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1.
Energy consumption is a major cause of air pollution in Beijing, and the adjustment of the energy structure is of strategic importance to the reduction of carbon intensity and the improvement of air quality. In this paper, we explored the future trend of energy structure adjustment in Beijing till 2020, designed five energy scenarios focusing on the fuel substitution in power plants and heating sectors, established emission inventories, and utilized the Mesoscale Modeling System Generation 5 (MM5) and the Models-3/Community Multiscale Air Quality Model (CMAQ) to evaluate the impact of these measures on air quality. By implementing this systematic energy structure adjustment, the emissions of PM10, PM2.5, SO2, NO x , and non-methane volatile organic compounds (NMVOCs) will decrease distinctly by 34.0%, 53.2%, 78.3%, 47.0%, and 30.6% respectively in the most coalintensive scenario of 2020 compared with 2005. Correspondingly, MM5-Models-3/CMAQ simulations indicate significant reduction in the concentrations of major pollutants, implying that energy structure adjustment can play an important role in improving Beijing??s air quality. By fuel substitution for power plants and heating boilers, PM10, PM2.5, SO2, NO x , and NMVOCs will be reduced further, but slightly by 1.7%, 4.5%, 11.4%, 13.5%, and 8.8% respectively in the least coal-intensive scenario. The air quality impacts of different scenarios in 2020 resemble each other, indicating that the potential of air quality improvement due to structure adjustment in power plants and heating sectors is limited. However, the CO2 emission is 10.0% lower in the least coal-intensive scenario than in the most coal-intensive one, contributing to Beijing??s ambition to build a low carbon city. Except for energy structure adjustment, it is necessary to take further measures to ensure the attainment of air quality standards.  相似文献   

2.
Zhang  Chao  Li  Sha  Guo  Gan-lan  Hao  Jing-wen  Cheng  Peng  Xiong  Li-lin  Chen  Shu-ting  Cao  Ji-yu  Guo  Yu-wen  Hao  Jia-hu 《Environmental geochemistry and health》2021,43(9):3393-3406

Numerous studies had focused on the association between air pollution and health outcomes in recent years. However, little evidence is available on associations between air pollutants and premature rupture of membranes (PROM). Therefore, we performed time-series analysis to evaluate the association between PROM and air pollution. The daily average concentrations of PM2.5, SO2 and NO2 were 54.58 μg/m3, 13.06 μg/m3 and 46.09 μg/m3, respectively, and daily maximum 8-h average O3 concentration was 95.67 μg/m3. The strongest effects of SO2, NO2 and O3 were found in lag4, lag06 and lag09, and an increase of 10 μg/m3 in SO2, NO2 and O3 was corresponding to increase in incidence of PROM of 8.74% (95% CI 2.12–15.79%), 3.09% (95% CI 0.64–5.59%) and 1.68% (95% CI 0.28–3.09%), respectively. There were no significant effects of PM2.5 on PROM. Season-specific analyses found that the effects of PM2.5, SO2 and O3 on PROM were more obvious in cold season, but the statistically significant effect of NO2 was observed in warm season. We also found the modifying effects by maternal age on PROM, and we found that the effects of SO2 and NO2 on PROM were higher among younger mothers (<?35 years) than advanced age mothers (≥?35 years); however,?≥?35 years group were more vulnerable to O3 than?<?35 years group. This study indicates that air pollution exposure is an important risk factor for PROM and we wish this study could provide evidence to local government to take rigid approaches to control emissions of air pollutants.

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3.
This work evaluates the influence of energy consumption on the future air quality in Beijing, using 2000 as the base year and 2008 as the target year. It establishes the emission inventory of primary PM10, SO2 and NOx related to energy utilization in eight areas of Beijing. The air quality model was adopted to simulate the temporal and spatial distribution of each pollutant concentration in the eight urban areas. Their emission, concentration distribution, and sectoral share responsibility rate were analyzed, and air quality in 2008 was predicted. The industrial sector contributed above 40% of primary PM10 and SO2 resulting from energy consumption, while vehicles accounted for about 65% of NOx. According to the current policy and development trend, air quality in the eight urban areas could become better in 2008 when the average concentrations of primary PM10, SO2 and NO2 related to energy utilization at each monitored site are predicted to be about 25, 50 and 51 μg/m3, respectively.  相似文献   

