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Mao Haobo Zhang Yingyi Wang Hong Cui Kunkun Yu Laihao Tan Tianbiao 《Environmental Chemistry Letters》2023,21(3):1659-1672
Environmental Chemistry Letters - Huge amounts of unwanted sewage sludge are generated in the process of wastewater treatment, calling for methods to recycle sewage sludges into value-added... 相似文献
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以共沉淀法制备的纳米Fe3O4为核,以正硅酸乙酯为硅源,通过溶胶-凝胶法制备了SiO2@Fe3O4壳-核结构纳米颗粒,再以钛酸四丁酯为钛源,通过溶胶-凝胶法、经焙烧制得TiO2/SiO2@γ-Fe2O3磁性纳米光催化剂。采用X射线衍射仪、透射电子显微镜、比表面分析仪、振动磁强计对光催化剂的结构进行了表征,以苯酚溶液为模拟废水对光催化剂的光催化性能进行了评价。实验结果表明:经500℃焙烧的光催化剂活性相为锐钛矿型TiO2;在苯酚溶液初始浓度为0.2mmol/L、苯酚溶液pH为7的条件下,COD去除率为70.9%。 相似文献
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Yingyi Zhang Senchao Lai Zhen Zhao Fobang Liu Hongwei Chen Shichun Zou Zhiyong Xie Ralf Ebinghaus 《Chemosphere》2013
An intensive campaign was conducted in September 2012 to collect surface water samples along the tributaries of the Pearl River in southern China. Thirteen perfluoroalkyl acids (PFAAs), including perfluorocarboxylates (PFCAs, C4–C11) and perfluorosulfonates (PFSAs, C4, C6–C8, and C10), were determined using high-performance liquid chromatography/negative electrospray ionization–tandem mass spectrometry (HPLC/(-)ESI–MS/MS). The concentrations of total PFAAs (ΣPFAAs) ranged from 3.0 to 52 ng L−1, with an average of 19 ± 12 ng L−1. The highest concentrations of ΣPFAAs were detected in the surface water of the Dong Jiang tributary (17–52 ng L−1), followed by the main stream (13–26 ng L−1) and the Sha Wan stream (3.0–4.5 ng L−1). Perfluorooctanoate (PFOA), perfluorobutane sulfonate (PFBS), and perfluorooctane sulfonate (PFOS) were the three most abundant PFAAs and on average accounted for 20%, 24%, and 19% of ΣPFAAs, respectively. PFBS was the most abundant PFAA in the Dong Jiang tributary, and PFOA was the highest PFAA in the samples from the main stream of the Pearl River. A correlation was found between PFBS and PFOA, which suggests that both of these PFAAs originate from common source(s) in the region. Nevertheless, the slope of PFBS/PFOA was different in the different tributaries sampled, which indicates a spatial difference in the source profiles of the PFAAs. 相似文献
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Yao Meng Junwei Song Lewei Zeng Yingyi Zhang Yan Zhao Xufei Liu Hai Guo Liuju Zhong Yubo Ou Yan Zhou Tao Zhang Dingli Yue Senchao Lai 《环境科学学报(英文版)》2022,34(1):104-117
We present the continuously measurements of volatile organic compounds(VOCs) at a receptor site(Wan Qing Sha, WQS) in the Pearl River Delta(PRD) region from September to November of 2017. The average mixing ratios of total VOCs(TVOCs) was 36.3 ± 27.9 ppbv with the dominant contribution from alkanes(55.5%), followed by aromatics(33.3%). The diurnal variation of TVOCs showed a strong photochemical consumption during daytime,resulting in the formation of ozone(O3). Five VOC sources were ... 相似文献
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林颖毅 《环境与可持续发展》2014,39(6)
针对船舶造成的海洋环境污染的现状,分析了船舶污染的途径、危害,进行了风险评价,提出防污染对策。研究表明,当前保护海洋环境和生态被社会各界重视,国际海事组织也不断修改船舶防污染公约,对防止船舶造成海洋环境污染的要求也越来越严格了。为此,我国应健全船舶防污染保护海洋机制。一是完善海面溢油监测系统;二是促进清污公司市场机制;三是优化船舶溢油应急设备器材库站点;四是加强船舶动态跟踪。 相似文献
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Xin Yan Wang Dongchuan Zhang Lihui Ma Yingyi Chen Xing Wang Haiqing Wang Hongyi Wang Kangjian Long Hui Chai Hua Gao Jianshe 《Environment, Development and Sustainability》2022,24(3):3687-3703
Environment, Development and Sustainability - The western region of China has always been the main battlefield for poverty alleviation. It is essential to explore the interaction mechanism between... 相似文献
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《中华人民共和国防治海岸工程建设项目污染损害海洋环境管理条例》颁布实施以来,对各评估单位进行环境评审的工作起了指导性作用,但在实施过程中,评估单位对《海洋环境影响报告》编制格式的理解偏差而造成某些章节所论述的内容与标题意图不符,或论述分析不够全面等问题。本文通过对《海洋环境影响报告》编制格式的剖析,提出了一些建议与看法以供各相关单位参考。 相似文献
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超声辅助EDDS/EGTA淋洗对土壤重金属形态、环境风险的影响及响应面优化 总被引:1,自引:0,他引:1
采用响应面法实验设计研究了超声辅助EDDS/EGTA淋洗对Cu、Zn、Pb和Cd等不同重金属的洗脱效果和对残留重金属化学形态分布的影响,以超声功率、初始pH、EDDS投加量、EGTA投加量作为考察对象,以各重金属去除率及其环境风险削减率为响应值进行了模拟和优化.结果表明,EDDS对Pb的洗脱效率最高,Cu、Zn次之,Cd最低;EGTA对Cd的洗脱效率最高,Pb、Zn次之,Cu最低;超声功率对Cu、Pb去除强化效果明显,对Cd影响小,对Zn无显著影响;初始pH值为酸性时,Cu和Zn去除率高,碱性时Pb去除率较高,Cd去除率有所下降.EDDS与EGTA投加量及EGTA投加量与初始pH值对环境风险总削减率存在交互作用.超声辅助EDDS/EGTA对可还原态重金属洗脱效果较好,但容易导致弱酸提取态Cu和Pb残留率有所升高.响应面优化结果表明,当EDDS和EGTA投加量分别为重金属总摩尔数的1.92和2.56倍、超声功率为600 W、淋洗液初始pH值为5.27时,环境风险总削减率达到77.58%,与模拟值相近,模型具有较好的模拟和预测能力. 相似文献