFs), and dioxin-like polychlorinated biphenyl (DL-PCBs) congeners were determined by high-resolution gas chromatography/mass spectrometry. The median total toxicity equivalent (TEQ) in the blood, which was calculated on the basis of the toxicity equivalency factors of WHO (2005), was 16 pg TEQ g−1 lipid. Principal component analysis identified five dietary patterns: Healthy diet (high intake of vegetables and fruits); Meat/High fat intake (high intake of meat, meat products, and eggs); Seafood and Alcohol (high intake of fish, shellfish, and alcoholic beverages); Miscellaneous; and Milk products and Alcohol intake (high intake of milk, Milk products, and alcoholic beverages). After adjusting for sex, age, body mass index, and smoking habits, the Seafood and Alcohol pattern scores were significantly related to higher blood levels of total TEQ and PCDDs/PCDFs/DL-PCBs, and the Milk products and Alcohol pattern scores were correlated with higher blood levels of DL-PCBs. More detailed analysis showed that the intake frequencies for alcoholic beverages and seafood were independently and positively associated with total TEQ and the TEQ of PCDFs and DL-PCBs. The association between alcoholic beverage intake and PCDDs was also significant. Analysis of dietary patterns may be useful for identifying the dietary characteristics of individuals with a high dioxin body burden. 相似文献
8.
9.
Fuminori Hashihama Haruko Umeda Chiaki Hamada Sakae Kudoh Toru Hirawake Kazuhiko Satoh Mitsuo Fukuchi Yasuhiro Kashino 《Marine Biology》2010,157(10):2263-2278
In high-latitude waters such as the Southern Ocean, the primary production of phytoplankton supports the ecosystem. To understand
the photo-acclimation strategy of such phytoplankton within cold environments, the vertical distribution profile of photosynthetic
pigments was analyzed in the Southern Ocean. Samples were taken along 110°E during the austral summer, and along 150°E and
around the edge of the seasonal sea ice of the Antarctic Continent during the austral autumn. Pigment extraction methods were
optimized for these samples. The standing crop of chlorophyll a was larger in the region along the edge of the seasonal sea ice than at sampling stations in open ocean areas. Chlorophyll
concentration seemed to be dependent on the formation of thermo- and haloclines along the edge of the seasonal sea ice, but
not in the open ocean where such clines are less pronounced. The marker pigments fucoxanthin and/or 19′-hexanoyloxyfucoxanthin
were dominant at most sampling stations throughout the water column, while other marker pigments such as alloxanthin were
quite low. This indicated that diatoms and/or haptophytes were the major phytoplankton in this area. Comparison of the relative
ratio of fucoxanthin with that of 19′-hexanoyloxyfucoxanthin allowed some stations to be characterized as either diatom-dominant
or haptophyte-dominant. The relative ratio of xanthophyll-cycle pigments (diadinoxanthin plus diatoxanthin) to chlorophyll
a was high in surface waters and decreased gradually with depth. This suggests that near the ice edge during summer in the
Southern Ocean, both diatoms and haptophytes acclimate to their light environments to protect their photosystems under high-light
conditions. 相似文献
10.
Katsuya Nakayama Kuchar Dalibor Keisuke Sakai Mitsuhiro Kubota Hitoki Matsuda 《Journal of Material Cycles and Waste Management》2008,10(2):102-109
The present work focuses on investigation of the effective recovery of heavy metals from molten fly ash by applying chloride-induced
volatilization. In particular, the effect of unburned carbon on the chloride-induced volatilization of lead, zinc, and copper
from model and real molten fly ashes was investigated in the temperature range 873–1173 K under a N2 atmosphere. As a result, almost 100% of lead and a significant proportion of zinc were volatilized from the real molten fly
ash samples at 1173 K. In contrast, for the model fly ash, volatilization ratios of lead and zinc at 1173 K were only 85%
and 25%, respectively. Further, the results of X-ray diffraction analysis suggested that PbO in molten fly ash was converted
either to Pb2OCl2 or Pb by respective chlorination and reduction reactions. Meanwhile ZnO and CuO in the molten fly ash were reduced to Zn
and Cu by reaction with unburned carbon. Subsequently, Pb, Zn, and Pb2OCl2 were volatilized, but Cu remained in the solid residue. Finally, the volatilization ratio of zinc increased with the addition
of carbon, and more than 98% of zinc was volatilized at 1173 K from a fly ash with a carbon content of 20%. 相似文献