4.
Air pollution poses a serious threat to human health in Asia. This study analyzes the association of air pollutants and greenness with incidence rates of allergic rhinitis in Seoul at the administrative district level to gain insight into district-level urban policies to improve public health. A spatial regression model is constructed to investigate the correlation between allergic rhinitis incidence rates and five air pollutants measured at 128 air pollution monitoring stations around Seoul: sulfur dioxide (SO2), particulate matter less than 10 μm (PM10), ozone (O3), nitrogen dioxide (NO2), and carbon monoxide (CO). The allergic rhinitis incidence data are derived from the National Health Insurance Service’s database that includes the number of allergic rhinitis-related clinic visits by the patients over 20 years of age and living in Seoul. A kriging geostatistical interpolation was used to estimate average air pollution level of 423 administrative districts. To assess pollen concentrations that can affect allergic rhinitis, the average normalized difference vegetation index (NDVI) is measured based on the urban greenness. The model, controlling for built environment and socio-economic attributes, identifies the possibility of a weak association between allergic rhinitis incidence rates and carbon monoxide levels. The NDVI value is negatively correlated with allergic rhinitis incidence rates, implying a complicated aspect in relation to the effect of urban greenness.  相似文献   

5.
We estimate the effect of short-term air pollution exposure (PM2.5 and ozone) on several categories of crime, with a particular emphasis on aggressive behavior. To identify this relationship, we combine detailed daily data on crime, air pollution, and weather for an eight-year period across the United States. Our primary identification strategy employs extremely high dimensional fixed effects and we perform a series of robustness checks to address confounding variation between temperature and air pollution. We find a robust positive effect of increased air pollution on violent crimes, and specifically assaults, but no relationship between increases in air pollution and property crimes. The effects are present in and out of the home, at levels well below Ambient Air Pollution Standards, and PM2.5 effects are strongest at lower temperatures. The results suggest that a 10% reduction in daily PM2.5 and ozone could save $1.4 billion in crime costs per year, a previously overlooked cost associated with pollution.  相似文献   

6.

Goal and Scope

The constant increase of traffic and the rising energy and material consumption both in industry and trade as well as in private households mean a constant challenge to environmental protection and to the air pollution control. With the commencement of the Federal ambient pollution control act in April 1974, the legal basis for the monitoring of air pollution was created. In future, the limit values laid down in the Council Directive 1999/30/EG, 2000/69/EG and 96/62/EG, will be valid. In town and regional planning there is a great demand for a simple index to evaluate the air quality. From the available data of PM10, NO2, O3, CO, SO2, trends of the air quality will be derived.

Methods

The indices LQI and TLQ suggested by Mayer et al. (2002) were calculated for selected stations of the air pollution monitoring network (ZIMEN) in Rhineland-Palatine. All analysis are based on hourly recorded value, Mean values and frequency distributions are used for the interpretation. Furthermore, the characteristics and trends of the indices under different weather conditions were examined and discussed.

Results

The examination figures out that the air pollutions indices at all stations show similar patterns in the period between January 2001 and December 2002. Neither the LQI, nor the TLQ shows an annual variation. Existing variations are mainly controlled by the general weather situation and the air temperature. High values of the indices appear at extremely high or low mean daily air temperature. The absolute value of the air pollution index is determined by local pollution factors.

Outlook and Recommendations

Both indices are well suitable to evaluate the air quality and to assess the effects of state-aided measures for air pollutant control. Therefore, the indices TLQ and LQI should be published as an additional information in the world wide web.  相似文献   

