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Mobility of heavy metals from tailings to stream waters in a mining activity contaminated site 总被引:6,自引:0,他引:6
In this paper the results of a recent characterization of Rio Piscinas (SW of Sardinia, Italy) hydrological basin are reported. In such area (about 50 km2), previous mining activities caused a serious heavy metal contamination of surface waters, groundwater, soils and biota. Acid mine drainage phenomena were observed in the area. The main sources of contamination are the tailings stored in mine tunnels and abandoned along fluvial banks. A methodological approach was adopted in order to identify relations between tailings and water contamination. Representative samples of tailings and stream sediments samples were collected. XRD analyses were performed for mineralogical characterization, while acid digestion was carried out for determining metal contents. Batch sequential leaching tests were performed in order to assess metal mobility. Also groundwater and stream water were sampled in specific locations and suitably characterized. All information collected allowed the understanding of the effect of tailings on water contamination, thus contributing to the qualitative prediction of pollution evolution on the basis of metal mobility. Finally, a potential remediation strategy of stream water is proposed. 相似文献
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Changes of copper speciation in maize rhizosphere soil 总被引:1,自引:0,他引:1
Tao S Chen YJ Xu FL Cao J Li BG 《Environmental pollution (Barking, Essex : 1987)》2003,122(3):447-454
Chemical forms of copper in the rhizosphere and bulk soil of maize were investigated using rhizobox cultivation and sequential extraction techniques. The copper accumulations were also determined. The results demonstrated that there were continuous changes in copper fractionation within the maize rhizosphere. Initially, the amount of exchangeable copper increased before dropping below the initial level after 40 days or so. Carbonate associated copper followed a similar trend of change, but with a slower pace than the exchangeable copper. The increase in carbonate associated copper only become evident after 30 days, with the net loss occurring after 60 days. There were also initial increases in oxide bound copper as well as decreases in the organic matter associated copper, both followed by a turnover after 40-50 days. The accumulation of copper in the maize plant was found to be biomass dependent. The amount of accumulated copper absorbed in the plant material exceeded the initial quantity of the exchangeable copper in the soil, revealing a transformation from less bioavailable to more bioavailable fractions. During cultivation, decreases in redox potential and increases in pH, dissolved organic carbon (DOC), and microbial activity in the maize rhizosphere were observed. The change in copper speciation may result from root-induced changes in DOC, redox potential, and microbial activity in the rhizosphere. 相似文献
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采用Oasis HLB柱固相萃取的前处理技术,以气相色谱质谱联用仪(GC/MS)的分析方法,对我国北方永定河上游黑土洼人工湿地中多环芳烃污染的特征以及分布规律进行了研究.结果表明,该湿地系统以低环数多环芳烃污染为主,其中浓度最高的是菲和蒽,未检出高环数(5环、6环)多环芳烃.通过比较进水和出水的浓度,湿地系统总体上不能有效去除进水中的多环芳烃.但是比较不同工艺单元进出水浓度,复氧、植物根系及微生物等均影响到多环芳烃的去除效果,去除率在28%~65%之间. 相似文献
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Status of trace elements in paddy soil and sediment in Taihu Lake region 总被引:14,自引:0,他引:14
Thirteen paddy soil profiles and river sediments which are sources of irrigation water were collected around the Taihu Lake, and the trace elements were estimated. The content of La and Ce in paddy soil and sediment were 39.3 and 68.6 mg/kg soil and 36.9 and 65.1 mg/kg soil, being within the range of background values. The values for Pb, Cu, Ni, Cr, Co, Mn, Zn, Se in paddy soil were 23.3, 27.8, 25.5, 63.5, 10.2, 386, 68.7 and 0.25 mg/kg soil respectively, all below the national permission level. There was a decline of Zn in paddy soil. Some of the river sediments were seriously polluted. The river in Yangjin site was most contaminated with 5.47 g Cu/kg and 7.4 g Zn/kg. The high concentration of Pb and Ni also was observed in this sediment. River in Weitang, Huashi, Xinzhuang and Meiyan were contaminated with Pb, Cu and Ni to some extent. Zn, Cu and Pb were the main pollutants in present experiment sites. The fast development of village/township industries have caused severe environmental pollution in the Taihu Lake region, especially irrigation river sediments. Se content in plant and seed was 0.04 and 0.03 mg/kg respectively, showed Se-deficiency in paddy soil in the Taihu Lake region. 相似文献
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Fu Li Chen Yi Yang Xinyi Yang Zuyao Liu Sha Pei Lei Feng Baixiang Cao Ganxiang Liu Xin Lin Hualiang Li Xing Ye Yufeng Zhang Bo Sun Jiufeng Xu Xiaojun Liu Tao Ma Wenjun 《Environmental science and pollution research international》2019,26(20):20137-20147
Environmental Science and Pollution Research - Fetal growth has been demonstrated to be an important predictor of perinatal and postnatal health. Although the effects of maternal exposure to air... 相似文献
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基于层次分析法的再生水补给型城市河湖水生态修复技术评价指标体系及其应用 总被引:1,自引:0,他引:1
由于城市水资源严重紧缺,再生水作为补给城市河湖景观水体的重要水源,用量逐年加大,随之带来的水环境问题也引起关注,往往需要采用适宜的技术和工程改善水质。然而对于现有的生态修复技术和工程,缺少相应的评价方法和指标体系对其修复效果和工程技术进行综合有效的评估。通过大量的文献及实地调研,结合再生水补给型城市河湖的特点,构建了包含环境效益、技术管理与维护及社会经济功能3个系统、7个准则和19个指标的再生水补给型城市河湖水生态修复技术评价指标体系,采用群组决策的层次分析法(AHP)确定各指标的权重,重要性排序前5位的指标依次是:藻类多样性、水生植物覆盖度、DO、TLI、PI(COD)。以北京市陶然亭湖水生态修复工程为例进行综合评价,研究结果表明,现阶段陶然亭湖水生态修复工程综合评分为3.35分,评价结果属于良。陶然亭湖经过水体生态修复后,水生态系统结构较好恢复;所选工程技术适宜;人员及经济投入适中;对周边环境产生较大正面影响;工程可优后进行推广 相似文献
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Ka-Hei Lui Wen-Ting Dai Chi-Sing Chan Linwei Tian Bo-Fu Ning Yiping Zhou Xiaolin Song Bei Wang Jinwen Li Jun-Ji Cao Shun-Cheng Lee Kin-Fai Ho 《Environmental science and pollution research international》2017,24(21):17500-17510
Airborne carbonyls were characterized from emitted indoor coal combustion. Samples were collected in Xuanwei (Yunnan Province), a region in China with a high rate of lung cancer. Eleven of 19 types of samples (58%) demonstrated formaldehyde concentrations higher than the World Health Organization exposure limit (a 30-min average of 100 μg m?3). Different positive significant correlations between glyoxal/methylglyoxal and formaldehyde/acetaldehyde concentrations were observed, suggesting possible different characteristics in emissions between two pairs of carbonyl compounds. A sample in the highest inhalation risk shows 29.2 times higher risk than the lowest sample, suggesting different coal sampling locations could contribute to the variation of inhalation risk. Inhabitants in Xuanwei also tend to spend more time cooking and more days per year indoors than the national average. The calculated cancer risk ranged from 2.2–63 × 10?5, which shows 13 types of samples at high-risk level. Cumulative effect in combination with different carbonyls could have contributed to the additive actual inhalation cancer risk. There is a need to explicitly address the health effects of environmentally relevant doses, considering life-long exposure in indoor dwellings. 相似文献