Discharge of 137Cs and 90Sr by Finnish rivers to the Baltic Sea in 1986-1996

The total amounts of 137Cs and 90Sr transported from Finland by rivers into the Gulf of Finland, Gulf of Bothnia and Archipelago Sea since 1986 were estimated. The estimates were based on long-term monitoring of 137Cs and 90Sr in river and other surface waters and on the statistics of water discharges from Finnish rivers to the above sub-areas of the Baltic Sea. The total amounts of 137Cs and 90Sr removed from Finland into the Baltic Sea during 1986-1996 were estimated to be 65 and 10 TBq, respectively. The results show that, although the deposition of 137Cs was much higher than that of 90Sr after the Chernobyl accident, the amount of 137Cs removed from Finland is only six times as high as that of 90Sr. This emphasizes the importance of 90Sr while considering radiation doses from surface waters and 137Cs while estimating doses via pathways from catchment soil, lake sediments and biota after a fallout situation.     

Isotope tracing of submarine groundwater discharge offshore Ubatuba, Brazil: results of the IAEA–UNESCO SGD project

Results of groundwater and seawater analyses for radioactive (³H, ²²²Rn, ²²³Ra, ²²⁴Ra, ²²⁶Ra, and ²²⁸Ra) and stable (D and ¹⁸O) isotopes are presented together with in situ spatial mapping and time series ²²²Rn measurements in seawater, direct seepage measurements using manual and automated seepage meters, pore water investigations using different tracers and piezometric techniques, and geoelectric surveys probing the coast. This study represents first time that such a new complex arsenal of radioactive and non-radioactive tracer techniques and geophysical methods have been used for simultaneous submarine groundwater discharge (SGD) investigations. Large fluctuations of SGD fluxes were observed at sites situated only a few meters apart (from 0 cm d⁻¹ to 360 cm d⁻¹; the unit represents cm³/cm²/day), as well as during a few hours (from 0 cm d⁻¹ to 110 cm d⁻¹), strongly depending on the tidal fluctuations. The average SGD flux estimated from continuous ²²²Rn measurements is 17 ± 10 cm d⁻¹. Integrated coastal SGD flux estimated for the Ubatuba coast using radium isotopes is about 7 × 10³ m³ d⁻¹ per km of the coast. The isotopic composition (δD and δ¹⁸O) of submarine waters was characterised by significant variability and heavy isotope enrichment, indicating that the contribution of groundwater in submarine waters varied from a small percentage to 20%. However, this contribution with increasing offshore distance became negligible. Automated seepage meters and time series measurements of ²²²Rn activity concentration showed a negative correlation between the SGD rates and tidal stage. This is likely caused by sea level changes as tidal effects induce variations of hydraulic gradients. The geoelectric probing and piezometric measurements contributed to better understanding of the spatial distribution of different water masses present along the coast. The radium isotope data showed scattered distributions with offshore distance, which imply that seawater in a complex coast with many small bays and islands was influenced by local currents and groundwater/seawater mixing. This has also been confirmed by a relatively short residence time of 1–2 weeks for water within 25 km offshore, as obtained by short-lived radium isotopes. The irregular distribution of SGD seen at Ubatuba is a characteristic of fractured rock aquifers, fed by coastal groundwater and recirculated seawater with small admixtures of groundwater, which is of potential environmental concern and has implications on the management of freshwater resources in the region.     

Current Contents of 90Sr and 137Cs in the Moss–Lichen Cover of Piedmont and Mountain Landscapes of the Northern Urals

The contents of long-lived artificial radionuclides, ⁹⁰Sr and ¹³⁷Cs, were determined in lichens and mosses of different taxa and in the samples of moss–lichen cover taken from the mountain and lowland plant communities of the Northern Urals. The effects of Chernobyl fallout and the dynamics of radionuclide contents in lichens and mosses were analyzed. The concentration of ¹³⁷Cs in the moss–lichen cover was higher in the mountain ecosystems than in the lowland plant communities.     

