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1.
In the framework of a 222Rn screening campaign that was carried out in 58 public secondary schools in Galicia (NW Spain), the largest radon-prone area in the Iberian Peninsula, a positive correlation between indoor 222Rn concentration and outdoor gamma exposure rate was obtained. A new approach to the data acquisition in screening surveys was tested, improving the performances of this type of study and gathering useful data for future remedial actions. Using short-period detectors (charcoal canisters) firstly, in order to detect places showing 222Rn concentrations over 400 Bq m−3, the number of locations to be measured with long-period detectors (etched track detectors) is reduced. In this screening campaign, 34% of the schools surveyed presented at least one site exceeding the 400 Bq m−3 recommended action level established by the EU, and 15% had at least one site with 222Rn values over 800 Bq m−3. The maximum value recorded was 2084 ± 63 Bq m−3. These results are discussed and compared with data obtained in schools of several countries with similar geology. Seven schools were also studied for seasonal variations of 222Rn activity concentration. The results were not conclusive, and no significant correlation between season and 222Rn concentration was established. Finally, a continuous 222Rn concentration monitor was placed in the secondary school exhibiting a mean value of the 222Rn concentration very close to 400 Bq m−3. Maximum 222Rn concentration values were found to occur at times when the school was unoccupied.  相似文献   

2.
The radionuclides 210Po and 210Pb widely present in the terrestrial environment are the final long-lived radionuclides in the decay of 238U in the earth’s crust. Their presence in the atmosphere is due to the decay of 222Rn diffusing from the ground. The range of activity concentrations in ground level air for 210Po is 0.03-0.3 Bq m−3 and for 210Pb 0.2-1.5 Bq m−3.In drinking water from private wells the activity concentration of 210Po is in the order of 7-48 mBq l−1 and for 210Pb around 11-40 mBq l−1. From water works, however, the activity concentration for both 210Po and 210Pb is only in the order of 3 mBq l−1.Mosses, lichens and peat have a high efficiency in capturing 210Po and 210Pb from atmospheric fallout and exhibit an inventory of both 210Po and 210Pb in the order of 0.5-5 kBq m−2 in mosses and in lichens around 0.6 kBq m−2. The activity concentrations in lichens lies around 250 Bq kg−1, dry mass.Reindeer and caribou graze lichen which results in an activity concentration of 210Po and 210Pb of about 1-15 Bq kg−1 in meat from these animals. The food chain lichen-reindeer or caribou, and Man constitutes a unique model for studying the uptake and retention of 210Po and 210Pb in humans. The effective annual dose due to 210Po and 210Pb in people with high consumption of reindeer/caribou meat is estimated to be around 260 and 132 μSv a−1 respectively.In soils, 210Po is adsorbed to clay and organic colloids and the activity concentration varies with soil type and also correlates with the amount of atmospheric precipitation. The average activity concentration levels of 210Po in various soils are in the range of 20-240 Bq kg−1.Plants become contaminated with radioactive nuclides both by absorption from the soil (supported Po) and by deposition of radioactive fallout on the plants directly (unsupported Po). In fresh leafy plants the level of 210Po is particularly high as the result of the direct deposition of 222Rn daughters from atmospheric deposition. Tobacco is a terrestrial product with high activity concentrations of 210Po and 210Pb. The overall average activity concentration of 210Po is 13 ± 2 Bq kg−1. It is rather constant over time and by geographical origin.The average median daily dietary intakes of 210Po and 210Pb for the adult world population was estimated to 160 mBq day−1 and 110 mBq day−1, corresponding to annual effective doses of 70 μSv a−1 and 28 μSv a−1, respectively. The dietary intakes of 210Po and 210Pb from vegetarian food was estimated to only 70 mBq day−1 and 40 mBq day−1 corresponding to annual effective doses of 30.6 μSv a−1 and 10 μSv a−1, respectively. Since the activity concentration of 210Po and 210Pb in seafood is significantly higher than in vegetarian food the effective dose to populations consuming a lot of seafood might be 5-15 fold higher.  相似文献   

