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61.
Copper-exchanged chabazite (Cu/CHA) catalysts have been found to be affected by alkali metal and alkaline earth ions. However, the effects of Na+ ions on Cu/SAPO-34 for ammonia selective catalytic reduction (NH3-SCR) are still unclear. In order to investigate the mechanism, five samples with various Na contents were synthesized and characterized. It was observed that the introduced Na+ ion-exchanges with H+ and Cu2 + of Cu/SAPO-34. The exchange of H+ is easier than that of isolated Cu2 +. The exchanged Cu2 + ions aggregate and form “CuAl2O4-like” species. The NH3-SCR activity of Cu/SAPO-34 decreases with increasing Na content, and the loss of isolated Cu2 + and acid sites is responsible for the activity loss. 相似文献
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结合旅游风景区举办大型体育赛事对环境的危害性,从减少污染排放源、从源头治理污染、加大管理层的监管力度等三方面进行环境污染监控管理。采用统计分析方法对环保治理效果进行量化评估,分析旅游风景区举办大型体育赛事期间的空气污染指数、废弃物排放数量以及水质污染情况,结合分组样本检验方法进行环保措施的有效性评价,并根据实际情况制定最优的环保措施,实现对旅游风景区的全方面环境治理,确保举办体育赛事对旅游景区的生态环境污染影响降到最低。 相似文献
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Gu B Watson DB Wu L Phillips DH White DC Zhou J 《Environmental monitoring and assessment》2002,77(3):293-309
Zero-valent iron (Fe0)-based permeable reactive barriertreatment has been generating great interest for passivegroundwater remediation, yet few studies have paid particularattention to the microbial activity and characteristics withinand in the vicinity of the Fe0-barrier matrix. The presentstudy was undertaken to evaluate the microbial population andcommunity composition in the reducing zone of influence byFe0 corrosion in the barrier at the Oak Ridge Y-12 Plantsite. Both phospholipid fatty acids and DNA analyses were usedto determine the total microbial population and microbialfunctional groups, including sulfate-reducing bacteria,denitrifying bacteria, and methanogens, in groundwater andsoil/iron core samples. A diverse microbial community wasidentified in the strongly reducing Fe0 environment despitea relatively high pH condition within the Fe0 barrier (up topH 10). In comparison with those found in the backgroundsoil/groundwater samples, the enhanced microbial populationranged from 1 to 3 orders of magnitude and appeared to increase from upgradient of the barrier to downgradient soil. Inaddition, microbial community composition appeared to change overtime, and the bacterial types of microorganismsincreased consistently as the barrier aged. DNA analysisindicated the presence of sulfate-reducing and denitrifyingbacteria in the barrier and its surrounding soil. However, theactivity of methanogens was found to be relatively low,presumably as a result of the competition by sulfate/metal-reducing bacteria and denitrifying bacteria because of the unlimited availability of sulfate and nitrate in the site groundwater. Results of this study provide evidenceof a diverse microbial population within and in the vicinity ofthe iron barrier, although the important roles of microbial activity, either beneficially or detrimentally, on the longevityand enduring efficiency of the Fe0 barriers are yet to be evaluated. 相似文献
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Soil Lead and Other Metal Levels in Industrial, Residential and Nature Reserve Areas in Singapore 总被引:4,自引:0,他引:4
C. Y. Zhou M. K. Wong L. L. Koh Y. C. Wee 《Environmental monitoring and assessment》1997,44(1-3):605-615
The use of pressure feedback microwave digestion technique has permitted rapid and efficient digestion of soil and sediment samples. The evaluation of different acid mixtures to digest soil samples were studied by mixed-level orthogonal array design. The selected acid mixture of HCl-HNO3-HF was employed in the survey of Pb, Zn, Cu, Cr and Mn in soil samples. Surface soil samples were collected from industrial, residential and nature reserve areas in Singapore. The five metal concentrations were determined by flame atomic absorption spectrometry and graphite furnace atomic absorption spectrometry. The lead and other metal contents in NBS SRM 1645, NIES CRM No. 2 and NRCC BCSS-1 sediment standard references were determined concurrently with the survey samples. Five measured metal loading on the surface soils was in the order: industrial area > residential area > nature reserve area. The trace metal concentrations in surface soil from areas of heavy traffic are higher than those from residential areas. The main sources of trace metal pollution are vehicular exhaust and industrial activities. 相似文献
70.
发光细菌法评价工业废水的毒性 总被引:5,自引:0,他引:5
用发光细菌测定法估算了两城市污水对河道水体污染的分担率,评价了工厂排放废水的毒性,并据此确定了污染源监督管理中应优先治理的工厂(车间)废水。 相似文献