Foliar uptake of Cs from the water column by aquatic macrophytes

A transplant experiment was performed to determine the relative importances of root uptake from the sediments and foliar uptake from the water column in determining the accumulation of ¹³⁷Cs by aquatic macrophytes. Uncontaminated individuals of three species, Brasenia schreberi, Nymphaea odorata and Nymphoides cordata, were transplanted into pots containing either contaminated sediments (i.e. 1.2 Bq ¹³⁷Cs g⁻¹ dry mass) or uncontaminated sediments (i.e. < 0.1 Bq g⁻¹ dry mass) and immersed in Pond B, a former reactor cooling pond where ¹³⁷Cs concentrations in surface waters range from 0.4 to 0.8 Bq liter⁻¹. The plants in uncontaminated sediments rapidly accumulated ¹³⁷Cs from the water column and after 35 days of immersion had ¹³⁷Cs concentrations in leaves that were: (1) not statistically significantly different from those for plants in contaminated sediments; and (2) similar to those for the same species growing naturally in Pond B. The similarity in ¹³⁷Cs concentrations between naturally-occurring plants and those in pots with uncontaminated sediments suggests that foliar uptake from the water column is the principal mode of Cs accumulation by these species in Pond B.     

137Cs in marine samples from the Brazilian southeastern coastal region

The present work presents the results of ¹³⁷Cs concentration in seawater, fish and sediments samples collect in 11 sampling points, crossing the Brazilian Southeastern coastal region, from Vitória (ES) to Santos (SP), on a routine basis from 1997 to 2002. This monitoring program was carried out by the Instituto de Radioproteção e Dosimetria (IRD/CNEN/MCT), in cooperation with the Instituto de Estudos do Mar Almirante Paulo Moreira (IEAPM/Brazilian Navy), aiming at determining artificial radionuclides in marine samples. Additionally to the ¹³⁷Cs results, ⁹⁰Sr concentrations in fish samples from 1998 to 2002 are also reported.The ¹³⁷Cs in seawater follows a lognormal distribution, with a geometric mean of 1.8 Bq m^-3 and a geometric standard deviation of 1.4 (n=54), decay corrected to June/2002. For ¹³⁷Cs levels in fish samples a geometric mean of 0.19 Bq kg⁻¹ and a geometric standard deviation of 2.9 (n=39), decay corrected to June/2002, with a range of 0.03 to 1.7 Bq kg⁻¹, were obtained. Based on the ¹³⁷Cs mean concentration in fish as well as in seawater, a transfer factor of 1 × 10² was calculated, which is quite in agreement with the recommended value found in the Safety Report Serie 19.     

Sedimentation of cobalt-60 and caesium-137 released in Träven, a Baltic bay

The amounts of cobalt-60 and caesium-137 bound in the sediment in a bay off the Studsvik research station were determined. Of the cumulative released activity during 22 years, 19% of ⁶⁰Co and 1.8% of ¹³⁷Cs were found in the sediments within an area of 23 km². The rate of input through sedimentation and the loss rate through physical decay were of the same order in 1981 and were close to steady state for ⁶⁰Co while for ¹³⁷Cs they had only reached 30% of that level. The sedimentation coefficients calculated for the bay were 6·5 year⁻¹ for ⁶⁰Co and 0·49 year⁻¹ for ¹³⁷Cs, higher values than many published previously. Cobalt-60 seemed to precipitate close to the outlet and to migrate near the bottom as bed-load.     

Foliar and root uptake of Cs, Sr and Zn in processing tomato plants (Lycopersicon esculentum Mill.)

The results of an experimental study on the behaviour of ¹³⁴Cs, ⁸⁵Sr and ⁶⁵Zn in processing tomato plants grown in peat substrate are presented. Plants were contaminated by wet deposition of ¹³⁴Cs, ⁸⁵Sr and ⁶⁵Zn, either by sprinkling the above ground part at two phenological stages or by administering ¹³⁴Cs, ⁸⁵Sr and ⁶⁵Zn to the soil. The plants contaminated at the second phenological stage intercepted 38.3% less than those contaminated at the first stage, although leaf area increased by more than double. Transfer coefficients from peat soil to ripe fruit for ¹³⁴Cs are significantly higher than those for ⁸⁵Sr and ⁶⁵Zn. Leaf to fruit transfer coefficients for ¹³⁴Cs are one order of magnitude higher than for ⁶⁵Zn and two orders higher than for ⁸⁵Sr. Only when deposition affects fruits, as at the second phenological stage, are transfer coefficients to fruits similar for the three radionuclides.     