3.
Considering the role of radon in epidemiology, an attempt was made to make a nation-wide map of indoor 222Rn and 220Rn for India. More than 5000 measurements have been carried out in 1500 dwellings across the country comprising urban and nonurban locations. The solid state nuclear track detectors based twin cup 222Rn/220Rn discrimination dosimeters were deployed for the measurement of indoor 222Rn, 220Rn and their progeny levels. The geometric means of estimated annual inhalation dose rate due to indoor 222Rn, 220Rn and their progeny in the dwellings was 0.94 mSvy−1 (geometric standard deviation 2.5). It was observed that the major contribution to the indoor inhalation dose was due to indoor 222Rn and its progeny. However, the contribution due to indoor 220Rn and its progeny was not trivial as it was found to be about 20% of the total indoor inhalation dose rates. The indoor 222Rn levels in dwellings was significantly different depending on the nature of walls and floorings.  相似文献   

4.
This study investigates the contribution of radon (222Rn)-bearing water to indoor 222Rn in thermal baths. The 222Rn concentrations in air were monitored in the bathroom and the bedroom. Particulate matter (PM, both PM10 and PM2.5) and carbon dioxide (CO2) were also monitored with portable analyzers. The bathrooms were supplied with hot spring water containing 66-260 kBq m−3 of 222Rn. The results show that the spray of hot spring water from the bath spouts is the dominant mechanism by which 222Rn is released into the air of the bathroom, and then it diffuses into the bedroom. Average 222Rn level was 110-410% higher in the bedrooms and 510-1200% higher in the bathrooms compared to the corresponding average levels when there was no use of hot spring water. The indoor 222Rn levels were influenced by the 222Rn concentrations in the hot spring water and the bathing times. The average 222Rn transfer coefficients from water to air were 6.2 × 10−4-4.1 × 10−3. The 24-h average levels of CO2 and PM10 in the hotel rooms were 89% and 22% higher than the present Indoor Air Quality (IAQ) standard of China. The main particle pollutant in the hotel rooms was PM2.5. Radon and PM10 levels in some hotel rooms were at much higher concentrations than guideline levels, and thus the potential health risks to tourists and especially to the hotel workers should be of great concern, and measures should be taken to lower inhalation exposure to these air pollutants.  相似文献   

5.
Radon-222 was measured in groundwater sources of Extremadura (Spain), analyzing 350 samples from private and public springs, wells, and spas by liquid scintillation counting (LSC) and gamma spectrometry. The 222Rn activity concentrations ranged from 0.24 to 1168 Bq L−1. The statistical analysis showed a log-normal distribution with a mean of (111 ± 7) Bq L−1 and a median of (36 ± 3) Bq L−1. A hydrogeological study revealed correlations between the activity concentration and the aquifer material's characteristics. A map of 222Rn in groundwater was elaborated and compared with the natural gamma radiation map for this region. About 35% of the samples showed 222Rn activity concentrations above the Euratom recommended limit of 100 Bq L−1. Three uranium series radionuclides (238U, 234U, and 226Ra) were also assayed by alpha-particle spectrometry, estimating the annual effective dose due to the presence of these natural radionuclides in drinking water.  相似文献   

6.
In China, as the economy is developing and the population is expanding, some underground buildings have been used as supermarkets, restaurants and entertainment places. Tunnels in mountains are one type of underground building, and the radon (222Rn) level in tunnels is an important issue. Radon levels in different type tunnels appear to differ, and relatively higher levels of 222Rn are associated with particular types of bedrock. The 222Rn levels in tunnels in five different geological characteristics were analyzed. Those built in granite had the highest 222Rn levels with a geometric mean (GM) of 280 Bq m−3, while those built in limestone (GM: 100 Bq m−3) and andesitic porphyry (GM: 96 Bq m−3) were lower. The sequence of 222Rn concentrations was: granite > tuff > quartz sandstone > limestone > andesitic porphyry, and the 222Rn in granite was statistically significantly higher than in limestone and andesitic porphyry. Tunnels built in granite, tuff, quartz sandstone, limestone tended to have higher 222Rn concentrations in summer than in winter, while the reverse tendency was true in andesitic porphyry tunnels. Only the difference in limestone was statistically significant.  相似文献   