7.
Ambient PM2.5 samples were collected at four sites in Xiamen, including Gulangyu (GLY), Hongwen (HW), Huli (HL) and Jimei (JM) during January, April, July and October 2013. Local source samples were obtained from coal burning power plants, industries, motor vehicles, biomass burning, fugitive dust, and sea salt for the source apportionment studies. The highest value of PM2.5 mass concentration and species related to human activities (SO4 2–, NO3 , Pb, Ni, V, Cu, Cd, organic carbon (OC) and elemental carbon (EC)) were found in the ambient samples from HL, and the highest and lowest loadings of PM2.5 and its components occurred in winter and summer, respectively. The reconstructed mass balance indicated that ambient PM2.5 consisted of 24% OM (organic matter), 23% sulfate, 14% nitrate, 9% ammonium, 9% geological material, 6% sea salt, 5% EC and 10% others. For the source profiles, the dominant components were OC for coal burning, motor vehicle, biomass burning and sea salt; SO4 2– for industry; and crustal elements for fugitive dust. Source contributions were calculated using a chemical mass balance (CMB) model based on ambient PM2.5 concentrations and the source profiles. GLY was characterized by high contributions from secondary sulfate and cooking, while HL and JM were most strongly affected by motor vehicle emissions, and biomass burning and fugitive dust, respectively. The CMB results indicated that PM2.5 from Xiamen is composed of 27.4% secondary inorganic components, 20.8% motor vehicle emissions, 11.7% fugitive dust, 9.9% sea salt, 9.3% coal burning, 5.0% biomass burning, 3.1% industry and 6.8% others.
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8.
In this study, we collected particles with aerodynamic diameter ?2.5 μm (PM2.5) from three different public indoor places (a supermarket, a commercial office, and a university dining hall) in Jinan, a medium-sized city located in northern China. Water-soluble inorganic ions of PM2.5 and particle size distributions were also measured. Both indoor and outdoor PM2.5 levels (102.3–143.8 μg·m?3 and 160.2–301.3 μg·m?3, respectively) were substantially higher than the value recommended by the World Health Organization (25 μg·m?3), and outdoor sources were found to be the major contributors to indoor pollutants. Diurnal particle number size distributions were different, while the maximum volume concentrations all appeared to be approximately 300 nm in the three indoor locations. Concentrations of indoor and outdoor PM2.5 were shown to exhibit the same variation trends for the supermarket and dining hall. For the office, PM2.5 concentrations during nighttime were observed to decrease sharply. Among others, SO 4 2? , NH 4 + and NO 3 ? were found to be the dominant water-soluble ions of both indoor and outdoor particles. Concentrations of NO 3 ? in the supermarket and office during the daytime were observed to decrease sharply, which might be attributed to the fact that the indoor temperature was much higher than the outdoor temperature. In addition, domestic activities such as cleaning, water usage, cooking, and smoking also played roles in degraded indoor air quality. However, the results obtained here might be negatively impacted by the small number of samples and short sampling durations.  相似文献   

9.
The pollution characteristics of PM2.5 and correlation analysis with meteorological parameters in Xinxiang during the Shanghai Cooperation Organization Prime Ministers’ Meeting were investigated. During the whole meeting, nine PM2.5 samples were collected at a suburban site of Xinxiang, and the average concentration of PM2.5 was 122.28 μg m?3. NO3 ?, NH4 +, SO4 2? accounted for 56.8% of the total water-soluble ions. In addition, with an exception of Cl?, all of water-soluble ions decreased during the meeting. Total concentrations of crustal elements ranged from 6.53 to 185.86 μg m?3, with an average concentration of 52.51 μg m?3, which accounted for 82.5% of total elements. The concentrations of organic carbon and elemental carbon were 7.71 and 1.52 μg m?3, respectively, lower than those before and after the meeting. It is indicated that during the meeting, limiting motor vehicles is to reduce exhaust emissions, delay heating is to reduce the fossil fuel combustion, and other measures are to reduce the concentration of PM2.5. The directly dispersing by mixing layerheight increase and the indirectly reducing the formation of secondary aerosol by low relative humidity, andthese are the only two key removing mechanisms of PM2.5 in Xinxiang during the meeting.  相似文献   