Migration of Cs and Sr in undisturbed soil profiles under controlled and close-to-real conditions

Migration of ¹³⁷Cs and ⁹⁰Sr in undisturbed soil was studied in large lysimeters three and four years after contamination, as part of a larger European project studying radionuclide soil–plant interactions. The lysimeters were installed in greenhouses with climate control and contaminated with radionuclides in an aerosol mixture, simulating fallout from a nuclear accident. The soil types studied were loam, silt loam, sandy loam and loamy sand. The soils were sampled to 30–40 cm depth in 1997 and 1998. The total deposition of ¹³⁷Cs ranged from 24 to 45 MBq/m², and of ⁹⁰Sr from 23 to 52 MBq/m². It was shown that migration of ¹³⁷Cs was fastest in sandy loam, and of ⁹⁰Sr fastest in sandy loam and loam. The slowest migration of both nuclides was found in loamy sand. Retention within the upper 5 cm was 60% for both ¹³⁷Cs and ⁹⁰Sr in sandy loam, while in loamy sand it was 97 and 96%, respectively. In 1998, migration rates, calculated as radionuclide weighted median depth (migration centre) divided by time since deposition were 1.1 cm/year for both ¹³⁷Cs and ⁹⁰Sr in sandy loam, 0.8 and 1.0 cm/year, respectively, in loam, 0.6 and 0.8 cm/year in silt loam, and 0.4 and 0.6 cm/year for ¹³⁷Cs and ⁹⁰Sr, respectively, in loamy sand. A distinction is made between short-term migration, caused by events soon after deposition and less affected by soil type, and long-term migration, more affected by e.g. soil texture. Three to four years after deposition, effects of short-term migration is still dominant in the studied soils.     

Distribution of radionuclides among the main components of Lake Chervyanoe in the Eastern Ural Radioactive Trace

Radioecological conditions have been estimated in Lake Chervyanoe located on the central axis of the Eastern Ural Radioactive Trace (EURT) about 100–110 km northeast of the Mayak Production Association. Data on the ⁹⁰Sr and ¹³⁷Cs contents in the main components of the lake, the distribution of these radionuclides over the profile of bottom sediments, and their amounts in the lake are presented. The experimental data have been used to construct mathematical models for estimating changes in the radionuclide concentrations and amounts in the water and bottom sediments of the lake over a long period after the nuclear accident, as well as the tritium content of the lake water in different periods of time.     

Migration of Cs in tributaries,lake water and sediment of Lago Maggiore (Italy,Switzerland) – analysis and comparison with Lago di Lugano and other lakes

This paper describes the behaviour of ¹³⁷Cs in Lago Maggiore and other pre-alpine lakes as a consequence of atmospheric nuclear weapons testing fallout and the fallout from the nuclear accident in Chernobyl. It presents data on the ¹³⁷Cs distribution in tributaries, lake water, bottom sediments and reveals the role of ¹³⁷Cs as a marker of the sedimentation processes. The run-off of ¹³⁷Cs from the watershed to the lake is described with a simple compartment model. Measurements of the activity concentration of ¹³⁷Cs in sediments are compared with the output of a model (diffusion–convection type) which describes the input of ¹³⁷Cs into and its vertical distribution within the sediment. Varying sedimentation rates (0.05–0.90 g (cm² y)⁻¹) in Lago Maggiore are compared with data of other authors. Sedimentation rates and total distribution coefficients (of about 10⁵ L kg⁻¹) in Lago Maggiore are discussed and compared with those of Lago di Lugano, Lake Constance, and Lake Vorsee.     

Mineral content of drinking water in lowland papua

This study presents concentration of nine minerals (Na, K, Mg, Ca, Cl, Mn, Zn, Cd, Pb) in 31 drinking water samples collected in the Papua New Guinea lowland, where coastal villagers draw water from artificial wells blended with sea water, riverside villagers utilize brackish river water, and inland villagers fetch creek or swamp water whose chemical composition is close to rain water. During the dry season, the coastal well water contains 500 mgL⁻¹ of sodium and 50–90 μgL⁻¹ of lead. The inland creek or swamp water contains very small amount of minerals; on the average, for instance, 0.64 mgL⁻¹ of magnesium, 0.84 mgL⁻¹ of calcium, and 4.78 mgL⁻¹ of water hardness (as CaCO₃). From some epidemiological evidence in industrialized countries, these mineral concentrations are judged to be indicative of high risk of cardiovascular disorders.     