7.
Total 210Pb and 7Be fallout rates were measured on the coastal region of Niteroi, Brazil. The monthly depositional flux of 210Pb and 7Be varied by a factor of 26, from 1.7 to 43.3 mBq cm−2 year−1 and ∼27, from 7.5 to 203.5 mBq cm−2 year−1, respectively. The relatively large oscillations in the depositional flux of 210Pb at this study site were likely due to variations in air mass sources, while the 7Be fluctuations may be driven by a combination of weather conditions. Local geology could support the periodic high fluxes of 210Pb from continental air masses, as shifting oceanic wind sources were affirmed by the uncorrelated 210Pb and 7Be fallout activities and 7Be/210Pb ratios. The 210Pb atmospheric deposition was found to be in agreement with local sediment inventories, an important consideration in geochemical studies that estimate sedimentation processes.  相似文献   

8.
The assembling of a system for field sampling and activity concentration measurement of radon dissolved in groundwater is described. Special attention is given in presenting the calibration procedure to obtain the radon activity concentration in groundwater from the raw counting rate registered in a portable scintillation detector and in establishing the precision of the activity concentration measurements. A field procedure was established and the system tested during one year of monthly observations of 222Rn activity concentration in groundwater drawn from two wells drilled on metamorphic rocks exposed at Eastern São Paulo State, Brazil. The observed mean 222Rn activity concentrations are 374 Bq/dm3 in one well and about 1275 Bq/dm3 in the other one. In both wells the 222Rn activity concentrations showed a seasonal variation similar to variations previously reported in the literature for the same region.  相似文献   

9.
Polonium-210 (210Po) radioactive concentrations were determined in human semen fluid of vasectomized non-smoker volunteers. The 210Po levels ranged from 0.10 to 0.39 mBq g−1 (mean: 0.23 ± 0.08 mBq g−1). This value decreased to 0.10 ± 0.02 mBq g−1 (range from 0.07 to 0.13 mBq g−1) after two weeks of a controlled diet, excluding fish and seafood. Then, volunteers ate during a single meal 200 g of the cooked mussel Perna perna L., and 210Po levels were determined again, during ten days, in semen fluid samples collected every morning. Volunteers continued with the controlled diet and maintained sexual abstinence through the period of the experiment. A 300% increase of 210Po level was observed the day following mussel consumption, with a later reduction, such that the level returned to near baseline by day 4.  相似文献   

10.
Phosphogypsum (PG) has been traditionally applied as Ca-amendment in saline marsh soils in SW Spain, where available PG has 710 ± 40 Bq kg−1 of 226Ra. This work assesses the potential radiological risk for farmers through 222Rn exhalation from PG-amended soils and by inhalation of PG-dust during its application. A three-year field experiment was conducted in a commercial farm involving two treatments: control and 25 t PG ha−1 with three replicates (each 0.5 ha plots). The 222Rn exhalation rate was positively correlated with potential evapotranspiration, which explained 67% of the variability. Statistically significant differences between the control and PG treatments were not found for 222Rn exhalation rates, and mean values were within the lowest quartile of the typical range for 222Rn exhalation from soils. Airborne dust samples were collected during the application of PG and sugar-beet sludge amendments. The highest PG-attributable 226Ra concentration in the dust samples was 3.3 × 102 μBq m−3, implying negligible dose increment for exposed workers.  相似文献   

11.
Radon and gamma radiation level measurements were carried out inside the La Carolina mine, one of the oldest gold mining camps of southern South America, which is open for touristic visits nowadays. CR-39 track-etch detectors and thermoluminescent dosimeters of natural CaF2 and LiF TLD-100 were exposed at 14 points along the mine tunnels in order to estimate the mean 222Rn concentration and the ambient dose equivalent during the summer season (November 2008 to February 2009). The values for the 222Rn concentration at each monitoring site ranged from 1.8 ± 0.1 kBq m−3 to 6.0 ± 0.5 kBq m−3, with a mean value of 4.8 kBq m−3, indicating that these measurements exceed in about three times the upper action level recommended by ICRP for workplaces. The correlations between radon and gamma radiation levels inside the mine were also investigated. Effective doses due to 222Rn and gamma rays inside the mine were determined, resulting in negligible values to tourists. Considering the effective dose to the mine tourist guides, values exceeding 20 mSv of internal contribution to the effective doses can be reached, depending on the number of working hours inside the mine.  相似文献   