10.
为明确NH_4~+、 NO_3~-、SO_4~(2-)及金属等组分在水溶性提取液对发光细菌的光抑制过程中所起的作用,参照PM_(2.5)样品提取液浓度,模拟配制与3级以上PM_(2.5)样品提取液中主要组分:硫酸盐、硝酸盐、氨盐相同浓度的溶液,同时选取与PM_(2.5)可溶性提取液发光抑制率相关性较强的铅、锌,配制不同浓度级别模拟溶液,测试各单一组分对发光细菌的发光抑制率及其混合溶液对发光细菌的联合影响效应。基于毒性单位法(TU)、相加指数法(AI)和混合毒性指数法(MTI)评价了混合体系联合影响的作用类型。结果表明,与3~6级PM_(2.5)可溶性提取液中硫酸氨、硫酸氢氨、硝酸氨、硫酸锌和硝酸铅浓度相同的模拟溶液对发光细菌的发光没有抑制作用。不同的评价方法对PM_(2.5)主要组分混合体系联合效应评价结果具有较好的一致性,硫酸氨、硝酸氨、硫酸氢氨混合溶液中,对发光细菌的光抑制均为硫酸氢氨的独立作用,硫酸锌与硝酸铅的混合体系,锌和铅对发光细菌的联合影响效应表现为协同,硫酸氨、硝酸氨、硫酸氢氨与硫酸锌、硝酸铅的多元混合体系呈现协同作用。  相似文献   

11.
This article assesses the air pollution data from two monitoring stations in Kuwait. The measurements cover major pollutants, i.e., CO, CO2, methanated and non-methanated hydrocarbons, NO x , SO2, O3, and particulate matter (PM10). The data also includes meteorological parameters, i.e., solar intensity, temperature, wind speed, and wind direction, and has been collected over a period 4 years, from 2001 to 2004. Data analysis includes the assessment of annual hourly averages and 1-h maxima. Typical pollutant concentration trends, similar to those previously reported for Kuwait and for other locations around the world, are observed except for particulate matter measurements, which have higher values because of proximity to the desert. Emissions of nitrogen oxides show a consistent increase over the years. This is caused by the increase in the number of motor vehicles and the expansion in power generation and industrial activities. The data collected is a subset of the air quality criteria, as defined by the US EPA (United States Environmental Protection Agency).  相似文献   

12.

Diesel engine railway traffic causes atmosphere pollution due to the exhaust emission which may be harmful to the passengers as well as workers. In this study, the air quality and PM10 concentrations were evaluated around a railway station in Northeast India where trains are operated with diesel engines. The gaseous pollutant (e.g. SO2, NO2, and NH3) was collected and measured by using ultraviolet–visible spectroscopy. The advanced level characterizations of the PM10 samples were carried out by using ion chromatography, Fourier-transform infrared, X-ray diffraction, inductively coupled plasma optical emission spectrometry , X-ray photoelectron spectroscopy, field-emission scanning electron microscopy with energy-dispersive spectroscopy, and high-resolution transmission electron microscopy with energy-dispersive spectroscopy techniques to know their possible environmental contaminants. High-performance liquid chromatography technique was used to determine the concentration of polycyclic aromatic hydrocarbons to estimate the possible atmospheric pollution level caused by the rail traffic in the enclosure. The average PM10 concentration was found to be 262.11 µg m−3 (maximum 24 hour) which indicates poor air quality (AQI category) around the rail traffic. The statistical and air mass trajectory analysis was also done to know their mutual correlation and source apportionment. This study will modify traditional studies where only models are used to simulate the origins.