Effect of liming on the behaviour of (90)Sr and (137)Cs in a lake ecosystem

Liming of lakes is considered one possible remedial action to reduce the accumulation of radionuclides into fish in the case of a radiological accident. These responses were tested in field conditions in a small acidified lake that was divided into two parts: one limed with CaCO₃ and the other half left as an unlimed control. The transfer of ⁹⁰Sr from water into fish decreased on average by 50% during the first year after liming. However, at the same time the ⁹⁰Sr concentration in water increased, reaching a maximum within 6 months after liming. Approximately 50% more ⁹⁰Sr was detected in water in the limed part of the lake than on control side during the first year. ⁹⁰Sr was most probably released from the sediment as the Ca concentration and pH of the water increased. As a result of these two processes, which counterbalanced each other (increased release of ⁹⁰Sr into water from sediment and decreased transfer of ⁹⁰Sr from water into fish), the ⁹⁰Sr concentration in fish did not notably differ between the limed and control sides of the lake. Liming may only be suitable as a remedial action if carried out immediately after a radiological accident, before significant amounts of radionuclides have been deposited in lake sediments. In the case of ¹³⁷Cs, the effect of liming was less pronounced. ¹³⁷Cs activity concentration in water increased in the first year by 20% and uptake by fish decreased by 20%.     

Association of organic matter, iron and inorganic phosphorus in lake waters

Gel permeation chromatography was used to fractionate ³²PO₄³⁻ labelled components by molecular size in filtered, destabilized lake foam, concentrated lake water, and lake sediment extracts. Evidence is presented for the abiotic formation of organic matter iron inorganic P complexes in lake foam, water and sediments. ³²PO₄^staggered was found to excahnge with low molecular weight, dissolved P fraction, probably an organic matter -Fe- inorganic P complex, but not with a high molecular weight, non-inorganic dissolved reactive P pool, hypothesized to be similar to the dimer. Our experiments suggest that inorganic P binding by high molecular weight organic matter may play a significant role in the P cycle. If the bound P is unavailable to algae and bacteria, the complexes could explain Rigler's (1968) hypothesis that the molybdenum blue technique may overestimate the free orthophosphate concentration by 10–100 times.     

Microbial extracellular enzyme activities in Humex Lake Skjervatjern

Two microbial extracellular enzyme activities (MEEA) were studied in HUMEX Lake Skjervatjern: acid phosphatase (APHA) and leucine aminopeptidase (LeuAMPA). Both enzyme activities varied in the vertical and horizontal scale in both lake sites. APHA varied in the acidfied Basin A between 945–1706 nmol L⁻¹ h⁻¹ and LeuAMPA between 3.7–25 nmol L⁻¹ h⁻¹. Both MEEA reached maxima in 0.5 m depth. In the control site (Basin B), APHA was lower by a factor of two, and varied between 156–669 nmol L⁻¹ h⁻¹. LeuAMPA reached similar values as in Basin A and varied between 7.8–34.8 nmol L⁻¹ h⁻¹. Maxima of APHA were found in the upper layer (0–2 m), while LeuAMPA had only one distinct maxima at 2–2.5 m depth. The number of bacteria (AFDC) varied between 4.4–8.8 10⁶ cells mL⁻¹ and was not significantly different in either side, but both had maxima in the thermocline. Highest specific LeuAMPA activities were found in the thermocline (3.2–4.5 fmol L⁻¹ h⁻¹ cell⁻¹) in both sides and varied between 0.4–4.5 fmol L⁻¹ h⁻¹ cell⁻¹ in both water columns. The main contributor (60–70%) to LeuAMPA was found in the microplankton fraction, retained on Nuclepore filters with pore sizes between 2.0-0.2 μm. APHA was retained less even on a filter with pore size smaller than 0.2 μm. About 50–70% of APHA passed through 0.2 μm-0.1 μm Nuclepore filters and could be found in the dissolved organic matter (DOM) fraction. APHA and bacteria counts (AFDC) showed a distinct gradient from the littoral zone to the pelagial in the surface water samples (0.2 m depth). APHA and LeuAMPA are regarded as important regulators for nutrient availability to microplankton. However, all data from vertical as important regulators for nutrient availability to microplankton. However, all data from vertical and horizontal samples showed that Lake Skjervatjern is a strongly gradient-dominated aquatic ecosystem. Watershed-littoral effects are more pronounced in the shallow, acidified Basin A than in the control side, Basin B.     