12.
Radon is emitted to the atmosphere with quasi constant emission rates depending on the radium concentration in the earth's crust and soil physical properties. In this way, the 222Rn and 220Rn concentration in air reflects significantly the thickness of the atmospheric boundary layer (ABL). The aerosol-associated, beta-emitting progeny nuclides of 222Rn were measured daily in the framework of the atmospheric radioactivity monitoring program of NIMH at Sofia. The 214Pb concentration was estimated from the measured short-lived beta activity of 24-h filter samples, changed daily at 6:00 GMT. The impact of some meteorological factors such as wind direction, wind velocity, humidity, and temperature on short-lived beta radionuclides is estimated, and the results show no simple statistical relationship. A seasonal pattern was observed with winter minima and late summer-early autumn maxima. High variability in daily morning concentrations and mean monthly values was observed. There were well pronounced differences between years. The height of the convective ABL was estimated from daily radio-soundings at 12:00 GMT for the period 2001-2006 and from seven soundings per day during the experimental campaign in Sofia in October 2003. In general, concentrations of short-lived 222Rn progeny nuclides decreased with increased convective ABL height.  相似文献   

13.
Results of groundwater and seawater analyses for radioactive (3H, 222Rn, 223Ra, 224Ra, 226Ra, and 228Ra) and stable (D and 18O) isotopes are presented together with in situ spatial mapping and time series 222Rn measurements in seawater, direct seepage measurements using manual and automated seepage meters, pore water investigations using different tracers and piezometric techniques, and geoelectric surveys probing the coast. This study represents first time that such a new complex arsenal of radioactive and non-radioactive tracer techniques and geophysical methods have been used for simultaneous submarine groundwater discharge (SGD) investigations. Large fluctuations of SGD fluxes were observed at sites situated only a few meters apart (from 0 cm d−1 to 360 cm d−1; the unit represents cm3/cm2/day), as well as during a few hours (from 0 cm d−1 to 110 cm d−1), strongly depending on the tidal fluctuations. The average SGD flux estimated from continuous 222Rn measurements is 17 ± 10 cm d−1. Integrated coastal SGD flux estimated for the Ubatuba coast using radium isotopes is about 7 × 103 m3 d−1 per km of the coast. The isotopic composition (δD and δ18O) of submarine waters was characterised by significant variability and heavy isotope enrichment, indicating that the contribution of groundwater in submarine waters varied from a small percentage to 20%. However, this contribution with increasing offshore distance became negligible. Automated seepage meters and time series measurements of 222Rn activity concentration showed a negative correlation between the SGD rates and tidal stage. This is likely caused by sea level changes as tidal effects induce variations of hydraulic gradients. The geoelectric probing and piezometric measurements contributed to better understanding of the spatial distribution of different water masses present along the coast. The radium isotope data showed scattered distributions with offshore distance, which imply that seawater in a complex coast with many small bays and islands was influenced by local currents and groundwater/seawater mixing. This has also been confirmed by a relatively short residence time of 1–2 weeks for water within 25 km offshore, as obtained by short-lived radium isotopes. The irregular distribution of SGD seen at Ubatuba is a characteristic of fractured rock aquifers, fed by coastal groundwater and recirculated seawater with small admixtures of groundwater, which is of potential environmental concern and has implications on the management of freshwater resources in the region.  相似文献   