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13.
A study has been conducted over a period of one year on measurements of air pollution in the Shuaiba Industrial Area (SIA) of Kuwait. The study included analysis of pollutant behaviour relative to the wind speed and direction. SIA comprises several large scale industries including three petroleum refineries, two power plants, two fertilizer plants, a cement plant, a chlorine and soda plant, a commercial harbour and two large oil loading terminals. Measurements of 15 parameters have been carried out every 5 minutes using a mobile laboratory fitted with an automatic calibrator and a data storage system. The pollutants studied include methane, non‐methane hydrocarbons (NMHC), carbon monoxide, carbon dioxide, nitrogen oxides (NO, NO2, and NO x ), sulphur dioxide, ozone and suspended dust. Meteorological parameters monitored simultaneously include wind speed and direction, air temperature, relative humidity, solar radiation, and barometric pressure. The air quality data collected using the mobile laboratory have been used to calculate the diurnal and monthly variations in the major primary and secondary pollutants. Distribution levels of these pollutants relative to wind direction and speed have also been used in the analysis. The results show large diurnal variations in some pollutant concentrations. Generally, two types of concentration variations have been found, depending on whether the species is a primary or a secondary pollutant. Diurnal variations with two maxima were observed in the concentrations of primary pollutants including NO, SO2, NMHC, CO and suspended dust, whereas a single maximum was observed for secondary pollutants such as O3and NO2. The monthly variations of SO2and NO x showed maximum values during the warm months. However, ozone showed a quite marked seasonal variation with maxima during spring and late summer and a minimum during the early summer. The results also indicated a common source for NO x , SO2, NMHC, CO and suspended dust to the North‐West (NW) of the monitoring station. Moreover for NO x and SO2, another less significant source is to the South‐South‐West (SSW) and South‐West (SW) of the monitoring station.  相似文献   

14.
Investigations on the fluctuation in PM10 air pollution in Volos, a medium-sized industrialized port city in the Mediterranean, are presented for the 5-year period between 2009 and 2014. The levels detected have been examined in relation to legislatively set limits, sampling year, and day of the week. A PM10 spring sampling campaign has been performed in 2014 and metals and other elements in the PM10 mass have been quantified. Source origin has been attempted for the latter sampling campaign and human health risk has been assessed. Results show compliance with the mean annual value of 40 μg m?3 of 2008/50/EC for the city; however, exceedances of the daily quality standard of 50 μg m?3 were frequently recorded. Shifts in PM10 concentrations and in contributing sources have been recorded; nevertheless, longer duration data series are needed for safe deductions. Element measurements have enabled source identification for early summer of 2014, with Earth's crust minerals and anthropogenic sources being the main factors. Cumulative non-carcinogenic risk may exceed the threshold value of 1. Possible involvement of sea salt aerosol and desert dust long-range transport has also been assessed. These results may furnish databases on PM pollution of Greek cities as well as other Mediterranean urban centers with similar characteristics.  相似文献   

15.
The paucity of data on air pollution indices in Nigeria prompted us to commence a national screening exercise regarding particulate matter loads. Six potential megacities (Aba, Abuja, Lagos, Kano, Maiduguri, and Port-Harcourt) representing the six geographical zones in Nigeria were chosen for the study. Sampling was achieved using a ‘Gent’ stacked filter unit sampler capable of collecting fractions of particulate matter with sizes of <10-μm and <2.5-μm simultaneously. The mean values for PM10 are 550, 35, 87, 340, 246 and 130 μg m?3 while for PM2.5 the mean values are 100, 14, 25, 67, 20 and 30 μg m?3 respectively for Aba, Abuja, Lagos, Kano, Maiduguri, and Port-Harcourt. Except for Abuja, the daily PM10 mass loads exceeded the World Health Organization (WHO) guidelines daily limit where as the PM2.5 values were within the WHO guideline limit. Their correlation matrix result indicates that some PM2.5 fractions mass fractions were strongly correlated than the PM10 fractions probably due to their long range transport potentials. Further work is in progress to determine the elemental profiles of both particulate fractions collected.  相似文献   

16.
Indoor and outdoor air pollution is known to contribute to increased lung cancer incidence. This study is the first to address the contribution of home heating fuel and geographical course particulate matter (PM10) concentrations to lung cancer rates in New Hampshire, USA. First, Pearson correlation analysis and geographically weighted regression were used to investigate spatial relationships between outdoor PM10 and lung cancer rates. While the aforementioned analyses did not indicate a significant contribution of PM10 to lung cancer in the state, there was a trend towards a significant association in the northern and southwestern regions of the state. Second, case-control data were used to estimate the contributions of indoor pollution and secondhand smoke to the risk of lung cancer with adjustment for confounders. Increased risk was found among those who used wood or coal to heat their homes for more than 10 winters before the age of 18, with a significant increase in risk per winter. Resulting data suggest that further investigation of the relationship between heating-related air pollution levels and lung cancer risk is needed.  相似文献   