Effects of radionuclide and rainfall characteristics on field loss parameters of grass

The decrease of foliar activity in vegetation after its initial contamination by foliar deposition is termed “field loss” (Chamberlain, 1970). This work investigated further laboratory data concerning field loss of ¹³⁴Cs, ¹³⁷Cs, ⁸⁵Sr, ¹³³Ba and ^123mTe deposited on grassland (Madoz-Escande et al., 2005). Treatments consisted in rainfall scenarios cumulating 14 mm per week, combining two levels of intensity (8 or 30 mm/h) and two levels of frequency/precocity (late once or early twice-a-week). The time course of field loss was monitored in the edible tissues which were sampled by mowing between the rainfalls. Data were analyzed with an offset exponential loss model which is applicable to chronic contamination and is consistent with approaches adopted in radiological assessment models. Its parameters were estimated by the maximum-likelihood method, and their accuracy was determined by nonparametric boostrap. Radionuclide and rainfall conditions significantly affected the estimated rate (λ₁) and extent (A₁) of field loss. Field loss rate (λ₁) and nonentrainable fraction (1 − A₁) varied by a factor 1.5–3. Cesium was very mobile but persistent. On the contrary Tellerium was found less labile, but eventually was almost completely eliminated. Strontium and Barium had intermediate behaviors. Field loss was more efficient for moderate late once-a-week rainfalls (8 mm/h). Higher rainfall intensity reduced more the radionuclides losses than higher rainfall frequency/precocity. This paper reports statistically relevant effects that should be considered for more realistic assessments.     

Screening of household products for the emission of volatile organic compounds

10 household products, eight waxes or polishes, and two detergents have been screened by a headspace technique for the emission of volatile organic compounds (VOC). Using Tenax sampling and analysis by combined gas chromatography-mass spectrometry (GC-MS) more than 80 single compounds or groups of isomers have been identified, and semiquantitative data on the initial emission rates (emission rate immediately after application) have been obtained. Products fall into two groups: those containing water as a main (80 to 90%) constituent and those without water. The initial emission rate of the first group ranged from 0.2 to 2 μg cm⁻²min⁻¹, whereas the second group had higher emission rates of up to 430 μg cm⁻²min⁻¹. Products of the second group emit essentially hydrocarbons (alkanes, alkenes, and terpenes), whereas most products of the first group emit oxygenated compounds including terpene alcohols and their acetates, aliphatic alcohols and esters, and alkoxy-alcohols.     

Variability of the sorption of Cs, Zn, Sr, Co, Cd, Ce, Ru, Tc and I at trace concentrations by a forest soil along a transect

The variability of the sorption properties (characterized by the distribution coefficient K_d) of a forest soil for Cs, Zn, Sr, Co, Cd, Ce, Ru, Tc, and I were determined along a transect of 150 m in regular intervals of 3 m. Radioactive tracers were used to ensure trace concentrations of these elements. For comparison, for each soil sample the loss on ignition, as a measure of the soil organic matter content, and the pH were also determined. On average, the K_d values increase in the sequence Tc < I < Ru ≈ Co ≈ Zn ≈ Sr < Cd < Ce < Cs; the spatial variability in the sequence I < Zn ≈ Sr ≈ Co ≈ Cd ≈ Ru ≈ Tc < Cs, and I ≈ Ce < Tc. Correlation analysis revealed that, when moving along the transect, the K_d values for some elements changed in a similar, and for others in a dissimilar pattern. In a few cases a correlation between the pH or the loss on ignition and the K_d values was also present. The spatial structure of the data was examined by semivariograms. For the elements Co, Cd, Zn, and Sr, the K_d values showed an almost periodic behaviour along the transect, which is probably due to periodic changes of some soil properties in a forest with regularly spaced trees.     

Cesium and strontium sorption by selected tropical and subtropical soils around nuclear facilities