14.
Large temporal variations of radon (222Rn) are often encountered in air in the geologic environment, at time scales from diurnal to annual. Interpretations as to the nature of these variations, unique to 222Rn, often invoke either above surface atmospheric variations, or the influence of subtle active geodynamic processes. So far the eventual geophysical drivers of the variation of 222Rn as well as its specific qualities enabling this temporal variation are not known. New insight on the temporal variation of 222Rn is gained by experimental simulation in confined air. Two short laboratory experiments, and one external experiment lasting over 3 years, were performed inside closed canisters and using natural and commercial 222Rn sources. Internal and external gamma and alpha detectors recorded variations of the radiation, up to around 20% of the equilibrium level. Radon signals of different time scale occurred with: a) periodic annual and semi-annual signals; b) non-periodic multi-day signals; c) periodic daily signals. Similar, related, inversely-related and dissimilar temporal patterns were manifested in the measured time series of the different sensors. Diurnal periodicity was dominated by the solar tide components S1, S2 and S3, exhibiting unlike relative amplitudes and different phases at the different sensors. A compound association occurs among the amplitudes and phases of the diurnal and seasonal periodicities of the daily 222Rn signal, linking the periodic phenomena to the rotation of earth around its axis and around the sun. 222Rn variation patterns in the frequency-time domain cannot be driven by the corresponding atmospheric variation patterns. These results, obtained under static and isolated conditions, are in disagreement with the expected radioactive equilibrium and its spatially uniform expression within and around the experimental volume. The external influence which drives the daily signals evolving from 222Rn inside the canister is non-atmospheric and seemed to be from a remote source and traversed a 5-cm thick lead shield. The similarities with observations on 222Rn signals from upper crustal levels imply that such an external influence, possibly as a component of solar irradiance, drives the 222Rn signals to a depth of at least 100 m. New combined prospects for the research are indicated in terms of the radioactive behavior of 222Rn in air and in terms of an above surface geophysical driver for this behavior.  相似文献   

15.
We report results of air monitoring started due to the recent natural catastrophe on 11 March 2011 in Japan and the severe ensuing damage to the Fukushima Dai-ichi nuclear reactor complex. On 17-18 March 2011, we registered the first arrival of the airborne fission products 131I, 132I, 132Te, 134Cs, and 137Cs in Seattle, WA, USA, by identifying their characteristic gamma rays using a germanium detector. We measured the evolution of the activities over a period of 23 days at the end of which the activities had mostly fallen below our detection limit. The highest detected activity from radionuclides attached to particulate matter amounted to 4.4 ± 1.3 mBq m−3 of 131I on 19-20 March.  相似文献   

16.
The paper presents the results of year-long measurements of radon (222Rn) concentration inside 129 buildings in Poland in relation to the geological conditions of their foundation. The authors took into account the division of the country into tectonic units, as well as the lithology of the rocks forming the bedrock of these buildings. As expected, the highest value of mean annual 222Rn concentration (845 Bq/m3) was recorded in a building situated in the area of the Sudetes, while the highest geometric mean (characteristic of the expected log-normal data distribution) was calculated based on measurements from buildings located within the East-European craton, in the area of Mazury-Podlasie monocline, where it reached 231 Bq/m3. Such results reflect geological conditions - the occurrence of crystalline rocks (especially U- and Ra-enriched granites and orthogneisses) on the surface in the Sudetes, and of young post-glacial sediments containing fragments of Scandinavian crystalline rocks, also enriched with U and Ra, in the area of Mazury-Podlasie monocline. However, the least expected result of the investigations was finding out that, contrary to the hitherto widespread belief, none of the major tectonic units of Poland can be excluded from the list of those containing buildings with mean annual 222Rn concentration exceeding 200 Bq/m3. The mean annual concentration of radon for all the buildings were much higher than the mean concentration value (49.1 Bq/m3) of indoor radon in Poland quoted so far. These results cast a completely new light on the necessity to perform measurements of radon concentration in residential buildings in Poland, no more with reference to small areas with outcrops of crystalline rocks (especially the Sudetes, being the Polish fragment of the European Variscan belt), but for all the major tectonic units within Poland.  相似文献   