17.
Does air quality influence road safety? We estimate the effect of increased air pollution on the number of road traffic accidents in the United Kingdom between 2009 and 2014. To address concerns of spurious correlation we exploit atmospheric temperature inversions as a source of plausibly exogenous variation in daily air pollution levels. We find an increase of 0.3–0.6% in the number of vehicles involved in accidents per day for each additional 1 μg/m3 of PM2.5. The finding suggests that less safe roads may present a large and previously overlooked cost of air pollution. The results are robust to a number of specifications and across various sub-samples.  相似文献   

18.
随着我国社会经济和城市化的快速发展,大气颗粒物是影响我国城市空气质量的首要污染物,大气细颗粒物污染已严重威胁我国居民健康。本文简要综述了PM2.5诱导的氧化应激和炎症反应在糖尿病的发生和发展中的分子作用机制。  相似文献   

19.
以东莞市5个镇区为研究对象,采集电镀企业周边大气样品,分析了样品中重金属(包括As、Co、Cd、Cr、Cu、Mn、Ni、Pb、Sb、V、Zn和Hg)的含量分布,使用富集因子(enrich factor)、地累积指数(index of geoaccumulation)、Hakanson法和美国国家环境保护局(US EPA)的人体暴露健康风险评价模型,对PM_(2.5)、PM_(10)、总悬浮颗粒物(TSP)中重金属进行人体健康风险评价。结果表明,PM_(2.5)、PM_(10)和TSP中As、Cd和Cr平均浓度皆超标。Cr、Ni和V元素在3种颗粒物中非富集,主要为自然源;As、Co、Cu、Pb和Zn,可能来源于自然源和叠加的工业污染。Cd、Hg和Sb浓度受人为污染影响严重。Cd、Sb、Cu、Zn、Pb为生物可利用元素(K>0.6),在环境中的可迁移性高且易于被生物体和人体吸收。Mn元素的非致癌风险值较其他重金属要高1~4个数量级,且儿童的非致癌暴露风险值HQ均高于成人的。3种颗粒物中重金属元素通过呼吸吸入途径产生的非致癌风险HI值均高于人体可接受的上限1.0,其主要贡献来源于Mn的影响,研究区非致癌风险较为严重。除PM_(10)中Co元素和TSP中Co、Cr的成人致癌风险CR值大于10-4之外,其余大部分重金属元素通过呼吸途径产生的致癌风险CR值均在可接受范围之内,此外,3种颗粒物中的成人的致癌暴露风险值CRT均高于儿童的CRT值,并且除了PM_(2.5)中儿童的重金属致癌暴露风险CRT值(4.70E-05)低于人体可接受范围的上限(10-4),其余CRT值均高于10-4,致癌风险较为严重。  相似文献   

20.
Air pollution has a deleterious impact on public health and the environment. There is few knowledge on the effect of air pollution on terrestrial microbial communities, despite the major role of microbes in ecosystems. Here, we designed an in situ trial ecosystem to assess the impact of moderate atmospheric pollution, below World Health Organization (WHO) thresholds, on an indigenous microbial communities, including bacteria, fungi, ciliates, algae, cyanobacteria, testate amoebae, rotifers and nematodes, extracted from terrestrial bryophytes. These micro-ecosystems were placed at a rural, an urban and an industrial site in France and were thus exposed to various levels of nitrogen dioxide (NO2), from 6.6–67.9 μg·m?3, and particulate matter, from 0.7–7.9 μg·m?3. Microbial analysis was performed by microscopy. We determined atmospheric temperature, relative humidity and particulate matter with diameter lower than 10 µm (PM10), Cu, Cr, Fe, Ni, Pb, Zn in PM10, and (NO2). Results show a significant impact of chronic moderate exposure to NO2 and copper Cu-associated particulate matter on the global microbial network complexity. This is evidenced by a loss of about 40 % of microbial co-occurrence links during incubation. Most lost microbial links are ecologically positive links. Moreover, most changes in community co-occurrence networks are related to testate amoebae, a major top predator of microbes. Overall, our findings demonstrate that air pollution can have strong deleterious effects on microbial interactions, even at levels below WHO thresholds.  相似文献   

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