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排序方式: 共有322条查询结果,搜索用时 46 毫秒
81.
Geiger H Becker KH Wiesen P 《Journal of the Air & Waste Management Association (1995)》2003,53(4):425-433
Based on exhaust gas analyses from the combustion of five different types of gasoline in a passenger car operated on a chassis dynamometer, box model simulations of the irradiation of exhaust/NOx/air mixtures using an established chemical mechanism for a standardized photosmog scenario were performed. The fuel matrix used covered wide fractional ranges for paraffinic, olefinic, and aromatic hydrocarbons. Two fuels also contained methyl tertiary butyl ether (MTBE). The different O3 profiles calculated for each run were compared and interpreted. The O3 levels obtained were strongly influenced by the exhaust gas concentrations of aromatic and olefinic hydrocarbons. The higher exhaust content of these compounds caused higher O3 production in the smog system investigated. The conclusion of the present study is that the composition of gasoline cannot be taken directly for the estimation of the emissions' O3 creation potential from its combustion. Variation of the dilution in the different calculations showed evidence for an additional influence of transport effects. Accordingly, further detailed exhaust gas analyses followed by more complex modeling studies are necessary for a proper characterization of the relationship between fuel blend and gasoline combustion products. 相似文献
82.
PCBs, DDTs and methyl sulphone metabolites in various tissues of harbour porpoises from Swedish waters 总被引:2,自引:0,他引:2
Karlson K Ishaq R Becker G Berggren P Broman D Colmsjö A 《Environmental pollution (Barking, Essex : 1987)》2000,110(1):29-46
Aryl methyl sulphones of polychlorinated biphenyls (PCBs) and 3-p,p'-DDE (MeSO(2)-PCBs and 3-MeSO(2)-p,p'-DDE), PCBs and Sigma DDTs were analysed in five different tissues (blubber, nuchal fat, liver, muscle, brain) of adult male harbour porpoises from the west coast of Sweden. Two different methods for MeSO(2)-PCBs and 3-MeSO(2)-p,p'-DDE determination were used, gas chromatography-mass spectrometry and gas chromatography-atomic emission detection. Highest concentrations of Sigma MeSO(2)-PCBs were found in liver (0.15-0.49 microg/g lipid wt.), which corresponded to 2.0-2.8% of the Sigma PCBs concentrations. Blubber and nuchal fat showed Sigma MeSO(2)-PCB concentrations that were three to five times lower than those in liver. Concentrations of 3-MeSO(2)-p,p'-DDE in liver, muscle and brain corresponded to 0.26-4.6% of the p,p'-DDE concentrations, while in blubber and nuchal fat, 3-MeSO(2)-p,p'-DDE constituted 0.033-0.21% of p,p'-DDE. The different tissues analysed showed similar levels (lipid wt.) of Sigma PCBs and Sigma DDTs, except for brain that had almost 10 times lower levels compared to the other tissues. Using the Sigma PCBs/Sigma MeSO(2)-PCBs ratio to estimate MeSO(2)-PCB formation and secondary metabolism capacity, the harbour porpoise showed a relatively low capacity of MeSO(2)-PCB formation compared to other small toothed whales and seals. Blubber sampled from five different anatomical locations showed that concentrations of contaminants may be unevenly distributed in blubber in certain animals. This should be taken into account when choosing sampling sites on the porpoise. 相似文献
83.
Christian Antileo Marlene Roeckel J?rg Lindemann Udo Wiesmann 《Water environment research》2007,79(9):1006-1014
Incomplete nitrification was studied in a completely and partially submerged rotating biological contactor (RBC). In a partially submerged RBC without additional aeration, 50 to 90% nitrite accumulation (alpha) was achieved at rotation speeds (omega) of 2 to 18 min(-1). In a completely submerged RBC operating during 80 days, a higher alpha of 96% was achieved at omega = 2 min(-1). Incomplete nitrification in a completely submerged RBC at oxygen concentrations of 1.5 to 6.8 mg O2/L indicated that the mass transfer of oxygen is rate-limiting. Modeling of the completely submerged RBC predicts that the oxygen profile will not penetrate the biofilm more than 30 microm, thereby strongly limiting the nitrite-oxidizer growth and causing high nitrite accumulation. Molecular analysis (i.e., fluorescence in situ hybridization) indicated that the nitrite-oxidizers are superficially located (<200 microm) and that the ammonia-oxidizers comprise up to approximately 800 microm of the biofilm. 相似文献
84.
Udo Muster Tom Schilling Harald Schobesberger Hertha Luttenberger Rolf Marr und Josef Draxler 《Umweltwissenschaften und Schadstoff-Forschung》1997,9(1):25-32
Zusammenfassung Bei einer genauen Kenntnis der vorliegenden Quecksilberverbindungen und ihrem Verhalten im Rauchgaspfad thermischer Anlagen
k?nnen durch entsprechende technische Ma?nahmen die Abscheideeffizienzen in trockenen, quasitrockenen und nassen Rauchgasreinigungsanlagen
erheblich gesteigert werden, so da? der derzeit gesetzlich vorgeschriebene Emissionsgrenzwert von 50 μg/m3 [i.N.tr.] eingehalten und unterschritten wird. Die in den letzten Jahren unternommenen Aktivit?ten und Fortschritte bei der
Reduzierung des Quecksilberaussto?es von thermischen Anlagen werden zusammenfassend dargestellt. Am Beispiel von tr?gerimmobilisierten
metall- und/oder metallsalzpartikelbelegten Tr?germaterialien (G/S-Reaktoren) wird die selektive Entfernung des Quecksilbers
bzw. dessen Verbindungen experimentell und theoretisch im Rauchgaspfad verdeutlicht. Aus der selektiven Abtrennung von Quecksilber
und seinen Verbindungen in der Gasphase resultieren auch entsprechende ?kologische und ?konomische Vorteile, die den allgemein
erkennbaren Trend der artspezifischen Abtrennung von Schadstoffen mit einer m?glichen Rückführung des Wertstoffes Quecksilber
in den Wirtschaftskreislauf unterstützen.
相似文献
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87.
Klaus Jung Udo Kristen Johannes Flachowsky Helmut Segner Gerrit Schüürmann 《Environmental Sciences Europe》1997,9(6):317-321
For risk assessment of environmental samples, rapid and sensitive screening assays for detection of toxic potencies are required. Using leachates from waste deposites in the industrial region Leipzig-Halle (Germany) as an example, we present a simple test procedure suitable for the detection of cytotoxic effects of samples. This method, the pollen tube growth test (PTG), works as follows: Pollen of tobacco (Nicotiana sylvestris Spegazz, & Comes) are suspended in mixtures of growth medium and buffered (pH 6,3 to 7,0) dumping ground leachates. After an 18h-incubation period, growth of pollen tubes is quantified by staining with Alcian blue and subsequent measurment of optical density in a photometer. Sample induced inhibition of pollen tube growth is calculated in relation to controls maintained in pure growth medium. The PTG test shows high sensitivity towards leachates of different chemical composition, and it shows good agreement with assay results from luminescent bacteria tests. We conclude that the PTG test is well suited to assess the hazardous potential of aqueous environmental samples. 相似文献
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