17.
Radon-222 and carbon dioxide concentrations have been measured during several years at several points in the atmosphere of an underground limestone quarry located at a depth of 18 m in Vincennes, near Paris, France. Both concentrations showed a seasonal cycle. Radon concentration varied from 1200 to 2000 Bq m−3 in summer to about 800-1400 Bq m−3 in winter, indicating winter ventilation rates varying from 0.6 to 2.5 × 10−6 s−1. Carbon dioxide concentration varied from 0.9 to 1.0% in summer, to about 0.1-0.3% in winter. Radon concentration can be corrected for natural ventilation using temperature measurements. The obtained model also accounts for the measured seasonal variation of carbon dioxide. After correction, radon concentrations still exhibit significant temporal variation, mostly associated with the variation of atmospheric pressure, with coupling coefficients varying from −7 to −26 Bq m−3 hPa−1. This variation can be accounted for using a barometric pumping model, coupled with natural ventilation in winter, and including internal mixing as well. After correction, radon concentrations exhibit residual temporal variation, poorly correlated between different points, with standard deviations varying from 3 to 6%. This study shows that temporal variation of radon concentrations in underground cavities can be understood to a satisfactory level of detail using non-linear and time-dependent modelling. It is important to understand the temporal variation of radon concentrations and the limitations in their modelling to monitor the properties of natural or artificial underground settings, and to be able to assess the existence of new processes, for example associated with the preparatory phases of volcanic eruptions or earthquakes.  相似文献   

18.
Radon-222 exhalation from the ground surface depends upon a number of variables such as the 226Ra activity concentration and its distribution in soil grains; soil grain size; soil porosity, temperature and moisture; atmospheric pressure, rainfall and temperature. In this study, 222Rn exhalation flux density measurements within and around the Ranger uranium mine in northern Australia were performed to investigate the effect of these variables within a tropical region. Measurements were taken at the waste rock dumps, ore stockpiles, mine pits, and at sites where effluent water with elevated 226Ra concentration has been spray irrigated over land, as well as at sites outside the mine. The sites selected represented a variety of geomorphic regions ranging from uranium-bearing rocks to ambient soils. Generally, wet season rains reduced 222Rn exhalation but at a few sites the onset of rains caused a step rise in exhalation flux densities. The results show that parameters such as 226Ra activity concentration, soil grain size and soil porosity have a marked effect on 222Rn flux densities. For similar geomorphic sites, 226Ra activity concentration is a dominant factor, but soil grain size and porosity also influence 222Rn exhalation. Surfaces with vegetation showed higher exhalation flux densities than their barren counterparts, perhaps because the associated root structure increases soil porosity and moisture retention. Repeated measurements over one year at eight sites enabled an analysis of precipitation and soil moisture effects on 222Rn exhalation. Soil moisture depth profiles varied both between seasons and at different times during the wet season, indicating that factors such as duration, intensity and time between precipitation events can influence 222Rn flux densities considerably.  相似文献   

19.
Based on an idealized model, both the annual and the seasonal radon ((222)Rn) flux densities from the soil surface at 1099 sites in China were estimated by linking a database of soil (226)Ra content and a global ecosystems database. Digital maps of the (222)Rn flux density in China were constructed in a spatial resolution of 25 km x 25 km by interpolation among the estimated data. An area-weighted annual average (222)Rn flux density from the soil surface across China was estimated to be 29.7+/-9.4 mBq m(-2)s(-1). Both regional and seasonal variations in the (222)Rn flux densities are significant in China. Annual average flux densities in the southeastern and northwestern China are generally higher than those in other regions of China, because of high soil (226)Ra content in the southeastern area and high soil aridity in the northwestern one. The seasonal average flux density is generally higher in summer/spring than winter, since relatively higher soil temperature and lower soil water saturation in summer/spring than other seasons are common in China.  相似文献   

20.
The indoor radon (222Rn) activity concentration was measured between January and June in the schools of two geothermal areas in Tuscany, central Italy. One of these areas (the Larderello area) is characterized by a large number of geothermal power plants, covering about 9% of the world’s geothermal power production. In contrast, the other area, Monte Pisano, has not any such facilities. About 250 measurements were made using track etch detectors. Only a slight difference in the concentrations between the two major sampling areas (98 Bq m−3 for Larderello area and 43 Bq m−3 for Monte Pisano area) was found, and this was related to different geological characteristics of the ground and not the presence of the geothermal plants. The measured radon concentrations were always well below the intervention levels in both areas, and health risks for students and personnel in the examined schools were excluded.  相似文献   

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