The dynamics of Cs and Sr sorption by soils, especially in the subtropics and tropics, as influenced by soil components are not fully understood. The rates and capacities of Cs and Sr sorption by selected subtropical and tropical soils in Taiwan were investigated to facilitate our understanding of the transformation and dynamics of Cs and Sr in soils developed under highly weathering intensity. The Langmuir isotherms and kinetic rates of Cs and Sr sorption on the Ap1 and Bt1 horizons of the Long-Tan (Lt) and the A and Bt1 horizons of the Kuan-Shan (Kt), Mao-Lin (Tml) and Chi-Lo (Cl) soils were selected for this study. Air-dried soil (<2 mm) samples were reacted with of 7.5 × 10⁻⁵ to 1.88 × 10⁻³ M of CsCl (pH 4.0) or 1.14 × 10⁻⁴ to 2.85 × 10⁻³ M of SrCl₂ (pH 4.0) solutions at 25 °C. The sorption maximum capacity (q_m) of Cs by the Ap1 and Bt1 horizons of the Lt soil (62.24 and 70.70 mmol Cs kg⁻¹ soil) were significantly (p < 0.05) higher than those by the A and Bt1 horizons of the Kt and Cl soils (26.46 and 27.49 mmol Cs kg⁻¹ soil in Kt soil and 34.83 and 29.96 mmol Cs kg⁻¹ soil in Cl soil, respectively), however, the sorption maximum capacity values of the Lt and Tml soils did not show significant differences. The amounts of pyrophosphate extractable Fe (Fe_p) were correlated significantly with the Cs and Sr sorption capacities (for Cs sorption, r² = 0.97, p < 1.0 × 10⁻⁴; for Sr sorption, r² = 0.82, p < 2.0 × 10⁻³). The partition coefficient of radiocesium sorbed on soil showed the following order: Cl soil ? Kt soil > Tml soil > Lt soil. It was due to clay minerals. The second-order kinetic model was applied to the Cs and Sr sorption data. The rate constant of Cs or Sr sorption on the four soils was substantiality increased with increasing temperature. This is attributable to the availability of more energy for bond breaking and bond formation brought about by the higher temperatures. The rate constant of Cs sorption at 308 K was 1.39-2.09 times higher than that at 278 K in the four soils. The activation energy of Cs and Sr sorbed by the four soils ranged from 7.2 to 16.7 kJ mol⁻¹ and from 15.2 to 22.4 kJ mol⁻¹, respectively. Therefore, the limiting step of the Cs⁺ or Sr²⁺ sorption on the soils was diffusion-controlled processes. The reactive components, which are significantly correlated with the Langmuir sorption maxima of Cs and Sr by these soils, substantially influenced their kinetic rates of Cs and Sr sorption. The data indicate that among components of the subtropical and tropical soils studied, short-range ordered sesquioxides especially Al- and Fe-oxides complexed with organics play important roles in influencing their capacity and dynamics of Cs and Sr sorption.     

Growth response of Scenedesmus to different concentrations of copper, cadmium, nickel, zinc, and lead

The fresh water alga Scenedesmus was cultured in graded concentration of Cu, Cd, Ni, Zn, and Pb to evaluate the effect of these cations on the growth response of Scenedesmus. The effective concentration of metal which depressed the Scenedesmus growth for Cu was 0.5 mg l⁻¹, for Cd 0.5 mg l⁻¹, for Ni 2 mg l⁻¹, and for Zn 2 mg l⁻¹. The alga exhibited tolerance for high Pb concentrations up to 30 mg l⁻¹. Exposure of a Scenedesmus cell to each metal revealed anatomical changes and chloroplast disruption especially at high metal concentrations.     

Inventories of Pu, Cs, and excess Pb in sediments from freshwater and brackish lakes in Rokkasho, Japan, adjacent to a spent nuclear fuel reprocessing plant

We investigated the vertical profiles of ^239+240Pu, ¹³⁷Cs, and excess ²¹⁰Pb (²¹⁰Pb_ex) in sediment core samples obtained from two freshwater lakes and two brackish lakes situated near the first commercial spent nuclear fuel reprocessing plant in Rokkasho, Japan, before the final test of the plant using actual spent nuclear fuel. The inventory of ^239+240Pu in those lakes was larger than that in soil in Rokkasho, which indicated the inflow of ^239+240Pu from the catchment area in addition to direct deposition on the lake surfaces. The ¹³⁷Cs inventory in sediments of the brackish lakes was lower than that in the soil, which showed that part of the ¹³⁷Cs was removed from the sediments by the brackish water or that it was not deposited into the sediments, because of the high solubility of Cs in brackish water. The ¹³⁷Cs inventory in sediments of the freshwater lakes was higher than that of the brackish lakes, and comparable with that in soil except for one core sample out of four. The ^239+240Pu/¹³⁷Cs ratio in freshwater lake sediments was higher than that in soil, and that indicated that part of the ¹³⁷Cs was lost from the sediments. The low inventory of ¹³⁷Cs may be attributable to competition for absorption sites in sediments with ammonium ions formed in the reducing environment which occurs from summer to fall in the sediments. Those data will be used as background data on the artificial radionuclides in the lakes to assess the effect of released radionuclides on their concentrations.